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Gaussian-Schell analysis of the transverse spatial properties of high-harmonic beams

High harmonic generation (HHG) is an established means of producing coherent, short wavelength, ultrafast pulses from a compact set-up. Table-top high-harmonic sources are increasingly being used to image physical and biological systems using emerging techniques such as coherent diffraction imaging...

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Autores principales: Lloyd, David T., O’Keeffe, Kevin, Anderson, Patrick N., Hooker, Simon M.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4964618/
https://www.ncbi.nlm.nih.gov/pubmed/27465654
http://dx.doi.org/10.1038/srep30504
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author Lloyd, David T.
O’Keeffe, Kevin
Anderson, Patrick N.
Hooker, Simon M.
author_facet Lloyd, David T.
O’Keeffe, Kevin
Anderson, Patrick N.
Hooker, Simon M.
author_sort Lloyd, David T.
collection PubMed
description High harmonic generation (HHG) is an established means of producing coherent, short wavelength, ultrafast pulses from a compact set-up. Table-top high-harmonic sources are increasingly being used to image physical and biological systems using emerging techniques such as coherent diffraction imaging and ptychography. These novel imaging methods require coherent illumination, and it is therefore important to both characterize the spatial coherence of high-harmonic beams and understand the processes which limit this property. Here we investigate the near- and far-field spatial properties of high-harmonic radiation generated in a gas cell. The variation with harmonic order of the intensity profile, wavefront curvature, and complex coherence factor is measured in the far-field by the SCIMITAR technique. Using the Gaussian-Schell model, the properties of the harmonic beam in the plane of generation are deduced. Our results show that the order-dependence of the harmonic spatial coherence is consistent with partial coherence induced by both variation of the intensity-dependent dipole phase as well as finite spatial coherence of the driving radiation. These findings are used to suggest ways in which the coherence of harmonic beams could be increased further, which would have direct benefits to imaging with high-harmonic radiation.
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spelling pubmed-49646182016-08-08 Gaussian-Schell analysis of the transverse spatial properties of high-harmonic beams Lloyd, David T. O’Keeffe, Kevin Anderson, Patrick N. Hooker, Simon M. Sci Rep Article High harmonic generation (HHG) is an established means of producing coherent, short wavelength, ultrafast pulses from a compact set-up. Table-top high-harmonic sources are increasingly being used to image physical and biological systems using emerging techniques such as coherent diffraction imaging and ptychography. These novel imaging methods require coherent illumination, and it is therefore important to both characterize the spatial coherence of high-harmonic beams and understand the processes which limit this property. Here we investigate the near- and far-field spatial properties of high-harmonic radiation generated in a gas cell. The variation with harmonic order of the intensity profile, wavefront curvature, and complex coherence factor is measured in the far-field by the SCIMITAR technique. Using the Gaussian-Schell model, the properties of the harmonic beam in the plane of generation are deduced. Our results show that the order-dependence of the harmonic spatial coherence is consistent with partial coherence induced by both variation of the intensity-dependent dipole phase as well as finite spatial coherence of the driving radiation. These findings are used to suggest ways in which the coherence of harmonic beams could be increased further, which would have direct benefits to imaging with high-harmonic radiation. Nature Publishing Group 2016-07-28 /pmc/articles/PMC4964618/ /pubmed/27465654 http://dx.doi.org/10.1038/srep30504 Text en Copyright © 2016, The Author(s) http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Lloyd, David T.
O’Keeffe, Kevin
Anderson, Patrick N.
Hooker, Simon M.
Gaussian-Schell analysis of the transverse spatial properties of high-harmonic beams
title Gaussian-Schell analysis of the transverse spatial properties of high-harmonic beams
title_full Gaussian-Schell analysis of the transverse spatial properties of high-harmonic beams
title_fullStr Gaussian-Schell analysis of the transverse spatial properties of high-harmonic beams
title_full_unstemmed Gaussian-Schell analysis of the transverse spatial properties of high-harmonic beams
title_short Gaussian-Schell analysis of the transverse spatial properties of high-harmonic beams
title_sort gaussian-schell analysis of the transverse spatial properties of high-harmonic beams
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4964618/
https://www.ncbi.nlm.nih.gov/pubmed/27465654
http://dx.doi.org/10.1038/srep30504
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