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Evolution of the intrinsic electronic phase separation in La(0.6)Er(0.1)Sr(0.3)MnO(3) perovskite

Magnetic and electronic transport properties of perovskite manganite La(0.6)Er(0.1)Sr(0.3)MnO(3) have been thoroughly examined through the measurements of magnetization, electron paramagnetic resonance(EPR), and resistivity. It was found that the substitution of Er(3+) for La(3+) ions introduced the...

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Autores principales: Chen, Lili, Fan, Jiyu, Tong, Wei, Hu, Dazhi, Ji, Yanda, Liu, Jindong, Zhang, Lei, Pi, Li, Zhang, Yuheng, Yang, Hao
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2016
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5431341/
https://www.ncbi.nlm.nih.gov/pubmed/28442764
http://dx.doi.org/10.1038/s41598-016-0009-0
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author Chen, Lili
Fan, Jiyu
Tong, Wei
Hu, Dazhi
Ji, Yanda
Liu, Jindong
Zhang, Lei
Pi, Li
Zhang, Yuheng
Yang, Hao
author_facet Chen, Lili
Fan, Jiyu
Tong, Wei
Hu, Dazhi
Ji, Yanda
Liu, Jindong
Zhang, Lei
Pi, Li
Zhang, Yuheng
Yang, Hao
author_sort Chen, Lili
collection PubMed
description Magnetic and electronic transport properties of perovskite manganite La(0.6)Er(0.1)Sr(0.3)MnO(3) have been thoroughly examined through the measurements of magnetization, electron paramagnetic resonance(EPR), and resistivity. It was found that the substitution of Er(3+) for La(3+) ions introduced the chemical disorder and additional strain in this sample. An extra resonance signal occurred in EPR spectra at high temperatures well above T(C) gives a strong evidence of electronic phase separation(EPS). The analysis of resistivity enable us to identify the polaronic transport mechanism in the paramagnetic region. At low temperature, a new ferromagnetic interaction generates in the microdomains of Er(3+)-disorder causing the second increase of magnetization. However, the new ferromagnetic interaction does not improve but decreases electronic transport due to the enhancement of interface resistance among neighboring domains. In view of a really wide temperature region for the EPS existence, this sample provides an ideal platform to uncover the evolution law of different magnetic structures in perovskite manganites.
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spelling pubmed-54313412017-05-17 Evolution of the intrinsic electronic phase separation in La(0.6)Er(0.1)Sr(0.3)MnO(3) perovskite Chen, Lili Fan, Jiyu Tong, Wei Hu, Dazhi Ji, Yanda Liu, Jindong Zhang, Lei Pi, Li Zhang, Yuheng Yang, Hao Sci Rep Article Magnetic and electronic transport properties of perovskite manganite La(0.6)Er(0.1)Sr(0.3)MnO(3) have been thoroughly examined through the measurements of magnetization, electron paramagnetic resonance(EPR), and resistivity. It was found that the substitution of Er(3+) for La(3+) ions introduced the chemical disorder and additional strain in this sample. An extra resonance signal occurred in EPR spectra at high temperatures well above T(C) gives a strong evidence of electronic phase separation(EPS). The analysis of resistivity enable us to identify the polaronic transport mechanism in the paramagnetic region. At low temperature, a new ferromagnetic interaction generates in the microdomains of Er(3+)-disorder causing the second increase of magnetization. However, the new ferromagnetic interaction does not improve but decreases electronic transport due to the enhancement of interface resistance among neighboring domains. In view of a really wide temperature region for the EPS existence, this sample provides an ideal platform to uncover the evolution law of different magnetic structures in perovskite manganites. Nature Publishing Group UK 2016-12-05 /pmc/articles/PMC5431341/ /pubmed/28442764 http://dx.doi.org/10.1038/s41598-016-0009-0 Text en © The Author(s) 2016 This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
spellingShingle Article
Chen, Lili
Fan, Jiyu
Tong, Wei
Hu, Dazhi
Ji, Yanda
Liu, Jindong
Zhang, Lei
Pi, Li
Zhang, Yuheng
Yang, Hao
Evolution of the intrinsic electronic phase separation in La(0.6)Er(0.1)Sr(0.3)MnO(3) perovskite
title Evolution of the intrinsic electronic phase separation in La(0.6)Er(0.1)Sr(0.3)MnO(3) perovskite
title_full Evolution of the intrinsic electronic phase separation in La(0.6)Er(0.1)Sr(0.3)MnO(3) perovskite
title_fullStr Evolution of the intrinsic electronic phase separation in La(0.6)Er(0.1)Sr(0.3)MnO(3) perovskite
title_full_unstemmed Evolution of the intrinsic electronic phase separation in La(0.6)Er(0.1)Sr(0.3)MnO(3) perovskite
title_short Evolution of the intrinsic electronic phase separation in La(0.6)Er(0.1)Sr(0.3)MnO(3) perovskite
title_sort evolution of the intrinsic electronic phase separation in la(0.6)er(0.1)sr(0.3)mno(3) perovskite
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5431341/
https://www.ncbi.nlm.nih.gov/pubmed/28442764
http://dx.doi.org/10.1038/s41598-016-0009-0
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