Cargando…

Simulated sample heating from a nanofocused X-ray beam

Recent developments in synchrotron brilliance and X-ray optics are pushing the flux density in nanofocusing experiments to unprecedented levels, which increases the risk of different types of radiation damage. The effect of X-ray induced sample heating has been investigated using time-resolved and s...

Descripción completa

Detalles Bibliográficos
Autores principales: Wallander, Harald, Wallentin, Jesper
Formato: Online Artículo Texto
Lenguaje:English
Publicado: International Union of Crystallography 2017
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5580787/
https://www.ncbi.nlm.nih.gov/pubmed/28862614
http://dx.doi.org/10.1107/S1600577517008712
_version_ 1783260951961665536
author Wallander, Harald
Wallentin, Jesper
author_facet Wallander, Harald
Wallentin, Jesper
author_sort Wallander, Harald
collection PubMed
description Recent developments in synchrotron brilliance and X-ray optics are pushing the flux density in nanofocusing experiments to unprecedented levels, which increases the risk of different types of radiation damage. The effect of X-ray induced sample heating has been investigated using time-resolved and steady-state three-dimensional finite-element modelling of representative nanostructures. Simulations of a semiconductor nanowire indicate that the heat generated by X-ray absorption is efficiently transported within the nanowire, and that the temperature becomes homogeneous after about 5 ns. The most important channel for heat loss is conduction to the substrate, where the heat transfer coefficient and the interfacial area are limiting the heat transport. While convective heat transfer to air is significant, the thermal radiation is negligible. The steady-state average temperature in the nanowire is 8 K above room temperature at the reference parameters. In the absence of heat transfer to the substrate, the temperature increase at the same flux reaches 55 K in air and far beyond the melting temperature in vacuum. Reducing the size of the X-ray focus at constant flux only increases the maximum temperature marginally. These results suggest that the key strategy for reducing the X-ray induced heating is to improve the heat transfer to the surrounding.
format Online
Article
Text
id pubmed-5580787
institution National Center for Biotechnology Information
language English
publishDate 2017
publisher International Union of Crystallography
record_format MEDLINE/PubMed
spelling pubmed-55807872017-09-05 Simulated sample heating from a nanofocused X-ray beam Wallander, Harald Wallentin, Jesper J Synchrotron Radiat Research Papers Recent developments in synchrotron brilliance and X-ray optics are pushing the flux density in nanofocusing experiments to unprecedented levels, which increases the risk of different types of radiation damage. The effect of X-ray induced sample heating has been investigated using time-resolved and steady-state three-dimensional finite-element modelling of representative nanostructures. Simulations of a semiconductor nanowire indicate that the heat generated by X-ray absorption is efficiently transported within the nanowire, and that the temperature becomes homogeneous after about 5 ns. The most important channel for heat loss is conduction to the substrate, where the heat transfer coefficient and the interfacial area are limiting the heat transport. While convective heat transfer to air is significant, the thermal radiation is negligible. The steady-state average temperature in the nanowire is 8 K above room temperature at the reference parameters. In the absence of heat transfer to the substrate, the temperature increase at the same flux reaches 55 K in air and far beyond the melting temperature in vacuum. Reducing the size of the X-ray focus at constant flux only increases the maximum temperature marginally. These results suggest that the key strategy for reducing the X-ray induced heating is to improve the heat transfer to the surrounding. International Union of Crystallography 2017-08-02 /pmc/articles/PMC5580787/ /pubmed/28862614 http://dx.doi.org/10.1107/S1600577517008712 Text en © Wallander and Wallentin 2017 http://creativecommons.org/licenses/by/2.0/uk/ This is an open-access article distributed under the terms of the Creative Commons Attribution (CC-BY) Licence, which permits unrestricted use, distribution, and reproduction in any medium, provided the original authors and source are cited.http://creativecommons.org/licenses/by/2.0/uk/
spellingShingle Research Papers
Wallander, Harald
Wallentin, Jesper
Simulated sample heating from a nanofocused X-ray beam
title Simulated sample heating from a nanofocused X-ray beam
title_full Simulated sample heating from a nanofocused X-ray beam
title_fullStr Simulated sample heating from a nanofocused X-ray beam
title_full_unstemmed Simulated sample heating from a nanofocused X-ray beam
title_short Simulated sample heating from a nanofocused X-ray beam
title_sort simulated sample heating from a nanofocused x-ray beam
topic Research Papers
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5580787/
https://www.ncbi.nlm.nih.gov/pubmed/28862614
http://dx.doi.org/10.1107/S1600577517008712
work_keys_str_mv AT wallanderharald simulatedsampleheatingfromananofocusedxraybeam
AT wallentinjesper simulatedsampleheatingfromananofocusedxraybeam