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Investigation of phonon coherence and backscattering using silicon nanomeshes

Phonons can display both wave-like and particle-like behaviour during thermal transport. While thermal transport in silicon nanomeshes has been previously interpreted by phonon wave effects due to interference with periodic structures, as well as phonon particle effects including backscattering, the...

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Autores principales: Lee, Jaeho, Lee, Woochul, Wehmeyer, Geoff, Dhuey, Scott, Olynick, Deirdre L., Cabrini, Stefano, Dames, Chris, Urban, Jeffrey J., Yang, Peidong
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2017
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5216120/
https://www.ncbi.nlm.nih.gov/pubmed/28051081
http://dx.doi.org/10.1038/ncomms14054
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author Lee, Jaeho
Lee, Woochul
Wehmeyer, Geoff
Dhuey, Scott
Olynick, Deirdre L.
Cabrini, Stefano
Dames, Chris
Urban, Jeffrey J.
Yang, Peidong
author_facet Lee, Jaeho
Lee, Woochul
Wehmeyer, Geoff
Dhuey, Scott
Olynick, Deirdre L.
Cabrini, Stefano
Dames, Chris
Urban, Jeffrey J.
Yang, Peidong
author_sort Lee, Jaeho
collection PubMed
description Phonons can display both wave-like and particle-like behaviour during thermal transport. While thermal transport in silicon nanomeshes has been previously interpreted by phonon wave effects due to interference with periodic structures, as well as phonon particle effects including backscattering, the dominant mechanism responsible for thermal conductivity reductions below classical predictions still remains unclear. Here we isolate the wave-related coherence effects by comparing periodic and aperiodic nanomeshes, and quantify the backscattering effect by comparing variable-pitch nanomeshes. We measure identical (within 6% uncertainty) thermal conductivities for periodic and aperiodic nanomeshes of the same average pitch, and reduced thermal conductivities for nanomeshes with smaller pitches. Ray tracing simulations support the measurement results. We conclude phonon coherence is unimportant for thermal transport in silicon nanomeshes with periodicities of 100 nm and higher and temperatures above 14 K, and phonon backscattering, as manifested in the classical size effect, is responsible for the thermal conductivity reduction.
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spelling pubmed-52161202017-01-06 Investigation of phonon coherence and backscattering using silicon nanomeshes Lee, Jaeho Lee, Woochul Wehmeyer, Geoff Dhuey, Scott Olynick, Deirdre L. Cabrini, Stefano Dames, Chris Urban, Jeffrey J. Yang, Peidong Nat Commun Article Phonons can display both wave-like and particle-like behaviour during thermal transport. While thermal transport in silicon nanomeshes has been previously interpreted by phonon wave effects due to interference with periodic structures, as well as phonon particle effects including backscattering, the dominant mechanism responsible for thermal conductivity reductions below classical predictions still remains unclear. Here we isolate the wave-related coherence effects by comparing periodic and aperiodic nanomeshes, and quantify the backscattering effect by comparing variable-pitch nanomeshes. We measure identical (within 6% uncertainty) thermal conductivities for periodic and aperiodic nanomeshes of the same average pitch, and reduced thermal conductivities for nanomeshes with smaller pitches. Ray tracing simulations support the measurement results. We conclude phonon coherence is unimportant for thermal transport in silicon nanomeshes with periodicities of 100 nm and higher and temperatures above 14 K, and phonon backscattering, as manifested in the classical size effect, is responsible for the thermal conductivity reduction. Nature Publishing Group 2017-01-04 /pmc/articles/PMC5216120/ /pubmed/28051081 http://dx.doi.org/10.1038/ncomms14054 Text en Copyright © 2017, The Author(s) http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article's Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Lee, Jaeho
Lee, Woochul
Wehmeyer, Geoff
Dhuey, Scott
Olynick, Deirdre L.
Cabrini, Stefano
Dames, Chris
Urban, Jeffrey J.
Yang, Peidong
Investigation of phonon coherence and backscattering using silicon nanomeshes
title Investigation of phonon coherence and backscattering using silicon nanomeshes
title_full Investigation of phonon coherence and backscattering using silicon nanomeshes
title_fullStr Investigation of phonon coherence and backscattering using silicon nanomeshes
title_full_unstemmed Investigation of phonon coherence and backscattering using silicon nanomeshes
title_short Investigation of phonon coherence and backscattering using silicon nanomeshes
title_sort investigation of phonon coherence and backscattering using silicon nanomeshes
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5216120/
https://www.ncbi.nlm.nih.gov/pubmed/28051081
http://dx.doi.org/10.1038/ncomms14054
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