Incommensurate spin correlations in highly oxidized cobaltates La(2−x)Sr(x)CoO(4)

We observe quasi-static incommensurate magnetic peaks in neutron scattering experiments on layered cobalt oxides La(2−x)Sr(x)CoO(4) with high Co oxidation states that have been reported to be paramagnetic. This enables us to measure the magnetic excitations in this highly hole-doped incommensurate regime and compare our results with those found in the low-doped incommensurate regime that exhibit hourglass magnetic spectra. The hourglass shape of magnetic excitations completely disappears given a high Sr doping. Moreover, broad low-energy excitations are found, which are not centered at the incommensurate magnetic peak positions but around the quarter-integer values that are typically exhibited by excitations in the checkerboard charge ordered phase. Our findings suggest that the strong inter-site exchange interactions in the undoped islands are critical for the emergence of hourglass spectra in the incommensurate magnetic phases of La(2−x)Sr(x)CoO(4).