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Surface Lattice Resonances for Enhanced and Directional Electroluminescence at High Current Densities

[Image: see text] Hybrid photonic-plasmonic modes in periodic arrays of metallic nanostructures offer a promising trade-off between high-quality cavities and subdiffraction mode confinement. However, their application in electrically driven light-emitting devices is hindered by their sensitivity to...

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Autores principales: Zakharko, Yuriy, Held, Martin, Graf, Arko, Rödlmeier, Tobias, Eckstein, Ralph, Hernandez-Sosa, Gerardo, Hähnlein, Bernd, Pezoldt, Jörg, Zaumseil, Jana
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2016
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5191620/
https://www.ncbi.nlm.nih.gov/pubmed/28042593
http://dx.doi.org/10.1021/acsphotonics.6b00491
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author Zakharko, Yuriy
Held, Martin
Graf, Arko
Rödlmeier, Tobias
Eckstein, Ralph
Hernandez-Sosa, Gerardo
Hähnlein, Bernd
Pezoldt, Jörg
Zaumseil, Jana
author_facet Zakharko, Yuriy
Held, Martin
Graf, Arko
Rödlmeier, Tobias
Eckstein, Ralph
Hernandez-Sosa, Gerardo
Hähnlein, Bernd
Pezoldt, Jörg
Zaumseil, Jana
author_sort Zakharko, Yuriy
collection PubMed
description [Image: see text] Hybrid photonic-plasmonic modes in periodic arrays of metallic nanostructures offer a promising trade-off between high-quality cavities and subdiffraction mode confinement. However, their application in electrically driven light-emitting devices is hindered by their sensitivity to the surrounding environment and to charge injecting metallic electrodes in particular. Here, we demonstrate that the planar structure of light-emitting field-effect transistor (LEFET) ensures undisturbed operation of the characteristic modes. We incorporate a square array of gold nanodisks into the charge transporting and emissive layer of a polymer LEFET in order to tailor directionality and emission efficiency via the Purcell effect and variation of the fractional local density of states in particular. Angle- and polarization-resolved spectra confirm that the enhanced electroluminescence correlates with the dispersion curves of the surface lattice resonances supported by these structures. These LEFETs reach current densities on the order of 10 kA/cm(2), which may pave the way toward practical optoelectronic devices with tailored emission patterns and potentially electrically pumped plasmonic lasers.
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spelling pubmed-51916202016-12-28 Surface Lattice Resonances for Enhanced and Directional Electroluminescence at High Current Densities Zakharko, Yuriy Held, Martin Graf, Arko Rödlmeier, Tobias Eckstein, Ralph Hernandez-Sosa, Gerardo Hähnlein, Bernd Pezoldt, Jörg Zaumseil, Jana ACS Photonics [Image: see text] Hybrid photonic-plasmonic modes in periodic arrays of metallic nanostructures offer a promising trade-off between high-quality cavities and subdiffraction mode confinement. However, their application in electrically driven light-emitting devices is hindered by their sensitivity to the surrounding environment and to charge injecting metallic electrodes in particular. Here, we demonstrate that the planar structure of light-emitting field-effect transistor (LEFET) ensures undisturbed operation of the characteristic modes. We incorporate a square array of gold nanodisks into the charge transporting and emissive layer of a polymer LEFET in order to tailor directionality and emission efficiency via the Purcell effect and variation of the fractional local density of states in particular. Angle- and polarization-resolved spectra confirm that the enhanced electroluminescence correlates with the dispersion curves of the surface lattice resonances supported by these structures. These LEFETs reach current densities on the order of 10 kA/cm(2), which may pave the way toward practical optoelectronic devices with tailored emission patterns and potentially electrically pumped plasmonic lasers. American Chemical Society 2016-11-09 2016-12-21 /pmc/articles/PMC5191620/ /pubmed/28042593 http://dx.doi.org/10.1021/acsphotonics.6b00491 Text en Copyright © 2016 American Chemical Society This is an open access article published under an ACS AuthorChoice License (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html) , which permits copying and redistribution of the article or any adaptations for non-commercial purposes.
spellingShingle Zakharko, Yuriy
Held, Martin
Graf, Arko
Rödlmeier, Tobias
Eckstein, Ralph
Hernandez-Sosa, Gerardo
Hähnlein, Bernd
Pezoldt, Jörg
Zaumseil, Jana
Surface Lattice Resonances for Enhanced and Directional Electroluminescence at High Current Densities
title Surface Lattice Resonances for Enhanced and Directional Electroluminescence at High Current Densities
title_full Surface Lattice Resonances for Enhanced and Directional Electroluminescence at High Current Densities
title_fullStr Surface Lattice Resonances for Enhanced and Directional Electroluminescence at High Current Densities
title_full_unstemmed Surface Lattice Resonances for Enhanced and Directional Electroluminescence at High Current Densities
title_short Surface Lattice Resonances for Enhanced and Directional Electroluminescence at High Current Densities
title_sort surface lattice resonances for enhanced and directional electroluminescence at high current densities
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5191620/
https://www.ncbi.nlm.nih.gov/pubmed/28042593
http://dx.doi.org/10.1021/acsphotonics.6b00491
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