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High Quality Factor Mechanical Resonators Based on WSe(2) Monolayers

[Image: see text] Suspended monolayer transition metal dichalcogenides (TMD) are membranes that combine ultralow mass and exceptional optical properties, making them intriguing materials for opto-mechanical applications. However, the low measured quality factor of TMD resonators has been a roadblock...

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Autores principales: Morell, Nicolas, Reserbat-Plantey, Antoine, Tsioutsios, Ioannis, Schädler, Kevin G., Dubin, François, Koppens, Frank H. L., Bachtold, Adrian
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2016
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5023224/
https://www.ncbi.nlm.nih.gov/pubmed/27459399
http://dx.doi.org/10.1021/acs.nanolett.6b02038
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author Morell, Nicolas
Reserbat-Plantey, Antoine
Tsioutsios, Ioannis
Schädler, Kevin G.
Dubin, François
Koppens, Frank H. L.
Bachtold, Adrian
author_facet Morell, Nicolas
Reserbat-Plantey, Antoine
Tsioutsios, Ioannis
Schädler, Kevin G.
Dubin, François
Koppens, Frank H. L.
Bachtold, Adrian
author_sort Morell, Nicolas
collection PubMed
description [Image: see text] Suspended monolayer transition metal dichalcogenides (TMD) are membranes that combine ultralow mass and exceptional optical properties, making them intriguing materials for opto-mechanical applications. However, the low measured quality factor of TMD resonators has been a roadblock so far. Here, we report an ultrasensitive optical readout of monolayer TMD resonators that allows us to reveal their mechanical properties at cryogenic temperatures. We find that the quality factor of monolayer WSe(2) resonators greatly increases below room temperature, reaching values as high as 1.6 × 10(4) at liquid nitrogen temperature and 4.7 × 10(4) at liquid helium temperature. This surpasses the quality factor of monolayer graphene resonators with similar surface areas. Upon cooling the resonator, the resonant frequency increases significantly due to the thermal contraction of the WSe(2) lattice. These measurements allow us to experimentally study the thermal expansion coefficient of WSe(2) monolayers for the first time. High Q-factors are also found in resonators based on MoS(2) and MoSe(2) monolayers. The high quality-factor found in this work opens new possibilities for coupling mechanical vibrational states to two-dimensional excitons, valley pseudospins, and single quantum emitters and for quantum opto-mechanical experiments based on the Casimir interaction.
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spelling pubmed-50232242016-09-19 High Quality Factor Mechanical Resonators Based on WSe(2) Monolayers Morell, Nicolas Reserbat-Plantey, Antoine Tsioutsios, Ioannis Schädler, Kevin G. Dubin, François Koppens, Frank H. L. Bachtold, Adrian Nano Lett [Image: see text] Suspended monolayer transition metal dichalcogenides (TMD) are membranes that combine ultralow mass and exceptional optical properties, making them intriguing materials for opto-mechanical applications. However, the low measured quality factor of TMD resonators has been a roadblock so far. Here, we report an ultrasensitive optical readout of monolayer TMD resonators that allows us to reveal their mechanical properties at cryogenic temperatures. We find that the quality factor of monolayer WSe(2) resonators greatly increases below room temperature, reaching values as high as 1.6 × 10(4) at liquid nitrogen temperature and 4.7 × 10(4) at liquid helium temperature. This surpasses the quality factor of monolayer graphene resonators with similar surface areas. Upon cooling the resonator, the resonant frequency increases significantly due to the thermal contraction of the WSe(2) lattice. These measurements allow us to experimentally study the thermal expansion coefficient of WSe(2) monolayers for the first time. High Q-factors are also found in resonators based on MoS(2) and MoSe(2) monolayers. The high quality-factor found in this work opens new possibilities for coupling mechanical vibrational states to two-dimensional excitons, valley pseudospins, and single quantum emitters and for quantum opto-mechanical experiments based on the Casimir interaction. American Chemical Society 2016-07-26 2016-08-10 /pmc/articles/PMC5023224/ /pubmed/27459399 http://dx.doi.org/10.1021/acs.nanolett.6b02038 Text en Copyright © 2016 American Chemical Society This is an open access article published under an ACS AuthorChoice License (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html) , which permits copying and redistribution of the article or any adaptations for non-commercial purposes.
spellingShingle Morell, Nicolas
Reserbat-Plantey, Antoine
Tsioutsios, Ioannis
Schädler, Kevin G.
Dubin, François
Koppens, Frank H. L.
Bachtold, Adrian
High Quality Factor Mechanical Resonators Based on WSe(2) Monolayers
title High Quality Factor Mechanical Resonators Based on WSe(2) Monolayers
title_full High Quality Factor Mechanical Resonators Based on WSe(2) Monolayers
title_fullStr High Quality Factor Mechanical Resonators Based on WSe(2) Monolayers
title_full_unstemmed High Quality Factor Mechanical Resonators Based on WSe(2) Monolayers
title_short High Quality Factor Mechanical Resonators Based on WSe(2) Monolayers
title_sort high quality factor mechanical resonators based on wse(2) monolayers
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5023224/
https://www.ncbi.nlm.nih.gov/pubmed/27459399
http://dx.doi.org/10.1021/acs.nanolett.6b02038
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