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Single-electron induced surface plasmons on a topological nanoparticle

It is rarely the case that a single electron affects the behaviour of several hundred thousands of atoms. Here we demonstrate a phenomenon where this happens. The key role is played by topological insulators—materials that have surface states protected by time-reversal symmetry. Such states are delo...

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Autores principales: Siroki, G., Lee, D.K.K., Haynes, P. D., Giannini, V.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4980453/
https://www.ncbi.nlm.nih.gov/pubmed/27491515
http://dx.doi.org/10.1038/ncomms12375
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author Siroki, G.
Lee, D.K.K.
Haynes, P. D.
Giannini, V.
author_facet Siroki, G.
Lee, D.K.K.
Haynes, P. D.
Giannini, V.
author_sort Siroki, G.
collection PubMed
description It is rarely the case that a single electron affects the behaviour of several hundred thousands of atoms. Here we demonstrate a phenomenon where this happens. The key role is played by topological insulators—materials that have surface states protected by time-reversal symmetry. Such states are delocalized over the surface and are immune to its imperfections in contrast to ordinary insulators. For topological insulators, the effects of these surface states will be more strongly pronounced in the case of nanoparticles. Here we show that under the influence of light a single electron in a topologically protected surface state creates a surface charge density similar to a plasmon in a metallic nanoparticle. Such an electron can act as a screening layer, which suppresses absorption inside the particle. In addition, it can couple phonons and light, giving rise to a previously unreported topological particle polariton mode. These effects may be useful in the areas of plasmonics, cavity electrodynamics and quantum information.
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spelling pubmed-49804532016-08-12 Single-electron induced surface plasmons on a topological nanoparticle Siroki, G. Lee, D.K.K. Haynes, P. D. Giannini, V. Nat Commun Article It is rarely the case that a single electron affects the behaviour of several hundred thousands of atoms. Here we demonstrate a phenomenon where this happens. The key role is played by topological insulators—materials that have surface states protected by time-reversal symmetry. Such states are delocalized over the surface and are immune to its imperfections in contrast to ordinary insulators. For topological insulators, the effects of these surface states will be more strongly pronounced in the case of nanoparticles. Here we show that under the influence of light a single electron in a topologically protected surface state creates a surface charge density similar to a plasmon in a metallic nanoparticle. Such an electron can act as a screening layer, which suppresses absorption inside the particle. In addition, it can couple phonons and light, giving rise to a previously unreported topological particle polariton mode. These effects may be useful in the areas of plasmonics, cavity electrodynamics and quantum information. Nature Publishing Group 2016-08-05 /pmc/articles/PMC4980453/ /pubmed/27491515 http://dx.doi.org/10.1038/ncomms12375 Text en Copyright © 2016, The Author(s) http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article's Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Siroki, G.
Lee, D.K.K.
Haynes, P. D.
Giannini, V.
Single-electron induced surface plasmons on a topological nanoparticle
title Single-electron induced surface plasmons on a topological nanoparticle
title_full Single-electron induced surface plasmons on a topological nanoparticle
title_fullStr Single-electron induced surface plasmons on a topological nanoparticle
title_full_unstemmed Single-electron induced surface plasmons on a topological nanoparticle
title_short Single-electron induced surface plasmons on a topological nanoparticle
title_sort single-electron induced surface plasmons on a topological nanoparticle
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4980453/
https://www.ncbi.nlm.nih.gov/pubmed/27491515
http://dx.doi.org/10.1038/ncomms12375
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