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Staircase Quantum Dots Configuration in Nanowires for Optimized Thermoelectric Power

The performance of thermoelectric energy harvesters can be improved by nanostructures that exploit inelastic transport processes. One prototype is the three-terminal hopping thermoelectric device where electron hopping between quantum-dots are driven by hot phonons. Such three-terminal hopping therm...

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Detalles Bibliográficos
Autores principales: Li, Lijie, Jiang, Jian-Hua
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4994073/
https://www.ncbi.nlm.nih.gov/pubmed/27550093
http://dx.doi.org/10.1038/srep31974
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author Li, Lijie
Jiang, Jian-Hua
author_facet Li, Lijie
Jiang, Jian-Hua
author_sort Li, Lijie
collection PubMed
description The performance of thermoelectric energy harvesters can be improved by nanostructures that exploit inelastic transport processes. One prototype is the three-terminal hopping thermoelectric device where electron hopping between quantum-dots are driven by hot phonons. Such three-terminal hopping thermoelectric devices have potential in achieving high efficiency or power via inelastic transport and without relying on heavy-elements or toxic compounds. We show in this work how output power of the device can be optimized via tuning the number and energy configuration of the quantum-dots embedded in parallel nanowires. We find that the staircase energy configuration with constant energy-step can improve the power factor over a serial connection of a single pair of quantum-dots. Moreover, for a fixed energy-step, there is an optimal length for the nanowire. Similarly for a fixed number of quantum-dots there is an optimal energy-step for the output power. Our results are important for future developments of high-performance nanostructured thermoelectric devices.
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spelling pubmed-49940732016-08-30 Staircase Quantum Dots Configuration in Nanowires for Optimized Thermoelectric Power Li, Lijie Jiang, Jian-Hua Sci Rep Article The performance of thermoelectric energy harvesters can be improved by nanostructures that exploit inelastic transport processes. One prototype is the three-terminal hopping thermoelectric device where electron hopping between quantum-dots are driven by hot phonons. Such three-terminal hopping thermoelectric devices have potential in achieving high efficiency or power via inelastic transport and without relying on heavy-elements or toxic compounds. We show in this work how output power of the device can be optimized via tuning the number and energy configuration of the quantum-dots embedded in parallel nanowires. We find that the staircase energy configuration with constant energy-step can improve the power factor over a serial connection of a single pair of quantum-dots. Moreover, for a fixed energy-step, there is an optimal length for the nanowire. Similarly for a fixed number of quantum-dots there is an optimal energy-step for the output power. Our results are important for future developments of high-performance nanostructured thermoelectric devices. Nature Publishing Group 2016-08-23 /pmc/articles/PMC4994073/ /pubmed/27550093 http://dx.doi.org/10.1038/srep31974 Text en Copyright © 2016, The Author(s) http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Li, Lijie
Jiang, Jian-Hua
Staircase Quantum Dots Configuration in Nanowires for Optimized Thermoelectric Power
title Staircase Quantum Dots Configuration in Nanowires for Optimized Thermoelectric Power
title_full Staircase Quantum Dots Configuration in Nanowires for Optimized Thermoelectric Power
title_fullStr Staircase Quantum Dots Configuration in Nanowires for Optimized Thermoelectric Power
title_full_unstemmed Staircase Quantum Dots Configuration in Nanowires for Optimized Thermoelectric Power
title_short Staircase Quantum Dots Configuration in Nanowires for Optimized Thermoelectric Power
title_sort staircase quantum dots configuration in nanowires for optimized thermoelectric power
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4994073/
https://www.ncbi.nlm.nih.gov/pubmed/27550093
http://dx.doi.org/10.1038/srep31974
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