Cargando…

Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography

Strong field photoelectron holography has been proposed as a means for interrogating the spatial and temporal information of electrons and ions in a dynamic system. After ionization, part of the electron wave packet may directly go to the detector (the reference wave), while another part may be driv...

Descripción completa

Detalles Bibliográficos
Autores principales: Song, Xiaohong, Lin, Cheng, Sheng, Zhihao, Liu, Peng, Chen, Zhangjin, Yang, Weifeng, Hu, Shilin, Lin, C. D., Chen, Jing
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4916607/
https://www.ncbi.nlm.nih.gov/pubmed/27329071
http://dx.doi.org/10.1038/srep28392
_version_ 1782438858571382784
author Song, Xiaohong
Lin, Cheng
Sheng, Zhihao
Liu, Peng
Chen, Zhangjin
Yang, Weifeng
Hu, Shilin
Lin, C. D.
Chen, Jing
author_facet Song, Xiaohong
Lin, Cheng
Sheng, Zhihao
Liu, Peng
Chen, Zhangjin
Yang, Weifeng
Hu, Shilin
Lin, C. D.
Chen, Jing
author_sort Song, Xiaohong
collection PubMed
description Strong field photoelectron holography has been proposed as a means for interrogating the spatial and temporal information of electrons and ions in a dynamic system. After ionization, part of the electron wave packet may directly go to the detector (the reference wave), while another part may be driven back and scatters off the ion(the signal wave). The interference hologram of the two waves may be used to extract target information embedded in the collision process. Unlike conventional optical holography, however, propagation of the electron wave packet is affected by the Coulomb potential as well as by the laser field. In addition, electrons are emitted over the whole laser pulse duration, thus multiple interferences may occur. In this work, we used a generalized quantum-trajectory Monte Carlo method to investigate the effect of Coulomb potential and the nonadiabatic subcycle ionization on the photoelectron hologram. We showed that photoelectron hologram can be well described only when the effect of nonadiabatic ionization is accounted for, and Coulomb potential can be neglected only in the tunnel ionization regime. Our results help paving the way for establishing photoelectron holography for probing spatial and dynamic properties of atoms and molecules.
format Online
Article
Text
id pubmed-4916607
institution National Center for Biotechnology Information
language English
publishDate 2016
publisher Nature Publishing Group
record_format MEDLINE/PubMed
spelling pubmed-49166072016-06-27 Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography Song, Xiaohong Lin, Cheng Sheng, Zhihao Liu, Peng Chen, Zhangjin Yang, Weifeng Hu, Shilin Lin, C. D. Chen, Jing Sci Rep Article Strong field photoelectron holography has been proposed as a means for interrogating the spatial and temporal information of electrons and ions in a dynamic system. After ionization, part of the electron wave packet may directly go to the detector (the reference wave), while another part may be driven back and scatters off the ion(the signal wave). The interference hologram of the two waves may be used to extract target information embedded in the collision process. Unlike conventional optical holography, however, propagation of the electron wave packet is affected by the Coulomb potential as well as by the laser field. In addition, electrons are emitted over the whole laser pulse duration, thus multiple interferences may occur. In this work, we used a generalized quantum-trajectory Monte Carlo method to investigate the effect of Coulomb potential and the nonadiabatic subcycle ionization on the photoelectron hologram. We showed that photoelectron hologram can be well described only when the effect of nonadiabatic ionization is accounted for, and Coulomb potential can be neglected only in the tunnel ionization regime. Our results help paving the way for establishing photoelectron holography for probing spatial and dynamic properties of atoms and molecules. Nature Publishing Group 2016-06-22 /pmc/articles/PMC4916607/ /pubmed/27329071 http://dx.doi.org/10.1038/srep28392 Text en Copyright © 2016, Macmillan Publishers Limited http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Song, Xiaohong
Lin, Cheng
Sheng, Zhihao
Liu, Peng
Chen, Zhangjin
Yang, Weifeng
Hu, Shilin
Lin, C. D.
Chen, Jing
Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography
title Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography
title_full Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography
title_fullStr Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography
title_full_unstemmed Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography
title_short Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography
title_sort unraveling nonadiabatic ionization and coulomb potential effect in strong-field photoelectron holography
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4916607/
https://www.ncbi.nlm.nih.gov/pubmed/27329071
http://dx.doi.org/10.1038/srep28392
work_keys_str_mv AT songxiaohong unravelingnonadiabaticionizationandcoulombpotentialeffectinstrongfieldphotoelectronholography
AT lincheng unravelingnonadiabaticionizationandcoulombpotentialeffectinstrongfieldphotoelectronholography
AT shengzhihao unravelingnonadiabaticionizationandcoulombpotentialeffectinstrongfieldphotoelectronholography
AT liupeng unravelingnonadiabaticionizationandcoulombpotentialeffectinstrongfieldphotoelectronholography
AT chenzhangjin unravelingnonadiabaticionizationandcoulombpotentialeffectinstrongfieldphotoelectronholography
AT yangweifeng unravelingnonadiabaticionizationandcoulombpotentialeffectinstrongfieldphotoelectronholography
AT hushilin unravelingnonadiabaticionizationandcoulombpotentialeffectinstrongfieldphotoelectronholography
AT lincd unravelingnonadiabaticionizationandcoulombpotentialeffectinstrongfieldphotoelectronholography
AT chenjing unravelingnonadiabaticionizationandcoulombpotentialeffectinstrongfieldphotoelectronholography