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Achieving High Performance in AC-Field Driven Organic Light Sources

Charge balance in organic light emitting structures is essential to simultaneously achieving high brightness and high efficiency. In DC-driven organic light emitting devices (OLEDs), this is relatively straight forward. However, in the newly emerging, capacitive, field-activated AC-driven organic de...

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Autores principales: Xu, Junwei, Carroll, David L., Smith, Gregory M., Dun, Chaochao, Cui, Yue
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4827088/
https://www.ncbi.nlm.nih.gov/pubmed/27063414
http://dx.doi.org/10.1038/srep24116
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author Xu, Junwei
Carroll, David L.
Smith, Gregory M.
Dun, Chaochao
Cui, Yue
author_facet Xu, Junwei
Carroll, David L.
Smith, Gregory M.
Dun, Chaochao
Cui, Yue
author_sort Xu, Junwei
collection PubMed
description Charge balance in organic light emitting structures is essential to simultaneously achieving high brightness and high efficiency. In DC-driven organic light emitting devices (OLEDs), this is relatively straight forward. However, in the newly emerging, capacitive, field-activated AC-driven organic devices, charge balance can be a challenge. In this work we introduce the concept of gating the compensation charge in AC-driven organic devices and demonstrate that this can result in exceptional increases in device performance. To do this we replace the insulator layer in a typical field-activated organic light emitting device with a nanostructured, wide band gap semiconductor layer. This layer acts as a gate between the emitter layer and the voltage contact. Time resolved device characterization shows that, at high-frequencies (over 40 kHz), the semiconductor layer allows for charge accumulation in the forward bias, light generating part of the AC cycle and charge compensation in the negative, quiescent part of the AC cycle. Such gated AC organic devices can achieve a non-output coupled luminance of 25,900 cd/m(2) with power efficiencies that exceed both the insulator-based AC devices and OLEDs using the same emitters. This work clearly demonstrates that by realizing balanced management of charge, AC-driven organic light emitting devices may well be able to rival today’s OLEDs in performance.
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spelling pubmed-48270882016-04-19 Achieving High Performance in AC-Field Driven Organic Light Sources Xu, Junwei Carroll, David L. Smith, Gregory M. Dun, Chaochao Cui, Yue Sci Rep Article Charge balance in organic light emitting structures is essential to simultaneously achieving high brightness and high efficiency. In DC-driven organic light emitting devices (OLEDs), this is relatively straight forward. However, in the newly emerging, capacitive, field-activated AC-driven organic devices, charge balance can be a challenge. In this work we introduce the concept of gating the compensation charge in AC-driven organic devices and demonstrate that this can result in exceptional increases in device performance. To do this we replace the insulator layer in a typical field-activated organic light emitting device with a nanostructured, wide band gap semiconductor layer. This layer acts as a gate between the emitter layer and the voltage contact. Time resolved device characterization shows that, at high-frequencies (over 40 kHz), the semiconductor layer allows for charge accumulation in the forward bias, light generating part of the AC cycle and charge compensation in the negative, quiescent part of the AC cycle. Such gated AC organic devices can achieve a non-output coupled luminance of 25,900 cd/m(2) with power efficiencies that exceed both the insulator-based AC devices and OLEDs using the same emitters. This work clearly demonstrates that by realizing balanced management of charge, AC-driven organic light emitting devices may well be able to rival today’s OLEDs in performance. Nature Publishing Group 2016-04-11 /pmc/articles/PMC4827088/ /pubmed/27063414 http://dx.doi.org/10.1038/srep24116 Text en Copyright © 2016, Macmillan Publishers Limited http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Xu, Junwei
Carroll, David L.
Smith, Gregory M.
Dun, Chaochao
Cui, Yue
Achieving High Performance in AC-Field Driven Organic Light Sources
title Achieving High Performance in AC-Field Driven Organic Light Sources
title_full Achieving High Performance in AC-Field Driven Organic Light Sources
title_fullStr Achieving High Performance in AC-Field Driven Organic Light Sources
title_full_unstemmed Achieving High Performance in AC-Field Driven Organic Light Sources
title_short Achieving High Performance in AC-Field Driven Organic Light Sources
title_sort achieving high performance in ac-field driven organic light sources
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4827088/
https://www.ncbi.nlm.nih.gov/pubmed/27063414
http://dx.doi.org/10.1038/srep24116
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