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Magneto-Optical Study of Defect Induced Sharp Photoluminescence in LaAlO(3) and SrTiO(3)

Strongly correlated electronic systems such as Transition Metal Oxides often possess various mid-gap states originating from intrinsic defects in these materials. In this paper, we investigate an extremely sharp Photoluminescence (PL) transition originating from such defect states in two widely used...

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Autores principales: Sarkar, Soumya, Saha, Surajit, Motapothula, M. R., Patra, Abhijeet, Cao, Bing-Chen, Prakash, Saurav, Cong, Chun Xiao, Mathew, Sinu, Ghosh, Siddhartha, Yu, Ting, Venkatesan, T.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5020611/
https://www.ncbi.nlm.nih.gov/pubmed/27619076
http://dx.doi.org/10.1038/srep33145
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author Sarkar, Soumya
Saha, Surajit
Motapothula, M. R.
Patra, Abhijeet
Cao, Bing-Chen
Prakash, Saurav
Cong, Chun Xiao
Mathew, Sinu
Ghosh, Siddhartha
Yu, Ting
Venkatesan, T.
author_facet Sarkar, Soumya
Saha, Surajit
Motapothula, M. R.
Patra, Abhijeet
Cao, Bing-Chen
Prakash, Saurav
Cong, Chun Xiao
Mathew, Sinu
Ghosh, Siddhartha
Yu, Ting
Venkatesan, T.
author_sort Sarkar, Soumya
collection PubMed
description Strongly correlated electronic systems such as Transition Metal Oxides often possess various mid-gap states originating from intrinsic defects in these materials. In this paper, we investigate an extremely sharp Photoluminescence (PL) transition originating from such defect states in two widely used perovskites, LaAlO(3) and SrTiO(3). A detailed study of the PL as a function of temperature and magnetic field has been conducted to understand the behavior and origin of the transition involved. The temperature dependence of the PL peak position for SrTiO(3) is observed to be opposite to that in LaAlO(3). Our results reveal the presence of a spin/orbital character in these transitions which is evident from the splitting of these defect energy levels under a high magnetic field. These PL transitions have the potential for enabling non-contact thermal and field sensors.
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spelling pubmed-50206112016-09-20 Magneto-Optical Study of Defect Induced Sharp Photoluminescence in LaAlO(3) and SrTiO(3) Sarkar, Soumya Saha, Surajit Motapothula, M. R. Patra, Abhijeet Cao, Bing-Chen Prakash, Saurav Cong, Chun Xiao Mathew, Sinu Ghosh, Siddhartha Yu, Ting Venkatesan, T. Sci Rep Article Strongly correlated electronic systems such as Transition Metal Oxides often possess various mid-gap states originating from intrinsic defects in these materials. In this paper, we investigate an extremely sharp Photoluminescence (PL) transition originating from such defect states in two widely used perovskites, LaAlO(3) and SrTiO(3). A detailed study of the PL as a function of temperature and magnetic field has been conducted to understand the behavior and origin of the transition involved. The temperature dependence of the PL peak position for SrTiO(3) is observed to be opposite to that in LaAlO(3). Our results reveal the presence of a spin/orbital character in these transitions which is evident from the splitting of these defect energy levels under a high magnetic field. These PL transitions have the potential for enabling non-contact thermal and field sensors. Nature Publishing Group 2016-09-13 /pmc/articles/PMC5020611/ /pubmed/27619076 http://dx.doi.org/10.1038/srep33145 Text en Copyright © 2016, The Author(s) http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Sarkar, Soumya
Saha, Surajit
Motapothula, M. R.
Patra, Abhijeet
Cao, Bing-Chen
Prakash, Saurav
Cong, Chun Xiao
Mathew, Sinu
Ghosh, Siddhartha
Yu, Ting
Venkatesan, T.
Magneto-Optical Study of Defect Induced Sharp Photoluminescence in LaAlO(3) and SrTiO(3)
title Magneto-Optical Study of Defect Induced Sharp Photoluminescence in LaAlO(3) and SrTiO(3)
title_full Magneto-Optical Study of Defect Induced Sharp Photoluminescence in LaAlO(3) and SrTiO(3)
title_fullStr Magneto-Optical Study of Defect Induced Sharp Photoluminescence in LaAlO(3) and SrTiO(3)
title_full_unstemmed Magneto-Optical Study of Defect Induced Sharp Photoluminescence in LaAlO(3) and SrTiO(3)
title_short Magneto-Optical Study of Defect Induced Sharp Photoluminescence in LaAlO(3) and SrTiO(3)
title_sort magneto-optical study of defect induced sharp photoluminescence in laalo(3) and srtio(3)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5020611/
https://www.ncbi.nlm.nih.gov/pubmed/27619076
http://dx.doi.org/10.1038/srep33145
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