Cargando…
Why the dipolar response in dielectrics and spin-glasses is unavoidably universal
Materials response to electric or magnetic fields is often dominated by the dynamics of dipoles in the system. This is for instance the case of polar dielectrics and many transition metal compounds. An essential and not yet well understood fact is that, despite their structural diversity, dielectric...
Autor principal: | |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group
2016
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4929973/ https://www.ncbi.nlm.nih.gov/pubmed/27366866 http://dx.doi.org/10.1038/srep29021 |
_version_ | 1782440684247056384 |
---|---|
author | Cuervo-Reyes, Eduardo |
author_facet | Cuervo-Reyes, Eduardo |
author_sort | Cuervo-Reyes, Eduardo |
collection | PubMed |
description | Materials response to electric or magnetic fields is often dominated by the dynamics of dipoles in the system. This is for instance the case of polar dielectrics and many transition metal compounds. An essential and not yet well understood fact is that, despite their structural diversity, dielectric solids exhibit a striking universality of frequency and time responses, sharing many aspects with the behaviour of spin-glasses. In this article I propose a stochastic approach to dipole dynamics within which the “universal frequency response” derives naturally with Debye’s relaxation mechanism as a special case. This formulation reveals constraints to the form of the relaxation functions, which are essential for a consistent representation of the dynamical slowing-down at the spin-glass transition. Relaxation functions with algebraic-, and exponential-tails, as well as damped oscillations, are shown to have a unified representation in which the stable limit of the distribution of waiting-times between dipole flips determines the present type of dynamics. |
format | Online Article Text |
id | pubmed-4929973 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2016 |
publisher | Nature Publishing Group |
record_format | MEDLINE/PubMed |
spelling | pubmed-49299732016-07-06 Why the dipolar response in dielectrics and spin-glasses is unavoidably universal Cuervo-Reyes, Eduardo Sci Rep Article Materials response to electric or magnetic fields is often dominated by the dynamics of dipoles in the system. This is for instance the case of polar dielectrics and many transition metal compounds. An essential and not yet well understood fact is that, despite their structural diversity, dielectric solids exhibit a striking universality of frequency and time responses, sharing many aspects with the behaviour of spin-glasses. In this article I propose a stochastic approach to dipole dynamics within which the “universal frequency response” derives naturally with Debye’s relaxation mechanism as a special case. This formulation reveals constraints to the form of the relaxation functions, which are essential for a consistent representation of the dynamical slowing-down at the spin-glass transition. Relaxation functions with algebraic-, and exponential-tails, as well as damped oscillations, are shown to have a unified representation in which the stable limit of the distribution of waiting-times between dipole flips determines the present type of dynamics. Nature Publishing Group 2016-07-01 /pmc/articles/PMC4929973/ /pubmed/27366866 http://dx.doi.org/10.1038/srep29021 Text en Copyright © 2016, Macmillan Publishers Limited http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ |
spellingShingle | Article Cuervo-Reyes, Eduardo Why the dipolar response in dielectrics and spin-glasses is unavoidably universal |
title | Why the dipolar response in dielectrics and spin-glasses is unavoidably universal |
title_full | Why the dipolar response in dielectrics and spin-glasses is unavoidably universal |
title_fullStr | Why the dipolar response in dielectrics and spin-glasses is unavoidably universal |
title_full_unstemmed | Why the dipolar response in dielectrics and spin-glasses is unavoidably universal |
title_short | Why the dipolar response in dielectrics and spin-glasses is unavoidably universal |
title_sort | why the dipolar response in dielectrics and spin-glasses is unavoidably universal |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4929973/ https://www.ncbi.nlm.nih.gov/pubmed/27366866 http://dx.doi.org/10.1038/srep29021 |
work_keys_str_mv | AT cuervoreyeseduardo whythedipolarresponseindielectricsandspinglassesisunavoidablyuniversal |