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Broadband Tunable, Polarization-Selective and Directional Emission of (6,5) Carbon Nanotubes Coupled to Plasmonic Crystals

[Image: see text] We demonstrate broadband tunability of light emission from dense (6,5) single-walled carbon nanotube thin films via efficient coupling to periodic arrays of gold nanodisks that support surface lattice resonances (SLRs). We thus eliminate the need to select single-walled carbon nano...

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Autores principales: Zakharko, Yuriy, Graf, Arko, Schießl, Stefan P., Hähnlein, Bernd, Pezoldt, Jörg, Gather, Malte C., Zaumseil, Jana
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2016
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4867777/
https://www.ncbi.nlm.nih.gov/pubmed/27105249
http://dx.doi.org/10.1021/acs.nanolett.6b00827
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author Zakharko, Yuriy
Graf, Arko
Schießl, Stefan P.
Hähnlein, Bernd
Pezoldt, Jörg
Gather, Malte C.
Zaumseil, Jana
author_facet Zakharko, Yuriy
Graf, Arko
Schießl, Stefan P.
Hähnlein, Bernd
Pezoldt, Jörg
Gather, Malte C.
Zaumseil, Jana
author_sort Zakharko, Yuriy
collection PubMed
description [Image: see text] We demonstrate broadband tunability of light emission from dense (6,5) single-walled carbon nanotube thin films via efficient coupling to periodic arrays of gold nanodisks that support surface lattice resonances (SLRs). We thus eliminate the need to select single-walled carbon nanotubes (SWNTs) with different chiralities to obtain narrow linewidth emission at specific near-infrared wavelengths. Emission from these hybrid films is spectrally narrow (20–40 meV) yet broadly tunable (∼1000–1500 nm) and highly directional (divergence <1.5°). In addition, SLR scattering renders the emission highly polarized, even though the SWNTs are randomly distributed. Numerical simulations are applied to correlate the increased local electric fields around the nanodisks with the observed enhancement of directional emission. The ability to control the emission properties of a single type of near-infrared emitting SWNTs over a wide range of wavelengths will enable application of carbon nanotubes in multifunctional photonic devices.
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spelling pubmed-48677772016-05-17 Broadband Tunable, Polarization-Selective and Directional Emission of (6,5) Carbon Nanotubes Coupled to Plasmonic Crystals Zakharko, Yuriy Graf, Arko Schießl, Stefan P. Hähnlein, Bernd Pezoldt, Jörg Gather, Malte C. Zaumseil, Jana Nano Lett [Image: see text] We demonstrate broadband tunability of light emission from dense (6,5) single-walled carbon nanotube thin films via efficient coupling to periodic arrays of gold nanodisks that support surface lattice resonances (SLRs). We thus eliminate the need to select single-walled carbon nanotubes (SWNTs) with different chiralities to obtain narrow linewidth emission at specific near-infrared wavelengths. Emission from these hybrid films is spectrally narrow (20–40 meV) yet broadly tunable (∼1000–1500 nm) and highly directional (divergence <1.5°). In addition, SLR scattering renders the emission highly polarized, even though the SWNTs are randomly distributed. Numerical simulations are applied to correlate the increased local electric fields around the nanodisks with the observed enhancement of directional emission. The ability to control the emission properties of a single type of near-infrared emitting SWNTs over a wide range of wavelengths will enable application of carbon nanotubes in multifunctional photonic devices. American Chemical Society 2016-04-22 2016-05-11 /pmc/articles/PMC4867777/ /pubmed/27105249 http://dx.doi.org/10.1021/acs.nanolett.6b00827 Text en Copyright © 2016 American Chemical Society This is an open access article published under an ACS AuthorChoice License (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html) , which permits copying and redistribution of the article or any adaptations for non-commercial purposes.
spellingShingle Zakharko, Yuriy
Graf, Arko
Schießl, Stefan P.
Hähnlein, Bernd
Pezoldt, Jörg
Gather, Malte C.
Zaumseil, Jana
Broadband Tunable, Polarization-Selective and Directional Emission of (6,5) Carbon Nanotubes Coupled to Plasmonic Crystals
title Broadband Tunable, Polarization-Selective and Directional Emission of (6,5) Carbon Nanotubes Coupled to Plasmonic Crystals
title_full Broadband Tunable, Polarization-Selective and Directional Emission of (6,5) Carbon Nanotubes Coupled to Plasmonic Crystals
title_fullStr Broadband Tunable, Polarization-Selective and Directional Emission of (6,5) Carbon Nanotubes Coupled to Plasmonic Crystals
title_full_unstemmed Broadband Tunable, Polarization-Selective and Directional Emission of (6,5) Carbon Nanotubes Coupled to Plasmonic Crystals
title_short Broadband Tunable, Polarization-Selective and Directional Emission of (6,5) Carbon Nanotubes Coupled to Plasmonic Crystals
title_sort broadband tunable, polarization-selective and directional emission of (6,5) carbon nanotubes coupled to plasmonic crystals
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4867777/
https://www.ncbi.nlm.nih.gov/pubmed/27105249
http://dx.doi.org/10.1021/acs.nanolett.6b00827
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