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Infrared probe of pseudogap in electron-doped Sr(2)IrO(4)

We report on infrared spectroscopy experiments on the electronic response in (Sr(1−x)La(x))(2)IrO(4) (x = 0, 0.021, and 0.067). Our data show that electron doping induced by La substitution leads to an insulator-to-metal transition. The evolution of the electronic structure across the transition rev...

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Autores principales: Seo, J. H., Ahn, G. H., Song, S. J., Chen, X., Wilson, S. D., Moon, S. J.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2017
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5585243/
https://www.ncbi.nlm.nih.gov/pubmed/28874789
http://dx.doi.org/10.1038/s41598-017-10725-z
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author Seo, J. H.
Ahn, G. H.
Song, S. J.
Chen, X.
Wilson, S. D.
Moon, S. J.
author_facet Seo, J. H.
Ahn, G. H.
Song, S. J.
Chen, X.
Wilson, S. D.
Moon, S. J.
author_sort Seo, J. H.
collection PubMed
description We report on infrared spectroscopy experiments on the electronic response in (Sr(1−x)La(x))(2)IrO(4) (x = 0, 0.021, and 0.067). Our data show that electron doping induced by La substitution leads to an insulator-to-metal transition. The evolution of the electronic structure across the transition reveals the robustness of the strong electronic correlations against the electron doping. The conductivity data of the metallic compound show the signature of the pseudogap that bears close similarity to the analogous studies of the pseudogap in the underdoped cuprates. While the low energy conductivity of the metallic compound is barely frequency dependent, the formation of the pseudogap is revealed by the gradual suppression of the featureless conductivity below a threshold frequency of about 17 meV. The threshold structure develops below about 100 K which is in the vicinity of the onset of the short-range antiferromagnetic order. Our results demonstrate that the electronic correlations play a crucial role in the anomalous charge dynamics in the (Sr(1−x)La(x))(2)IrO(4) system.
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spelling pubmed-55852432017-09-06 Infrared probe of pseudogap in electron-doped Sr(2)IrO(4) Seo, J. H. Ahn, G. H. Song, S. J. Chen, X. Wilson, S. D. Moon, S. J. Sci Rep Article We report on infrared spectroscopy experiments on the electronic response in (Sr(1−x)La(x))(2)IrO(4) (x = 0, 0.021, and 0.067). Our data show that electron doping induced by La substitution leads to an insulator-to-metal transition. The evolution of the electronic structure across the transition reveals the robustness of the strong electronic correlations against the electron doping. The conductivity data of the metallic compound show the signature of the pseudogap that bears close similarity to the analogous studies of the pseudogap in the underdoped cuprates. While the low energy conductivity of the metallic compound is barely frequency dependent, the formation of the pseudogap is revealed by the gradual suppression of the featureless conductivity below a threshold frequency of about 17 meV. The threshold structure develops below about 100 K which is in the vicinity of the onset of the short-range antiferromagnetic order. Our results demonstrate that the electronic correlations play a crucial role in the anomalous charge dynamics in the (Sr(1−x)La(x))(2)IrO(4) system. Nature Publishing Group UK 2017-09-05 /pmc/articles/PMC5585243/ /pubmed/28874789 http://dx.doi.org/10.1038/s41598-017-10725-z Text en © The Author(s) 2017 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Seo, J. H.
Ahn, G. H.
Song, S. J.
Chen, X.
Wilson, S. D.
Moon, S. J.
Infrared probe of pseudogap in electron-doped Sr(2)IrO(4)
title Infrared probe of pseudogap in electron-doped Sr(2)IrO(4)
title_full Infrared probe of pseudogap in electron-doped Sr(2)IrO(4)
title_fullStr Infrared probe of pseudogap in electron-doped Sr(2)IrO(4)
title_full_unstemmed Infrared probe of pseudogap in electron-doped Sr(2)IrO(4)
title_short Infrared probe of pseudogap in electron-doped Sr(2)IrO(4)
title_sort infrared probe of pseudogap in electron-doped sr(2)iro(4)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5585243/
https://www.ncbi.nlm.nih.gov/pubmed/28874789
http://dx.doi.org/10.1038/s41598-017-10725-z
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