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Lithium-ion-based solid electrolyte tuning of the carrier density in graphene

We have developed a technique to tune the carrier density in graphene using a lithium-ion-based solid electrolyte. We demonstrate that the solid electrolyte can be used as both a substrate to support graphene and a back gate. It can induce a change in the carrier density as large as 1 × 10(14) cm(−2...

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Detalles Bibliográficos
Autores principales: Zhao, Jialin, Wang, Meng, Li, Hui, Zhang, Xuefu, You, Lixing, Qiao, Shan, Gao, Bo, Xie, Xiaoming, Jiang, Mianheng
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5048137/
https://www.ncbi.nlm.nih.gov/pubmed/27698413
http://dx.doi.org/10.1038/srep34816
Descripción
Sumario:We have developed a technique to tune the carrier density in graphene using a lithium-ion-based solid electrolyte. We demonstrate that the solid electrolyte can be used as both a substrate to support graphene and a back gate. It can induce a change in the carrier density as large as 1 × 10(14) cm(−2), which is much larger than that induced with oxide-film dielectrics, and it is comparable with that induced by liquid electrolytes. Gate modulation of the carrier density is still visible at 150 K, which is lower than the glass transition temperature of most liquid gating electrolytes.