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53-attosecond X-ray pulses reach the carbon K-edge

The motion of electrons in the microcosm occurs on a time scale set by the atomic unit of time—24 attoseconds. Attosecond pulses at photon energies corresponding to the fundamental absorption edges of matter, which lie in the soft X-ray regime above 200 eV, permit the probing of electronic excitatio...

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Detalles Bibliográficos
Autores principales: Li, Jie, Ren, Xiaoming, Yin, Yanchun, Zhao, Kun, Chew, Andrew, Cheng, Yan, Cunningham, Eric, Wang, Yang, Hu, Shuyuan, Wu, Yi, Chini, Michael, Chang, Zenghu
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2017
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5543167/
https://www.ncbi.nlm.nih.gov/pubmed/28775272
http://dx.doi.org/10.1038/s41467-017-00321-0
Descripción
Sumario:The motion of electrons in the microcosm occurs on a time scale set by the atomic unit of time—24 attoseconds. Attosecond pulses at photon energies corresponding to the fundamental absorption edges of matter, which lie in the soft X-ray regime above 200 eV, permit the probing of electronic excitation, chemical state, and atomic structure. Here we demonstrate a soft X-ray pulse duration of 53 as and single pulse streaking reaching the carbon K-absorption edge (284 eV) by utilizing intense two-cycle driving pulses near 1.8-μm center wavelength. Such pulses permit studies of electron dynamics in live biological samples and next-generation electronic materials such as diamond.