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Magneto-Optical Study of Defect Induced Sharp Photoluminescence in LaAlO(3) and SrTiO(3)

Strongly correlated electronic systems such as Transition Metal Oxides often possess various mid-gap states originating from intrinsic defects in these materials. In this paper, we investigate an extremely sharp Photoluminescence (PL) transition originating from such defect states in two widely used...

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Detalles Bibliográficos
Autores principales: Sarkar, Soumya, Saha, Surajit, Motapothula, M. R., Patra, Abhijeet, Cao, Bing-Chen, Prakash, Saurav, Cong, Chun Xiao, Mathew, Sinu, Ghosh, Siddhartha, Yu, Ting, Venkatesan, T.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5020611/
https://www.ncbi.nlm.nih.gov/pubmed/27619076
http://dx.doi.org/10.1038/srep33145
Descripción
Sumario:Strongly correlated electronic systems such as Transition Metal Oxides often possess various mid-gap states originating from intrinsic defects in these materials. In this paper, we investigate an extremely sharp Photoluminescence (PL) transition originating from such defect states in two widely used perovskites, LaAlO(3) and SrTiO(3). A detailed study of the PL as a function of temperature and magnetic field has been conducted to understand the behavior and origin of the transition involved. The temperature dependence of the PL peak position for SrTiO(3) is observed to be opposite to that in LaAlO(3). Our results reveal the presence of a spin/orbital character in these transitions which is evident from the splitting of these defect energy levels under a high magnetic field. These PL transitions have the potential for enabling non-contact thermal and field sensors.