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Origin of uranium isotope variations in early solar nebula condensates
High-temperature condensates found in meteorites display uranium isotopic variations ((235)U/(238)U), which complicate dating the solar system’s formation and whose origin remains mysterious. It is possible that these variations are due to the decay of the short-lived radionuclide (247)Cm (t(1/2) =...
Autores principales: | , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
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American Association for the Advancement of Science
2016
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4783122/ https://www.ncbi.nlm.nih.gov/pubmed/26973874 http://dx.doi.org/10.1126/sciadv.1501400 |
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author | Tissot, François L. H. Dauphas, Nicolas Grossman, Lawrence |
author_facet | Tissot, François L. H. Dauphas, Nicolas Grossman, Lawrence |
author_sort | Tissot, François L. H. |
collection | PubMed |
description | High-temperature condensates found in meteorites display uranium isotopic variations ((235)U/(238)U), which complicate dating the solar system’s formation and whose origin remains mysterious. It is possible that these variations are due to the decay of the short-lived radionuclide (247)Cm (t(1/2) = 15.6 My) into (235)U, but they could also be due to uranium kinetic isotopic fractionation during condensation. We report uranium isotope measurements of meteoritic refractory inclusions that reveal excesses of (235)U reaching ~+6% relative to average solar system composition, which can only be due to the decay of (247)Cm. This allows us to constrain the (247)Cm/(235)U ratio at solar system formation to (1.1 ± 0.3) × 10(−4). This value provides new clues on the universality of the nucleosynthetic r-process of rapid neutron capture. |
format | Online Article Text |
id | pubmed-4783122 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2016 |
publisher | American Association for the Advancement of Science |
record_format | MEDLINE/PubMed |
spelling | pubmed-47831222016-03-11 Origin of uranium isotope variations in early solar nebula condensates Tissot, François L. H. Dauphas, Nicolas Grossman, Lawrence Sci Adv Research Articles High-temperature condensates found in meteorites display uranium isotopic variations ((235)U/(238)U), which complicate dating the solar system’s formation and whose origin remains mysterious. It is possible that these variations are due to the decay of the short-lived radionuclide (247)Cm (t(1/2) = 15.6 My) into (235)U, but they could also be due to uranium kinetic isotopic fractionation during condensation. We report uranium isotope measurements of meteoritic refractory inclusions that reveal excesses of (235)U reaching ~+6% relative to average solar system composition, which can only be due to the decay of (247)Cm. This allows us to constrain the (247)Cm/(235)U ratio at solar system formation to (1.1 ± 0.3) × 10(−4). This value provides new clues on the universality of the nucleosynthetic r-process of rapid neutron capture. American Association for the Advancement of Science 2016-03-04 /pmc/articles/PMC4783122/ /pubmed/26973874 http://dx.doi.org/10.1126/sciadv.1501400 Text en Copyright © 2016, The Authors http://creativecommons.org/licenses/by-nc/4.0/ This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (http://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited. |
spellingShingle | Research Articles Tissot, François L. H. Dauphas, Nicolas Grossman, Lawrence Origin of uranium isotope variations in early solar nebula condensates |
title | Origin of uranium isotope variations in early solar nebula condensates |
title_full | Origin of uranium isotope variations in early solar nebula condensates |
title_fullStr | Origin of uranium isotope variations in early solar nebula condensates |
title_full_unstemmed | Origin of uranium isotope variations in early solar nebula condensates |
title_short | Origin of uranium isotope variations in early solar nebula condensates |
title_sort | origin of uranium isotope variations in early solar nebula condensates |
topic | Research Articles |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4783122/ https://www.ncbi.nlm.nih.gov/pubmed/26973874 http://dx.doi.org/10.1126/sciadv.1501400 |
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