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Why the dipolar response in dielectrics and spin-glasses is unavoidably universal

Materials response to electric or magnetic fields is often dominated by the dynamics of dipoles in the system. This is for instance the case of polar dielectrics and many transition metal compounds. An essential and not yet well understood fact is that, despite their structural diversity, dielectric...

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Autor principal: Cuervo-Reyes, Eduardo
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4929973/
https://www.ncbi.nlm.nih.gov/pubmed/27366866
http://dx.doi.org/10.1038/srep29021
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author Cuervo-Reyes, Eduardo
author_facet Cuervo-Reyes, Eduardo
author_sort Cuervo-Reyes, Eduardo
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description Materials response to electric or magnetic fields is often dominated by the dynamics of dipoles in the system. This is for instance the case of polar dielectrics and many transition metal compounds. An essential and not yet well understood fact is that, despite their structural diversity, dielectric solids exhibit a striking universality of frequency and time responses, sharing many aspects with the behaviour of spin-glasses. In this article I propose a stochastic approach to dipole dynamics within which the “universal frequency response” derives naturally with Debye’s relaxation mechanism as a special case. This formulation reveals constraints to the form of the relaxation functions, which are essential for a consistent representation of the dynamical slowing-down at the spin-glass transition. Relaxation functions with algebraic-, and exponential-tails, as well as damped oscillations, are shown to have a unified representation in which the stable limit of the distribution of waiting-times between dipole flips determines the present type of dynamics.
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spelling pubmed-49299732016-07-06 Why the dipolar response in dielectrics and spin-glasses is unavoidably universal Cuervo-Reyes, Eduardo Sci Rep Article Materials response to electric or magnetic fields is often dominated by the dynamics of dipoles in the system. This is for instance the case of polar dielectrics and many transition metal compounds. An essential and not yet well understood fact is that, despite their structural diversity, dielectric solids exhibit a striking universality of frequency and time responses, sharing many aspects with the behaviour of spin-glasses. In this article I propose a stochastic approach to dipole dynamics within which the “universal frequency response” derives naturally with Debye’s relaxation mechanism as a special case. This formulation reveals constraints to the form of the relaxation functions, which are essential for a consistent representation of the dynamical slowing-down at the spin-glass transition. Relaxation functions with algebraic-, and exponential-tails, as well as damped oscillations, are shown to have a unified representation in which the stable limit of the distribution of waiting-times between dipole flips determines the present type of dynamics. Nature Publishing Group 2016-07-01 /pmc/articles/PMC4929973/ /pubmed/27366866 http://dx.doi.org/10.1038/srep29021 Text en Copyright © 2016, Macmillan Publishers Limited http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Cuervo-Reyes, Eduardo
Why the dipolar response in dielectrics and spin-glasses is unavoidably universal
title Why the dipolar response in dielectrics and spin-glasses is unavoidably universal
title_full Why the dipolar response in dielectrics and spin-glasses is unavoidably universal
title_fullStr Why the dipolar response in dielectrics and spin-glasses is unavoidably universal
title_full_unstemmed Why the dipolar response in dielectrics and spin-glasses is unavoidably universal
title_short Why the dipolar response in dielectrics and spin-glasses is unavoidably universal
title_sort why the dipolar response in dielectrics and spin-glasses is unavoidably universal
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4929973/
https://www.ncbi.nlm.nih.gov/pubmed/27366866
http://dx.doi.org/10.1038/srep29021
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