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Coherent structural trapping through wave packet dispersion during photoinduced spin state switching

The description of ultrafast nonadiabatic chemical dynamics during molecular photo-transformations remains challenging because electronic and nuclear configurations impact each other and cannot be treated independently. Here we gain experimental insights, beyond the Born–Oppenheimer approximation, i...

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Detalles Bibliográficos
Autores principales: Lemke, Henrik T., Kjær, Kasper S., Hartsock, Robert, van Driel, Tim B., Chollet, Matthieu, Glownia, James M., Song, Sanghoon, Zhu, Diling, Pace, Elisabetta, Matar, Samir F., Nielsen, Martin M., Benfatto, Maurizio, Gaffney, Kelly J., Collet, Eric, Cammarata, Marco
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group 2017
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5458100/
https://www.ncbi.nlm.nih.gov/pubmed/28537270
http://dx.doi.org/10.1038/ncomms15342

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