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Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography
Strong field photoelectron holography has been proposed as a means for interrogating the spatial and temporal information of electrons and ions in a dynamic system. After ionization, part of the electron wave packet may directly go to the detector (the reference wave), while another part may be driv...
Autores principales: | , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group
2016
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4916607/ https://www.ncbi.nlm.nih.gov/pubmed/27329071 http://dx.doi.org/10.1038/srep28392 |
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author | Song, Xiaohong Lin, Cheng Sheng, Zhihao Liu, Peng Chen, Zhangjin Yang, Weifeng Hu, Shilin Lin, C. D. Chen, Jing |
author_facet | Song, Xiaohong Lin, Cheng Sheng, Zhihao Liu, Peng Chen, Zhangjin Yang, Weifeng Hu, Shilin Lin, C. D. Chen, Jing |
author_sort | Song, Xiaohong |
collection | PubMed |
description | Strong field photoelectron holography has been proposed as a means for interrogating the spatial and temporal information of electrons and ions in a dynamic system. After ionization, part of the electron wave packet may directly go to the detector (the reference wave), while another part may be driven back and scatters off the ion(the signal wave). The interference hologram of the two waves may be used to extract target information embedded in the collision process. Unlike conventional optical holography, however, propagation of the electron wave packet is affected by the Coulomb potential as well as by the laser field. In addition, electrons are emitted over the whole laser pulse duration, thus multiple interferences may occur. In this work, we used a generalized quantum-trajectory Monte Carlo method to investigate the effect of Coulomb potential and the nonadiabatic subcycle ionization on the photoelectron hologram. We showed that photoelectron hologram can be well described only when the effect of nonadiabatic ionization is accounted for, and Coulomb potential can be neglected only in the tunnel ionization regime. Our results help paving the way for establishing photoelectron holography for probing spatial and dynamic properties of atoms and molecules. |
format | Online Article Text |
id | pubmed-4916607 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2016 |
publisher | Nature Publishing Group |
record_format | MEDLINE/PubMed |
spelling | pubmed-49166072016-06-27 Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography Song, Xiaohong Lin, Cheng Sheng, Zhihao Liu, Peng Chen, Zhangjin Yang, Weifeng Hu, Shilin Lin, C. D. Chen, Jing Sci Rep Article Strong field photoelectron holography has been proposed as a means for interrogating the spatial and temporal information of electrons and ions in a dynamic system. After ionization, part of the electron wave packet may directly go to the detector (the reference wave), while another part may be driven back and scatters off the ion(the signal wave). The interference hologram of the two waves may be used to extract target information embedded in the collision process. Unlike conventional optical holography, however, propagation of the electron wave packet is affected by the Coulomb potential as well as by the laser field. In addition, electrons are emitted over the whole laser pulse duration, thus multiple interferences may occur. In this work, we used a generalized quantum-trajectory Monte Carlo method to investigate the effect of Coulomb potential and the nonadiabatic subcycle ionization on the photoelectron hologram. We showed that photoelectron hologram can be well described only when the effect of nonadiabatic ionization is accounted for, and Coulomb potential can be neglected only in the tunnel ionization regime. Our results help paving the way for establishing photoelectron holography for probing spatial and dynamic properties of atoms and molecules. Nature Publishing Group 2016-06-22 /pmc/articles/PMC4916607/ /pubmed/27329071 http://dx.doi.org/10.1038/srep28392 Text en Copyright © 2016, Macmillan Publishers Limited http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ |
spellingShingle | Article Song, Xiaohong Lin, Cheng Sheng, Zhihao Liu, Peng Chen, Zhangjin Yang, Weifeng Hu, Shilin Lin, C. D. Chen, Jing Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography |
title | Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography |
title_full | Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography |
title_fullStr | Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography |
title_full_unstemmed | Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography |
title_short | Unraveling nonadiabatic ionization and Coulomb potential effect in strong-field photoelectron holography |
title_sort | unraveling nonadiabatic ionization and coulomb potential effect in strong-field photoelectron holography |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4916607/ https://www.ncbi.nlm.nih.gov/pubmed/27329071 http://dx.doi.org/10.1038/srep28392 |
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