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Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy

The dynamic behaviour of atomic-size disarrangements of atoms—point defects (self-interstitial atoms (SIAs) and vacancies)—often governs the macroscopic properties of crystalline materials. However, the dynamics of SIAs have not been fully uncovered because of their rapid migration. Using a combinat...

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Autores principales: Amino, T., Arakawa, K., Mori, H.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4869112/
https://www.ncbi.nlm.nih.gov/pubmed/27185352
http://dx.doi.org/10.1038/srep26099
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author Amino, T.
Arakawa, K.
Mori, H.
author_facet Amino, T.
Arakawa, K.
Mori, H.
author_sort Amino, T.
collection PubMed
description The dynamic behaviour of atomic-size disarrangements of atoms—point defects (self-interstitial atoms (SIAs) and vacancies)—often governs the macroscopic properties of crystalline materials. However, the dynamics of SIAs have not been fully uncovered because of their rapid migration. Using a combination of high-voltage transmission electron microscopy and exhaustive kinetic Monte Carlo simulations, we determine the dynamics of the rapidly migrating SIAs from the formation process of the nanoscale SIA clusters in tungsten as a typical body-centred cubic (BCC) structure metal under the constant-rate production of both types of point defects with high-energy electron irradiation, which must reflect the dynamics of individual SIAs. We reveal that the migration dimension of SIAs is not three-dimensional (3D) but one-dimensional (1D). This result overturns the long-standing and well-accepted view of SIAs in BCC metals and supports recent results obtained by ab-initio simulations. The SIA dynamics clarified here will be one of the key factors to accurately predict the lifetimes of nuclear fission and fusion materials.
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spelling pubmed-48691122016-06-01 Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy Amino, T. Arakawa, K. Mori, H. Sci Rep Article The dynamic behaviour of atomic-size disarrangements of atoms—point defects (self-interstitial atoms (SIAs) and vacancies)—often governs the macroscopic properties of crystalline materials. However, the dynamics of SIAs have not been fully uncovered because of their rapid migration. Using a combination of high-voltage transmission electron microscopy and exhaustive kinetic Monte Carlo simulations, we determine the dynamics of the rapidly migrating SIAs from the formation process of the nanoscale SIA clusters in tungsten as a typical body-centred cubic (BCC) structure metal under the constant-rate production of both types of point defects with high-energy electron irradiation, which must reflect the dynamics of individual SIAs. We reveal that the migration dimension of SIAs is not three-dimensional (3D) but one-dimensional (1D). This result overturns the long-standing and well-accepted view of SIAs in BCC metals and supports recent results obtained by ab-initio simulations. The SIA dynamics clarified here will be one of the key factors to accurately predict the lifetimes of nuclear fission and fusion materials. Nature Publishing Group 2016-05-17 /pmc/articles/PMC4869112/ /pubmed/27185352 http://dx.doi.org/10.1038/srep26099 Text en Copyright © 2016, Macmillan Publishers Limited http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Amino, T.
Arakawa, K.
Mori, H.
Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy
title Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy
title_full Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy
title_fullStr Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy
title_full_unstemmed Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy
title_short Detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy
title_sort detection of one-dimensional migration of single self-interstitial atoms in tungsten using high-voltage electron microscopy
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4869112/
https://www.ncbi.nlm.nih.gov/pubmed/27185352
http://dx.doi.org/10.1038/srep26099
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