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Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy
The dynamic behaviour of atomic-size disarrangements of atoms—point defects (self-interstitial atoms (SIAs) and vacancies)—often governs the macroscopic properties of crystalline materials. However, the dynamics of SIAs have not been fully uncovered because of their rapid migration. Using a combinat...
Autores principales: | , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group
2016
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4869112/ https://www.ncbi.nlm.nih.gov/pubmed/27185352 http://dx.doi.org/10.1038/srep26099 |
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author | Amino, T. Arakawa, K. Mori, H. |
author_facet | Amino, T. Arakawa, K. Mori, H. |
author_sort | Amino, T. |
collection | PubMed |
description | The dynamic behaviour of atomic-size disarrangements of atoms—point defects (self-interstitial atoms (SIAs) and vacancies)—often governs the macroscopic properties of crystalline materials. However, the dynamics of SIAs have not been fully uncovered because of their rapid migration. Using a combination of high-voltage transmission electron microscopy and exhaustive kinetic Monte Carlo simulations, we determine the dynamics of the rapidly migrating SIAs from the formation process of the nanoscale SIA clusters in tungsten as a typical body-centred cubic (BCC) structure metal under the constant-rate production of both types of point defects with high-energy electron irradiation, which must reflect the dynamics of individual SIAs. We reveal that the migration dimension of SIAs is not three-dimensional (3D) but one-dimensional (1D). This result overturns the long-standing and well-accepted view of SIAs in BCC metals and supports recent results obtained by ab-initio simulations. The SIA dynamics clarified here will be one of the key factors to accurately predict the lifetimes of nuclear fission and fusion materials. |
format | Online Article Text |
id | pubmed-4869112 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2016 |
publisher | Nature Publishing Group |
record_format | MEDLINE/PubMed |
spelling | pubmed-48691122016-06-01 Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy Amino, T. Arakawa, K. Mori, H. Sci Rep Article The dynamic behaviour of atomic-size disarrangements of atoms—point defects (self-interstitial atoms (SIAs) and vacancies)—often governs the macroscopic properties of crystalline materials. However, the dynamics of SIAs have not been fully uncovered because of their rapid migration. Using a combination of high-voltage transmission electron microscopy and exhaustive kinetic Monte Carlo simulations, we determine the dynamics of the rapidly migrating SIAs from the formation process of the nanoscale SIA clusters in tungsten as a typical body-centred cubic (BCC) structure metal under the constant-rate production of both types of point defects with high-energy electron irradiation, which must reflect the dynamics of individual SIAs. We reveal that the migration dimension of SIAs is not three-dimensional (3D) but one-dimensional (1D). This result overturns the long-standing and well-accepted view of SIAs in BCC metals and supports recent results obtained by ab-initio simulations. The SIA dynamics clarified here will be one of the key factors to accurately predict the lifetimes of nuclear fission and fusion materials. Nature Publishing Group 2016-05-17 /pmc/articles/PMC4869112/ /pubmed/27185352 http://dx.doi.org/10.1038/srep26099 Text en Copyright © 2016, Macmillan Publishers Limited http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ |
spellingShingle | Article Amino, T. Arakawa, K. Mori, H. Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy |
title | Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy |
title_full | Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy |
title_fullStr | Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy |
title_full_unstemmed | Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy |
title_short | Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy |
title_sort | detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4869112/ https://www.ncbi.nlm.nih.gov/pubmed/27185352 http://dx.doi.org/10.1038/srep26099 |
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