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Molecular alignment in degenerated dissociation channels in strong laser fields
In this work, we study strong-field molecular alignment in, for the first time, degenerated channels following the same charged states of molecules. By measuring the angular distribution of dissociation fragments from two degenerated N(+) + N(+) channels of N(2), we observe an opposite angular distr...
Autores principales: | , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2017
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5451389/ https://www.ncbi.nlm.nih.gov/pubmed/28566695 http://dx.doi.org/10.1038/s41598-017-02738-5 |
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author | Lai, Wei Heins, Alan Guo, Chunlei |
author_facet | Lai, Wei Heins, Alan Guo, Chunlei |
author_sort | Lai, Wei |
collection | PubMed |
description | In this work, we study strong-field molecular alignment in, for the first time, degenerated channels following the same charged states of molecules. By measuring the angular distribution of dissociation fragments from two degenerated N(+) + N(+) channels of N(2), we observe an opposite angular distribution development in these two channels, one expanding and one contracting, when the laser intensity increases. Our further study shows that the expanding channel comes from a nonsequential transition, while the contracting channel involves a sequential transition. We also study the time sequence of the sequential and nonsequential transitions and find that the opposite angular distribution development is due to the different degrees of molecular alignment in these two degenerated channels. |
format | Online Article Text |
id | pubmed-5451389 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2017 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-54513892017-06-01 Molecular alignment in degenerated dissociation channels in strong laser fields Lai, Wei Heins, Alan Guo, Chunlei Sci Rep Article In this work, we study strong-field molecular alignment in, for the first time, degenerated channels following the same charged states of molecules. By measuring the angular distribution of dissociation fragments from two degenerated N(+) + N(+) channels of N(2), we observe an opposite angular distribution development in these two channels, one expanding and one contracting, when the laser intensity increases. Our further study shows that the expanding channel comes from a nonsequential transition, while the contracting channel involves a sequential transition. We also study the time sequence of the sequential and nonsequential transitions and find that the opposite angular distribution development is due to the different degrees of molecular alignment in these two degenerated channels. Nature Publishing Group UK 2017-05-31 /pmc/articles/PMC5451389/ /pubmed/28566695 http://dx.doi.org/10.1038/s41598-017-02738-5 Text en © The Author(s) 2017 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Lai, Wei Heins, Alan Guo, Chunlei Molecular alignment in degenerated dissociation channels in strong laser fields |
title | Molecular alignment in degenerated dissociation channels in strong laser fields |
title_full | Molecular alignment in degenerated dissociation channels in strong laser fields |
title_fullStr | Molecular alignment in degenerated dissociation channels in strong laser fields |
title_full_unstemmed | Molecular alignment in degenerated dissociation channels in strong laser fields |
title_short | Molecular alignment in degenerated dissociation channels in strong laser fields |
title_sort | molecular alignment in degenerated dissociation channels in strong laser fields |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5451389/ https://www.ncbi.nlm.nih.gov/pubmed/28566695 http://dx.doi.org/10.1038/s41598-017-02738-5 |
work_keys_str_mv | AT laiwei molecularalignmentindegenerateddissociationchannelsinstronglaserfields AT heinsalan molecularalignmentindegenerateddissociationchannelsinstronglaserfields AT guochunlei molecularalignmentindegenerateddissociationchannelsinstronglaserfields |