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Unconventional electron states in δ-doped SmTiO(3)

The Mott-insulating distorted perovskite SmTiO(3), doped with a single SrO layer in a quantum-well architecture is studied by the combination of density functional theory with dynamical mean-field theory. A rich correlated electronic structure in line with recent experimental investigations is revea...

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Detalles Bibliográficos
Autor principal: Lechermann, Frank
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2017
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5431486/
https://www.ncbi.nlm.nih.gov/pubmed/28484238
http://dx.doi.org/10.1038/s41598-017-01847-5
Descripción
Sumario:The Mott-insulating distorted perovskite SmTiO(3), doped with a single SrO layer in a quantum-well architecture is studied by the combination of density functional theory with dynamical mean-field theory. A rich correlated electronic structure in line with recent experimental investigations is revealed by the given realistic many-body approach to a large-unit-cell oxide heterostructure. Coexistence of conducting and Mott-insulating TiO(2) layers prone to magnetic order gives rise to multi-orbital electronic transport beyond standard Fermi-liquid theory. First hints towards a pseudogap opening due to electron-electron scattering within a background of ferromagnetic and antiferromagnetic fluctuations are detected.