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The effect of acid–base clustering and ions on the growth of atmospheric nano-particles

The growth of freshly formed aerosol particles can be the bottleneck in their survival to cloud condensation nuclei. It is therefore crucial to understand how particles grow in the atmosphere. Insufficient experimental data has impeded a profound understanding of nano-particle growth under atmospher...

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Autores principales: Lehtipalo, Katrianne, Rondo, Linda, Kontkanen, Jenni, Schobesberger, Siegfried, Jokinen, Tuija, Sarnela, Nina, Kürten, Andreas, Ehrhart, Sebastian, Franchin, Alessandro, Nieminen, Tuomo, Riccobono, Francesco, Sipilä, Mikko, Yli-Juuti, Taina, Duplissy, Jonathan, Adamov, Alexey, Ahlm, Lars, Almeida, João, Amorim, Antonio, Bianchi, Federico, Breitenlechner, Martin, Dommen, Josef, Downard, Andrew J., Dunne, Eimear M., Flagan, Richard C., Guida, Roberto, Hakala, Jani, Hansel, Armin, Jud, Werner, Kangasluoma, Juha, Kerminen, Veli-Matti, Keskinen, Helmi, Kim, Jaeseok, Kirkby, Jasper, Kupc, Agnieszka, Kupiainen-Määttä, Oona, Laaksonen, Ari, Lawler, Michael J., Leiminger, Markus, Mathot, Serge, Olenius, Tinja, Ortega, Ismael K., Onnela, Antti, Petäjä, Tuukka, Praplan, Arnaud, Rissanen, Matti P., Ruuskanen, Taina, Santos, Filipe D., Schallhart, Simon, Schnitzhofer, Ralf, Simon, Mario, Smith, James N., Tröstl, Jasmin, Tsagkogeorgas, Georgios, Tomé, António, Vaattovaara, Petri, Vehkamäki, Hanna, Vrtala, Aron E., Wagner, Paul E., Williamson, Christina, Wimmer, Daniela, Winkler, Paul M., Virtanen, Annele, Donahue, Neil M., Carslaw, Kenneth S., Baltensperger, Urs, Riipinen, Ilona, Curtius, Joachim, Worsnop, Douglas R., Kulmala, Markku
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4876472/
https://www.ncbi.nlm.nih.gov/pubmed/27197574
http://dx.doi.org/10.1038/ncomms11594
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author Lehtipalo, Katrianne
Rondo, Linda
Kontkanen, Jenni
Schobesberger, Siegfried
Jokinen, Tuija
Sarnela, Nina
Kürten, Andreas
Ehrhart, Sebastian
Franchin, Alessandro
Nieminen, Tuomo
Riccobono, Francesco
Sipilä, Mikko
Yli-Juuti, Taina
Duplissy, Jonathan
Adamov, Alexey
Ahlm, Lars
Almeida, João
Amorim, Antonio
Bianchi, Federico
Breitenlechner, Martin
Dommen, Josef
Downard, Andrew J.
Dunne, Eimear M.
Flagan, Richard C.
Guida, Roberto
Hakala, Jani
Hansel, Armin
Jud, Werner
Kangasluoma, Juha
Kerminen, Veli-Matti
Keskinen, Helmi
Kim, Jaeseok
Kirkby, Jasper
Kupc, Agnieszka
Kupiainen-Määttä, Oona
Laaksonen, Ari
Lawler, Michael J.
Leiminger, Markus
Mathot, Serge
Olenius, Tinja
Ortega, Ismael K.
Onnela, Antti
Petäjä, Tuukka
Praplan, Arnaud
Rissanen, Matti P.
Ruuskanen, Taina
Santos, Filipe D.
Schallhart, Simon
Schnitzhofer, Ralf
Simon, Mario
Smith, James N.
Tröstl, Jasmin
Tsagkogeorgas, Georgios
Tomé, António
Vaattovaara, Petri
Vehkamäki, Hanna
Vrtala, Aron E.
Wagner, Paul E.
Williamson, Christina
Wimmer, Daniela
Winkler, Paul M.
Virtanen, Annele
Donahue, Neil M.
Carslaw, Kenneth S.
Baltensperger, Urs
Riipinen, Ilona
Curtius, Joachim
Worsnop, Douglas R.
Kulmala, Markku
author_facet Lehtipalo, Katrianne
Rondo, Linda
Kontkanen, Jenni
Schobesberger, Siegfried
Jokinen, Tuija
Sarnela, Nina
Kürten, Andreas
Ehrhart, Sebastian
Franchin, Alessandro
Nieminen, Tuomo
Riccobono, Francesco
Sipilä, Mikko
Yli-Juuti, Taina
Duplissy, Jonathan
Adamov, Alexey
Ahlm, Lars
Almeida, João
Amorim, Antonio
Bianchi, Federico
Breitenlechner, Martin
Dommen, Josef
Downard, Andrew J.
Dunne, Eimear M.
Flagan, Richard C.
Guida, Roberto
Hakala, Jani
Hansel, Armin
Jud, Werner
Kangasluoma, Juha
Kerminen, Veli-Matti
Keskinen, Helmi
Kim, Jaeseok
Kirkby, Jasper
Kupc, Agnieszka
Kupiainen-Määttä, Oona
Laaksonen, Ari
Lawler, Michael J.
Leiminger, Markus
Mathot, Serge
Olenius, Tinja
Ortega, Ismael K.
Onnela, Antti
Petäjä, Tuukka
Praplan, Arnaud
Rissanen, Matti P.
Ruuskanen, Taina
Santos, Filipe D.
Schallhart, Simon
Schnitzhofer, Ralf
Simon, Mario
Smith, James N.
Tröstl, Jasmin
Tsagkogeorgas, Georgios
Tomé, António
Vaattovaara, Petri
Vehkamäki, Hanna
Vrtala, Aron E.
Wagner, Paul E.
Williamson, Christina
Wimmer, Daniela
Winkler, Paul M.
Virtanen, Annele
Donahue, Neil M.
Carslaw, Kenneth S.
Baltensperger, Urs
Riipinen, Ilona
Curtius, Joachim
Worsnop, Douglas R.
Kulmala, Markku
author_sort Lehtipalo, Katrianne
collection PubMed
description The growth of freshly formed aerosol particles can be the bottleneck in their survival to cloud condensation nuclei. It is therefore crucial to understand how particles grow in the atmosphere. Insufficient experimental data has impeded a profound understanding of nano-particle growth under atmospheric conditions. Here we study nano-particle growth in the CLOUD (Cosmics Leaving OUtdoors Droplets) chamber, starting from the formation of molecular clusters. We present measured growth rates at sub-3 nm sizes with different atmospherically relevant concentrations of sulphuric acid, water, ammonia and dimethylamine. We find that atmospheric ions and small acid-base clusters, which are not generally accounted for in the measurement of sulphuric acid vapour, can participate in the growth process, leading to enhanced growth rates. The availability of compounds capable of stabilizing sulphuric acid clusters governs the magnitude of these effects and thus the exact growth mechanism. We bring these observations into a coherent framework and discuss their significance in the atmosphere.
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spelling pubmed-48764722016-06-02 The effect of acid–base clustering and ions on the growth of atmospheric nano-particles Lehtipalo, Katrianne Rondo, Linda Kontkanen, Jenni Schobesberger, Siegfried Jokinen, Tuija Sarnela, Nina Kürten, Andreas Ehrhart, Sebastian Franchin, Alessandro Nieminen, Tuomo Riccobono, Francesco Sipilä, Mikko Yli-Juuti, Taina Duplissy, Jonathan Adamov, Alexey Ahlm, Lars Almeida, João Amorim, Antonio Bianchi, Federico Breitenlechner, Martin Dommen, Josef Downard, Andrew J. Dunne, Eimear M. Flagan, Richard C. Guida, Roberto Hakala, Jani Hansel, Armin Jud, Werner Kangasluoma, Juha Kerminen, Veli-Matti Keskinen, Helmi Kim, Jaeseok Kirkby, Jasper Kupc, Agnieszka Kupiainen-Määttä, Oona Laaksonen, Ari Lawler, Michael J. Leiminger, Markus Mathot, Serge Olenius, Tinja Ortega, Ismael K. Onnela, Antti Petäjä, Tuukka Praplan, Arnaud Rissanen, Matti P. Ruuskanen, Taina Santos, Filipe D. Schallhart, Simon Schnitzhofer, Ralf Simon, Mario Smith, James N. Tröstl, Jasmin Tsagkogeorgas, Georgios Tomé, António Vaattovaara, Petri Vehkamäki, Hanna Vrtala, Aron E. Wagner, Paul E. Williamson, Christina Wimmer, Daniela Winkler, Paul M. Virtanen, Annele Donahue, Neil M. Carslaw, Kenneth S. Baltensperger, Urs Riipinen, Ilona Curtius, Joachim Worsnop, Douglas R. Kulmala, Markku Nat Commun Article The growth of freshly formed aerosol particles can be the bottleneck in their survival to cloud condensation nuclei. It is therefore crucial to understand how particles grow in the atmosphere. Insufficient experimental data has impeded a profound understanding of nano-particle growth under atmospheric conditions. Here we study nano-particle growth in the CLOUD (Cosmics Leaving OUtdoors Droplets) chamber, starting from the formation of molecular clusters. We present measured growth rates at sub-3 nm sizes with different atmospherically relevant concentrations of sulphuric acid, water, ammonia and dimethylamine. We find that atmospheric ions and small acid-base clusters, which are not generally accounted for in the measurement of sulphuric acid vapour, can participate in the growth process, leading to enhanced growth rates. The availability of compounds capable of stabilizing sulphuric acid clusters governs the magnitude of these effects and thus the exact growth mechanism. We bring these observations into a coherent framework and discuss their significance in the atmosphere. Nature Publishing Group 2016-05-20 /pmc/articles/PMC4876472/ /pubmed/27197574 http://dx.doi.org/10.1038/ncomms11594 Text en Copyright © 2016, Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved. http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article's Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Lehtipalo, Katrianne
Rondo, Linda
Kontkanen, Jenni
Schobesberger, Siegfried
Jokinen, Tuija
Sarnela, Nina
Kürten, Andreas
Ehrhart, Sebastian
Franchin, Alessandro
Nieminen, Tuomo
Riccobono, Francesco
Sipilä, Mikko
Yli-Juuti, Taina
Duplissy, Jonathan
Adamov, Alexey
Ahlm, Lars
Almeida, João
Amorim, Antonio
Bianchi, Federico
Breitenlechner, Martin
Dommen, Josef
Downard, Andrew J.
Dunne, Eimear M.
Flagan, Richard C.
Guida, Roberto
Hakala, Jani
Hansel, Armin
Jud, Werner
Kangasluoma, Juha
Kerminen, Veli-Matti
Keskinen, Helmi
Kim, Jaeseok
Kirkby, Jasper
Kupc, Agnieszka
Kupiainen-Määttä, Oona
Laaksonen, Ari
Lawler, Michael J.
Leiminger, Markus
Mathot, Serge
Olenius, Tinja
Ortega, Ismael K.
Onnela, Antti
Petäjä, Tuukka
Praplan, Arnaud
Rissanen, Matti P.
Ruuskanen, Taina
Santos, Filipe D.
Schallhart, Simon
Schnitzhofer, Ralf
Simon, Mario
Smith, James N.
Tröstl, Jasmin
Tsagkogeorgas, Georgios
Tomé, António
Vaattovaara, Petri
Vehkamäki, Hanna
Vrtala, Aron E.
Wagner, Paul E.
Williamson, Christina
Wimmer, Daniela
Winkler, Paul M.
Virtanen, Annele
Donahue, Neil M.
Carslaw, Kenneth S.
Baltensperger, Urs
Riipinen, Ilona
Curtius, Joachim
Worsnop, Douglas R.
Kulmala, Markku
The effect of acid–base clustering and ions on the growth of atmospheric nano-particles
title The effect of acid–base clustering and ions on the growth of atmospheric nano-particles
title_full The effect of acid–base clustering and ions on the growth of atmospheric nano-particles
title_fullStr The effect of acid–base clustering and ions on the growth of atmospheric nano-particles
title_full_unstemmed The effect of acid–base clustering and ions on the growth of atmospheric nano-particles
title_short The effect of acid–base clustering and ions on the growth of atmospheric nano-particles
title_sort effect of acid–base clustering and ions on the growth of atmospheric nano-particles
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4876472/
https://www.ncbi.nlm.nih.gov/pubmed/27197574
http://dx.doi.org/10.1038/ncomms11594
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