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Ultra-low threshold polariton lasing at room temperature in a GaN membrane microcavity with a zero-dimensional trap

Polariton lasers are coherent light sources based on the condensation of exciton-polaritons in semiconductor microcavities, which occurs either in the kinetic or thermodynamic (Bose-Einstein) regime. Besides their fundamental interest, polariton lasers have the potential of extremely low operating t...

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Autores principales: Jayaprakash, R., Kalaitzakis, F. G., Christmann, G., Tsagaraki, K., Hocevar, M., Gayral, B., Monroy, E., Pelekanos, N. T.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2017
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5514101/
https://www.ncbi.nlm.nih.gov/pubmed/28717162
http://dx.doi.org/10.1038/s41598-017-06125-y
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author Jayaprakash, R.
Kalaitzakis, F. G.
Christmann, G.
Tsagaraki, K.
Hocevar, M.
Gayral, B.
Monroy, E.
Pelekanos, N. T.
author_facet Jayaprakash, R.
Kalaitzakis, F. G.
Christmann, G.
Tsagaraki, K.
Hocevar, M.
Gayral, B.
Monroy, E.
Pelekanos, N. T.
author_sort Jayaprakash, R.
collection PubMed
description Polariton lasers are coherent light sources based on the condensation of exciton-polaritons in semiconductor microcavities, which occurs either in the kinetic or thermodynamic (Bose-Einstein) regime. Besides their fundamental interest, polariton lasers have the potential of extremely low operating thresholds. Here, we demonstrate ultra-low threshold polariton lasing at room temperature, using an all-dielectric, GaN membrane-based microcavity, with a spontaneously-formed zero-dimensional trap. The microcavity is fabricated using an innovative method, which involves photo-electrochemical etching of an InGaN sacrificial layer and allows for the incorporation of optimally-grown GaN active quantum wells inside a cavity with atomically-smooth surfaces. The resulting structure presents near-theoretical Q-factors and pronounced strong-coupling effects, with a record-high Rabi splitting of 64 meV at room-temperature. Polariton lasing is observed at threshold carrier densities 2.5 orders of magnitude lower than the exciton saturation density. Above threshold, angle-resolved emission spectra reveal an ordered pattern in k-space, attributed to polariton condensation at discrete levels of a single confinement site. This confinement mechanism along with the high material and optical quality of the microcavity, accounts for the enhanced performance of our polariton laser, and pave the way for further developments in the area of robust room temperature polaritonic devices.
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spelling pubmed-55141012017-07-19 Ultra-low threshold polariton lasing at room temperature in a GaN membrane microcavity with a zero-dimensional trap Jayaprakash, R. Kalaitzakis, F. G. Christmann, G. Tsagaraki, K. Hocevar, M. Gayral, B. Monroy, E. Pelekanos, N. T. Sci Rep Article Polariton lasers are coherent light sources based on the condensation of exciton-polaritons in semiconductor microcavities, which occurs either in the kinetic or thermodynamic (Bose-Einstein) regime. Besides their fundamental interest, polariton lasers have the potential of extremely low operating thresholds. Here, we demonstrate ultra-low threshold polariton lasing at room temperature, using an all-dielectric, GaN membrane-based microcavity, with a spontaneously-formed zero-dimensional trap. The microcavity is fabricated using an innovative method, which involves photo-electrochemical etching of an InGaN sacrificial layer and allows for the incorporation of optimally-grown GaN active quantum wells inside a cavity with atomically-smooth surfaces. The resulting structure presents near-theoretical Q-factors and pronounced strong-coupling effects, with a record-high Rabi splitting of 64 meV at room-temperature. Polariton lasing is observed at threshold carrier densities 2.5 orders of magnitude lower than the exciton saturation density. Above threshold, angle-resolved emission spectra reveal an ordered pattern in k-space, attributed to polariton condensation at discrete levels of a single confinement site. This confinement mechanism along with the high material and optical quality of the microcavity, accounts for the enhanced performance of our polariton laser, and pave the way for further developments in the area of robust room temperature polaritonic devices. Nature Publishing Group UK 2017-07-17 /pmc/articles/PMC5514101/ /pubmed/28717162 http://dx.doi.org/10.1038/s41598-017-06125-y Text en © The Author(s) 2017 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Jayaprakash, R.
Kalaitzakis, F. G.
Christmann, G.
Tsagaraki, K.
Hocevar, M.
Gayral, B.
Monroy, E.
Pelekanos, N. T.
Ultra-low threshold polariton lasing at room temperature in a GaN membrane microcavity with a zero-dimensional trap
title Ultra-low threshold polariton lasing at room temperature in a GaN membrane microcavity with a zero-dimensional trap
title_full Ultra-low threshold polariton lasing at room temperature in a GaN membrane microcavity with a zero-dimensional trap
title_fullStr Ultra-low threshold polariton lasing at room temperature in a GaN membrane microcavity with a zero-dimensional trap
title_full_unstemmed Ultra-low threshold polariton lasing at room temperature in a GaN membrane microcavity with a zero-dimensional trap
title_short Ultra-low threshold polariton lasing at room temperature in a GaN membrane microcavity with a zero-dimensional trap
title_sort ultra-low threshold polariton lasing at room temperature in a gan membrane microcavity with a zero-dimensional trap
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5514101/
https://www.ncbi.nlm.nih.gov/pubmed/28717162
http://dx.doi.org/10.1038/s41598-017-06125-y
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