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Accelerated crystallization of colloidal glass by mechanical oscillation
Crystallization of a hard-sphere colloidal glass by mechanical oscillation is investigated, and accelerated crystallization is found at a specific frequency. The crystallization frequency increases as attractive force between particles increases, indicating that interparticle interaction affects the...
Autores principales: | , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2017
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5430959/ https://www.ncbi.nlm.nih.gov/pubmed/28465535 http://dx.doi.org/10.1038/s41598-017-01484-y |
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author | Nakamura, Nobutomo Inayama, Kyosuke Okuno, Tasuku Ogi, Hirotsugu Hirao, Masahiko |
author_facet | Nakamura, Nobutomo Inayama, Kyosuke Okuno, Tasuku Ogi, Hirotsugu Hirao, Masahiko |
author_sort | Nakamura, Nobutomo |
collection | PubMed |
description | Crystallization of a hard-sphere colloidal glass by mechanical oscillation is investigated, and accelerated crystallization is found at a specific frequency. The crystallization frequency increases as attractive force between particles increases, indicating that interparticle interaction affects the crystallization frequency. Time scale of the mechanical oscillation is different from that of the slow relaxation, and notable relationship with the low-frequency mode is not observed. The experimental results are not explained by the previously proposed model for crystallization by oscillatory shear. Conversely, we speculate that activations of the fast relaxation and particle motion in crystal-like clusters are possible causes of the observations. |
format | Online Article Text |
id | pubmed-5430959 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2017 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-54309592017-05-16 Accelerated crystallization of colloidal glass by mechanical oscillation Nakamura, Nobutomo Inayama, Kyosuke Okuno, Tasuku Ogi, Hirotsugu Hirao, Masahiko Sci Rep Article Crystallization of a hard-sphere colloidal glass by mechanical oscillation is investigated, and accelerated crystallization is found at a specific frequency. The crystallization frequency increases as attractive force between particles increases, indicating that interparticle interaction affects the crystallization frequency. Time scale of the mechanical oscillation is different from that of the slow relaxation, and notable relationship with the low-frequency mode is not observed. The experimental results are not explained by the previously proposed model for crystallization by oscillatory shear. Conversely, we speculate that activations of the fast relaxation and particle motion in crystal-like clusters are possible causes of the observations. Nature Publishing Group UK 2017-05-02 /pmc/articles/PMC5430959/ /pubmed/28465535 http://dx.doi.org/10.1038/s41598-017-01484-y Text en © The Author(s) 2017 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Nakamura, Nobutomo Inayama, Kyosuke Okuno, Tasuku Ogi, Hirotsugu Hirao, Masahiko Accelerated crystallization of colloidal glass by mechanical oscillation |
title | Accelerated crystallization of colloidal glass by mechanical oscillation |
title_full | Accelerated crystallization of colloidal glass by mechanical oscillation |
title_fullStr | Accelerated crystallization of colloidal glass by mechanical oscillation |
title_full_unstemmed | Accelerated crystallization of colloidal glass by mechanical oscillation |
title_short | Accelerated crystallization of colloidal glass by mechanical oscillation |
title_sort | accelerated crystallization of colloidal glass by mechanical oscillation |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5430959/ https://www.ncbi.nlm.nih.gov/pubmed/28465535 http://dx.doi.org/10.1038/s41598-017-01484-y |
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