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Structure of the magnetic excitations in the spin-1/2 triangular-lattice Heisenberg antiferromagnet Ba(3)CoSb(2)O(9)

A spin-1/2 triangular-lattice Heisenberg antiferromagnet (TLHAF) is a prototypical frustrated quantum magnet, which exhibits remarkable quantum many-body effects that arise from the synergy between spin frustration and quantum fluctuation. The ground-state properties of a spin-1/2 TLHAF are theoreti...

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Autores principales: Ito, Saya, Kurita, Nobuyuki, Tanaka, Hidekazu, Ohira-Kawamura, Seiko, Nakajima, Kenji, Itoh, Shinichi, Kuwahara, Keitaro, Kakurai, Kazuhisa
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2017
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5550445/
https://www.ncbi.nlm.nih.gov/pubmed/28794443
http://dx.doi.org/10.1038/s41467-017-00316-x
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author Ito, Saya
Kurita, Nobuyuki
Tanaka, Hidekazu
Ohira-Kawamura, Seiko
Nakajima, Kenji
Itoh, Shinichi
Kuwahara, Keitaro
Kakurai, Kazuhisa
author_facet Ito, Saya
Kurita, Nobuyuki
Tanaka, Hidekazu
Ohira-Kawamura, Seiko
Nakajima, Kenji
Itoh, Shinichi
Kuwahara, Keitaro
Kakurai, Kazuhisa
author_sort Ito, Saya
collection PubMed
description A spin-1/2 triangular-lattice Heisenberg antiferromagnet (TLHAF) is a prototypical frustrated quantum magnet, which exhibits remarkable quantum many-body effects that arise from the synergy between spin frustration and quantum fluctuation. The ground-state properties of a spin-1/2 TLHAF are theoretically well understood. However, the theoretical consensus regarding the magnetic excitations is limited. The experimental study of the magnetic excitations in spin-1/2 TLHAFs has also been limited. Here we show the structure of magnetic excitations in the spin-1/2 TLHAF Ba(3)CoSb(2)O(9) investigated by inelastic neutron scattering. Significantly different from theoretical expectations, the excitation spectrum has a three-stage energy structure. The lowest-energy first stage is composed of dispersion branches of single-magnon excitations. The second and third stages are dispersive continua accompanied by a columnar continuum extending above 10 meV, which is six times larger than the exchange interaction J = 1.67 meV. Our results indicate the shortcomings of the current theoretical framework.
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spelling pubmed-55504452017-08-14 Structure of the magnetic excitations in the spin-1/2 triangular-lattice Heisenberg antiferromagnet Ba(3)CoSb(2)O(9) Ito, Saya Kurita, Nobuyuki Tanaka, Hidekazu Ohira-Kawamura, Seiko Nakajima, Kenji Itoh, Shinichi Kuwahara, Keitaro Kakurai, Kazuhisa Nat Commun Article A spin-1/2 triangular-lattice Heisenberg antiferromagnet (TLHAF) is a prototypical frustrated quantum magnet, which exhibits remarkable quantum many-body effects that arise from the synergy between spin frustration and quantum fluctuation. The ground-state properties of a spin-1/2 TLHAF are theoretically well understood. However, the theoretical consensus regarding the magnetic excitations is limited. The experimental study of the magnetic excitations in spin-1/2 TLHAFs has also been limited. Here we show the structure of magnetic excitations in the spin-1/2 TLHAF Ba(3)CoSb(2)O(9) investigated by inelastic neutron scattering. Significantly different from theoretical expectations, the excitation spectrum has a three-stage energy structure. The lowest-energy first stage is composed of dispersion branches of single-magnon excitations. The second and third stages are dispersive continua accompanied by a columnar continuum extending above 10 meV, which is six times larger than the exchange interaction J = 1.67 meV. Our results indicate the shortcomings of the current theoretical framework. Nature Publishing Group UK 2017-08-10 /pmc/articles/PMC5550445/ /pubmed/28794443 http://dx.doi.org/10.1038/s41467-017-00316-x Text en © The Author(s) 2017 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Ito, Saya
Kurita, Nobuyuki
Tanaka, Hidekazu
Ohira-Kawamura, Seiko
Nakajima, Kenji
Itoh, Shinichi
Kuwahara, Keitaro
Kakurai, Kazuhisa
Structure of the magnetic excitations in the spin-1/2 triangular-lattice Heisenberg antiferromagnet Ba(3)CoSb(2)O(9)
title Structure of the magnetic excitations in the spin-1/2 triangular-lattice Heisenberg antiferromagnet Ba(3)CoSb(2)O(9)
title_full Structure of the magnetic excitations in the spin-1/2 triangular-lattice Heisenberg antiferromagnet Ba(3)CoSb(2)O(9)
title_fullStr Structure of the magnetic excitations in the spin-1/2 triangular-lattice Heisenberg antiferromagnet Ba(3)CoSb(2)O(9)
title_full_unstemmed Structure of the magnetic excitations in the spin-1/2 triangular-lattice Heisenberg antiferromagnet Ba(3)CoSb(2)O(9)
title_short Structure of the magnetic excitations in the spin-1/2 triangular-lattice Heisenberg antiferromagnet Ba(3)CoSb(2)O(9)
title_sort structure of the magnetic excitations in the spin-1/2 triangular-lattice heisenberg antiferromagnet ba(3)cosb(2)o(9)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5550445/
https://www.ncbi.nlm.nih.gov/pubmed/28794443
http://dx.doi.org/10.1038/s41467-017-00316-x
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