Cargando…

Size distribution of ring polymers

We present an exact solution for the distribution of sample averaged monomer to monomer distance of ring polymers. For non-interacting and local-interaction models these distributions correspond to the distribution of the area under the reflected Bessel bridge and the Bessel excursion respectively,...

Descripción completa

Detalles Bibliográficos
Autores principales: Medalion, Shlomi, Aghion, Erez, Meirovitch, Hagai, Barkai, Eli, Kessler, David A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4908590/
https://www.ncbi.nlm.nih.gov/pubmed/27302596
http://dx.doi.org/10.1038/srep27661
_version_ 1782437711590719488
author Medalion, Shlomi
Aghion, Erez
Meirovitch, Hagai
Barkai, Eli
Kessler, David A.
author_facet Medalion, Shlomi
Aghion, Erez
Meirovitch, Hagai
Barkai, Eli
Kessler, David A.
author_sort Medalion, Shlomi
collection PubMed
description We present an exact solution for the distribution of sample averaged monomer to monomer distance of ring polymers. For non-interacting and local-interaction models these distributions correspond to the distribution of the area under the reflected Bessel bridge and the Bessel excursion respectively, and are shown to be identical in dimension d ≥ 2, albeit with pronounced finite size effects at the critical dimension, d = 2. A symmetry of the problem reveals that dimension d and 4 − d are equivalent, thus the celebrated Airy distribution describing the areal distribution of the d = 1 Brownian excursion describes also a polymer in three dimensions. For a self-avoiding polymer in dimension d we find numerically that the fluctuations of the scaled averaged distance are nearly identical in dimension d = 2, 3 and are well described to a first approximation by the non-interacting excursion model in dimension 5.
format Online
Article
Text
id pubmed-4908590
institution National Center for Biotechnology Information
language English
publishDate 2016
publisher Nature Publishing Group
record_format MEDLINE/PubMed
spelling pubmed-49085902016-06-16 Size distribution of ring polymers Medalion, Shlomi Aghion, Erez Meirovitch, Hagai Barkai, Eli Kessler, David A. Sci Rep Article We present an exact solution for the distribution of sample averaged monomer to monomer distance of ring polymers. For non-interacting and local-interaction models these distributions correspond to the distribution of the area under the reflected Bessel bridge and the Bessel excursion respectively, and are shown to be identical in dimension d ≥ 2, albeit with pronounced finite size effects at the critical dimension, d = 2. A symmetry of the problem reveals that dimension d and 4 − d are equivalent, thus the celebrated Airy distribution describing the areal distribution of the d = 1 Brownian excursion describes also a polymer in three dimensions. For a self-avoiding polymer in dimension d we find numerically that the fluctuations of the scaled averaged distance are nearly identical in dimension d = 2, 3 and are well described to a first approximation by the non-interacting excursion model in dimension 5. Nature Publishing Group 2016-06-15 /pmc/articles/PMC4908590/ /pubmed/27302596 http://dx.doi.org/10.1038/srep27661 Text en Copyright © 2016, Macmillan Publishers Limited http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Medalion, Shlomi
Aghion, Erez
Meirovitch, Hagai
Barkai, Eli
Kessler, David A.
Size distribution of ring polymers
title Size distribution of ring polymers
title_full Size distribution of ring polymers
title_fullStr Size distribution of ring polymers
title_full_unstemmed Size distribution of ring polymers
title_short Size distribution of ring polymers
title_sort size distribution of ring polymers
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4908590/
https://www.ncbi.nlm.nih.gov/pubmed/27302596
http://dx.doi.org/10.1038/srep27661
work_keys_str_mv AT medalionshlomi sizedistributionofringpolymers
AT aghionerez sizedistributionofringpolymers
AT meirovitchhagai sizedistributionofringpolymers
AT barkaieli sizedistributionofringpolymers
AT kesslerdavida sizedistributionofringpolymers