Cargando…

A room temperature continuous-wave nanolaser using colloidal quantum wells

Colloidal semiconductor nanocrystals have emerged as promising active materials for solution-processable optoelectronic and light-emitting devices. In particular, the development of nanocrystal lasers is currently experiencing rapid progress. However, these lasers require large pump powers, and real...

Descripción completa

Detalles Bibliográficos
Autores principales: Yang, Zhili, Pelton, Matthew, Fedin, Igor, Talapin, Dmitri V., Waks, Edo
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2017
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5529567/
https://www.ncbi.nlm.nih.gov/pubmed/28747633
http://dx.doi.org/10.1038/s41467-017-00198-z
_version_ 1783253152244432896
author Yang, Zhili
Pelton, Matthew
Fedin, Igor
Talapin, Dmitri V.
Waks, Edo
author_facet Yang, Zhili
Pelton, Matthew
Fedin, Igor
Talapin, Dmitri V.
Waks, Edo
author_sort Yang, Zhili
collection PubMed
description Colloidal semiconductor nanocrystals have emerged as promising active materials for solution-processable optoelectronic and light-emitting devices. In particular, the development of nanocrystal lasers is currently experiencing rapid progress. However, these lasers require large pump powers, and realizing an efficient low-power nanocrystal laser has remained a difficult challenge. Here, we demonstrate a nanolaser using colloidal nanocrystals that exhibits a threshold input power of less than 1 μW, a very low threshold for any laser using colloidal emitters. We use CdSe/CdS core-shell nanoplatelets, which are efficient nanocrystal emitters with the electronic structure of quantum wells, coupled to a photonic-crystal nanobeam cavity that attains high coupling efficiencies. The device achieves stable continuous-wave lasing at room temperature, which is essential for many photonic and optoelectronic applications. Our results show that colloidal nanocrystals are suitable for compact and efficient optoelectronic devices based on versatile and inexpensive solution-processable materials.
format Online
Article
Text
id pubmed-5529567
institution National Center for Biotechnology Information
language English
publishDate 2017
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-55295672017-08-01 A room temperature continuous-wave nanolaser using colloidal quantum wells Yang, Zhili Pelton, Matthew Fedin, Igor Talapin, Dmitri V. Waks, Edo Nat Commun Article Colloidal semiconductor nanocrystals have emerged as promising active materials for solution-processable optoelectronic and light-emitting devices. In particular, the development of nanocrystal lasers is currently experiencing rapid progress. However, these lasers require large pump powers, and realizing an efficient low-power nanocrystal laser has remained a difficult challenge. Here, we demonstrate a nanolaser using colloidal nanocrystals that exhibits a threshold input power of less than 1 μW, a very low threshold for any laser using colloidal emitters. We use CdSe/CdS core-shell nanoplatelets, which are efficient nanocrystal emitters with the electronic structure of quantum wells, coupled to a photonic-crystal nanobeam cavity that attains high coupling efficiencies. The device achieves stable continuous-wave lasing at room temperature, which is essential for many photonic and optoelectronic applications. Our results show that colloidal nanocrystals are suitable for compact and efficient optoelectronic devices based on versatile and inexpensive solution-processable materials. Nature Publishing Group UK 2017-07-26 /pmc/articles/PMC5529567/ /pubmed/28747633 http://dx.doi.org/10.1038/s41467-017-00198-z Text en © The Author(s) 2017 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Yang, Zhili
Pelton, Matthew
Fedin, Igor
Talapin, Dmitri V.
Waks, Edo
A room temperature continuous-wave nanolaser using colloidal quantum wells
title A room temperature continuous-wave nanolaser using colloidal quantum wells
title_full A room temperature continuous-wave nanolaser using colloidal quantum wells
title_fullStr A room temperature continuous-wave nanolaser using colloidal quantum wells
title_full_unstemmed A room temperature continuous-wave nanolaser using colloidal quantum wells
title_short A room temperature continuous-wave nanolaser using colloidal quantum wells
title_sort room temperature continuous-wave nanolaser using colloidal quantum wells
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5529567/
https://www.ncbi.nlm.nih.gov/pubmed/28747633
http://dx.doi.org/10.1038/s41467-017-00198-z
work_keys_str_mv AT yangzhili aroomtemperaturecontinuouswavenanolaserusingcolloidalquantumwells
AT peltonmatthew aroomtemperaturecontinuouswavenanolaserusingcolloidalquantumwells
AT fedinigor aroomtemperaturecontinuouswavenanolaserusingcolloidalquantumwells
AT talapindmitriv aroomtemperaturecontinuouswavenanolaserusingcolloidalquantumwells
AT waksedo aroomtemperaturecontinuouswavenanolaserusingcolloidalquantumwells
AT yangzhili roomtemperaturecontinuouswavenanolaserusingcolloidalquantumwells
AT peltonmatthew roomtemperaturecontinuouswavenanolaserusingcolloidalquantumwells
AT fedinigor roomtemperaturecontinuouswavenanolaserusingcolloidalquantumwells
AT talapindmitriv roomtemperaturecontinuouswavenanolaserusingcolloidalquantumwells
AT waksedo roomtemperaturecontinuouswavenanolaserusingcolloidalquantumwells