Cargando…

Nano-plasmonic near field phase matching of attosecond pulses

Nano-structures excited by light can enhance locally the electric field when tuned to plasmonic resonances. This phenomenon can be used to boost non-linear processes such as harmonic generation in crystals or in gases, Raman excitation, and four wave mixing. Here we present a theoretical investigati...

Descripción completa

Detalles Bibliográficos
Autores principales: Shaaran, Tahir, Nicolas, Rana, Iwan, Bianca, Kovacev, Milutin, Merdji, Hamed
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2017
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5527109/
https://www.ncbi.nlm.nih.gov/pubmed/28743976
http://dx.doi.org/10.1038/s41598-017-06491-7
_version_ 1783252920336121856
author Shaaran, Tahir
Nicolas, Rana
Iwan, Bianca
Kovacev, Milutin
Merdji, Hamed
author_facet Shaaran, Tahir
Nicolas, Rana
Iwan, Bianca
Kovacev, Milutin
Merdji, Hamed
author_sort Shaaran, Tahir
collection PubMed
description Nano-structures excited by light can enhance locally the electric field when tuned to plasmonic resonances. This phenomenon can be used to boost non-linear processes such as harmonic generation in crystals or in gases, Raman excitation, and four wave mixing. Here we present a theoretical investigation of the near-field phase matching of attosecond pulses emitted by high-order harmonic generation (HHG) of an atom immersed in a multi-cycle femtosecond infrared laser field and a spatially inhomogeneous plasmonic field. We demonstrate that the spatial inhomogeneity factor of the plasmonic field strongly affects the electron trajectory and recombination time which can be used to control the attosecond emission. For further insight into the plasmonic field effect, we monitor the phase of each quantum path as a function of the inhomogeneity strength. Moreover, we investigate the attosecond emission as a function of near-field phase matching effects. This is achieved by calculating the coherent field superposition of attosecond pulses emitted from various intensities or field inhomogeneities. Finally, far-field and near-field phase matching effects are combined to modulate the harmonic spectral phase towards the emission of a single attosecond pulse.
format Online
Article
Text
id pubmed-5527109
institution National Center for Biotechnology Information
language English
publishDate 2017
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-55271092017-08-02 Nano-plasmonic near field phase matching of attosecond pulses Shaaran, Tahir Nicolas, Rana Iwan, Bianca Kovacev, Milutin Merdji, Hamed Sci Rep Article Nano-structures excited by light can enhance locally the electric field when tuned to plasmonic resonances. This phenomenon can be used to boost non-linear processes such as harmonic generation in crystals or in gases, Raman excitation, and four wave mixing. Here we present a theoretical investigation of the near-field phase matching of attosecond pulses emitted by high-order harmonic generation (HHG) of an atom immersed in a multi-cycle femtosecond infrared laser field and a spatially inhomogeneous plasmonic field. We demonstrate that the spatial inhomogeneity factor of the plasmonic field strongly affects the electron trajectory and recombination time which can be used to control the attosecond emission. For further insight into the plasmonic field effect, we monitor the phase of each quantum path as a function of the inhomogeneity strength. Moreover, we investigate the attosecond emission as a function of near-field phase matching effects. This is achieved by calculating the coherent field superposition of attosecond pulses emitted from various intensities or field inhomogeneities. Finally, far-field and near-field phase matching effects are combined to modulate the harmonic spectral phase towards the emission of a single attosecond pulse. Nature Publishing Group UK 2017-07-25 /pmc/articles/PMC5527109/ /pubmed/28743976 http://dx.doi.org/10.1038/s41598-017-06491-7 Text en © The Author(s) 2017 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Shaaran, Tahir
Nicolas, Rana
Iwan, Bianca
Kovacev, Milutin
Merdji, Hamed
Nano-plasmonic near field phase matching of attosecond pulses
title Nano-plasmonic near field phase matching of attosecond pulses
title_full Nano-plasmonic near field phase matching of attosecond pulses
title_fullStr Nano-plasmonic near field phase matching of attosecond pulses
title_full_unstemmed Nano-plasmonic near field phase matching of attosecond pulses
title_short Nano-plasmonic near field phase matching of attosecond pulses
title_sort nano-plasmonic near field phase matching of attosecond pulses
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5527109/
https://www.ncbi.nlm.nih.gov/pubmed/28743976
http://dx.doi.org/10.1038/s41598-017-06491-7
work_keys_str_mv AT shaarantahir nanoplasmonicnearfieldphasematchingofattosecondpulses
AT nicolasrana nanoplasmonicnearfieldphasematchingofattosecondpulses
AT iwanbianca nanoplasmonicnearfieldphasematchingofattosecondpulses
AT kovacevmilutin nanoplasmonicnearfieldphasematchingofattosecondpulses
AT merdjihamed nanoplasmonicnearfieldphasematchingofattosecondpulses