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Core-Shell Co/CoO Integrated on 3D Nitrogen Doped Reduced Graphene Oxide Aerogel as an Enhanced Electrocatalyst for the Oxygen Reduction Reaction

Here, we demonstrate that Cobalt/cobalt oxide core-shell nanoparticles integrated on nitrogen-doped (N-doped) three-dimensional reduced graphene oxide aerogel-based architecture (Co/CoO-NGA) were synthesized through a facile hydrothermal method followed by annealing treatment. The unique endurable p...

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Detalles Bibliográficos
Autores principales: Wang, Meng, Hou, Yuyang, Slade, Robert C. T., Wang, Jiazhao, Shi, Dongqi, Wexler, David, Liu, Huakun, Chen, Jun
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Frontiers Media S.A. 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4992675/
https://www.ncbi.nlm.nih.gov/pubmed/27597939
http://dx.doi.org/10.3389/fchem.2016.00036
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author Wang, Meng
Hou, Yuyang
Slade, Robert C. T.
Wang, Jiazhao
Shi, Dongqi
Wexler, David
Liu, Huakun
Chen, Jun
author_facet Wang, Meng
Hou, Yuyang
Slade, Robert C. T.
Wang, Jiazhao
Shi, Dongqi
Wexler, David
Liu, Huakun
Chen, Jun
author_sort Wang, Meng
collection PubMed
description Here, we demonstrate that Cobalt/cobalt oxide core-shell nanoparticles integrated on nitrogen-doped (N-doped) three-dimensional reduced graphene oxide aerogel-based architecture (Co/CoO-NGA) were synthesized through a facile hydrothermal method followed by annealing treatment. The unique endurable porous structure could provide sufficient mass transfer channels and ample active sites on Co/CoO-NGA to facilitate the catalytic reaction. The synthesized Co/CoO-NGA was explored as an electrocatalyst for the oxygen reduction reaction, showing comparable oxygen reduction performance with excellent methanol resistance and better durability compared with Pt/C.
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spelling pubmed-49926752016-09-05 Core-Shell Co/CoO Integrated on 3D Nitrogen Doped Reduced Graphene Oxide Aerogel as an Enhanced Electrocatalyst for the Oxygen Reduction Reaction Wang, Meng Hou, Yuyang Slade, Robert C. T. Wang, Jiazhao Shi, Dongqi Wexler, David Liu, Huakun Chen, Jun Front Chem Chemistry Here, we demonstrate that Cobalt/cobalt oxide core-shell nanoparticles integrated on nitrogen-doped (N-doped) three-dimensional reduced graphene oxide aerogel-based architecture (Co/CoO-NGA) were synthesized through a facile hydrothermal method followed by annealing treatment. The unique endurable porous structure could provide sufficient mass transfer channels and ample active sites on Co/CoO-NGA to facilitate the catalytic reaction. The synthesized Co/CoO-NGA was explored as an electrocatalyst for the oxygen reduction reaction, showing comparable oxygen reduction performance with excellent methanol resistance and better durability compared with Pt/C. Frontiers Media S.A. 2016-08-22 /pmc/articles/PMC4992675/ /pubmed/27597939 http://dx.doi.org/10.3389/fchem.2016.00036 Text en Copyright © 2016 Wang, Hou, Slade, Wang, Shi, Wexler, Liu and Chen. http://creativecommons.org/licenses/by/4.0/ This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) or licensor are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.
spellingShingle Chemistry
Wang, Meng
Hou, Yuyang
Slade, Robert C. T.
Wang, Jiazhao
Shi, Dongqi
Wexler, David
Liu, Huakun
Chen, Jun
Core-Shell Co/CoO Integrated on 3D Nitrogen Doped Reduced Graphene Oxide Aerogel as an Enhanced Electrocatalyst for the Oxygen Reduction Reaction
title Core-Shell Co/CoO Integrated on 3D Nitrogen Doped Reduced Graphene Oxide Aerogel as an Enhanced Electrocatalyst for the Oxygen Reduction Reaction
title_full Core-Shell Co/CoO Integrated on 3D Nitrogen Doped Reduced Graphene Oxide Aerogel as an Enhanced Electrocatalyst for the Oxygen Reduction Reaction
title_fullStr Core-Shell Co/CoO Integrated on 3D Nitrogen Doped Reduced Graphene Oxide Aerogel as an Enhanced Electrocatalyst for the Oxygen Reduction Reaction
title_full_unstemmed Core-Shell Co/CoO Integrated on 3D Nitrogen Doped Reduced Graphene Oxide Aerogel as an Enhanced Electrocatalyst for the Oxygen Reduction Reaction
title_short Core-Shell Co/CoO Integrated on 3D Nitrogen Doped Reduced Graphene Oxide Aerogel as an Enhanced Electrocatalyst for the Oxygen Reduction Reaction
title_sort core-shell co/coo integrated on 3d nitrogen doped reduced graphene oxide aerogel as an enhanced electrocatalyst for the oxygen reduction reaction
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4992675/
https://www.ncbi.nlm.nih.gov/pubmed/27597939
http://dx.doi.org/10.3389/fchem.2016.00036
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