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Origin of uranium isotope variations in early solar nebula condensates

High-temperature condensates found in meteorites display uranium isotopic variations ((235)U/(238)U), which complicate dating the solar system’s formation and whose origin remains mysterious. It is possible that these variations are due to the decay of the short-lived radionuclide (247)Cm (t(1/2) =...

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Autores principales: Tissot, François L. H., Dauphas, Nicolas, Grossman, Lawrence
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4783122/
https://www.ncbi.nlm.nih.gov/pubmed/26973874
http://dx.doi.org/10.1126/sciadv.1501400
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author Tissot, François L. H.
Dauphas, Nicolas
Grossman, Lawrence
author_facet Tissot, François L. H.
Dauphas, Nicolas
Grossman, Lawrence
author_sort Tissot, François L. H.
collection PubMed
description High-temperature condensates found in meteorites display uranium isotopic variations ((235)U/(238)U), which complicate dating the solar system’s formation and whose origin remains mysterious. It is possible that these variations are due to the decay of the short-lived radionuclide (247)Cm (t(1/2) = 15.6 My) into (235)U, but they could also be due to uranium kinetic isotopic fractionation during condensation. We report uranium isotope measurements of meteoritic refractory inclusions that reveal excesses of (235)U reaching ~+6% relative to average solar system composition, which can only be due to the decay of (247)Cm. This allows us to constrain the (247)Cm/(235)U ratio at solar system formation to (1.1 ± 0.3) × 10(−4). This value provides new clues on the universality of the nucleosynthetic r-process of rapid neutron capture.
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spelling pubmed-47831222016-03-11 Origin of uranium isotope variations in early solar nebula condensates Tissot, François L. H. Dauphas, Nicolas Grossman, Lawrence Sci Adv Research Articles High-temperature condensates found in meteorites display uranium isotopic variations ((235)U/(238)U), which complicate dating the solar system’s formation and whose origin remains mysterious. It is possible that these variations are due to the decay of the short-lived radionuclide (247)Cm (t(1/2) = 15.6 My) into (235)U, but they could also be due to uranium kinetic isotopic fractionation during condensation. We report uranium isotope measurements of meteoritic refractory inclusions that reveal excesses of (235)U reaching ~+6% relative to average solar system composition, which can only be due to the decay of (247)Cm. This allows us to constrain the (247)Cm/(235)U ratio at solar system formation to (1.1 ± 0.3) × 10(−4). This value provides new clues on the universality of the nucleosynthetic r-process of rapid neutron capture. American Association for the Advancement of Science 2016-03-04 /pmc/articles/PMC4783122/ /pubmed/26973874 http://dx.doi.org/10.1126/sciadv.1501400 Text en Copyright © 2016, The Authors http://creativecommons.org/licenses/by-nc/4.0/ This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (http://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
spellingShingle Research Articles
Tissot, François L. H.
Dauphas, Nicolas
Grossman, Lawrence
Origin of uranium isotope variations in early solar nebula condensates
title Origin of uranium isotope variations in early solar nebula condensates
title_full Origin of uranium isotope variations in early solar nebula condensates
title_fullStr Origin of uranium isotope variations in early solar nebula condensates
title_full_unstemmed Origin of uranium isotope variations in early solar nebula condensates
title_short Origin of uranium isotope variations in early solar nebula condensates
title_sort origin of uranium isotope variations in early solar nebula condensates
topic Research Articles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4783122/
https://www.ncbi.nlm.nih.gov/pubmed/26973874
http://dx.doi.org/10.1126/sciadv.1501400
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