Cargando…

Visual Understanding of Light Absorption and Waveguiding in Standing Nanowires with 3D Fluorescence Confocal Microscopy

[Image: see text] Semiconductor nanowires are promising building blocks for next-generation photonics. Indirect proofs of large absorption cross sections have been reported in nanostructures with subwavelength diameters, an effect that is even more prominent in vertically standing nanowires. In this...

Descripción completa

Detalles Bibliográficos
Autores principales: Frederiksen, Rune, Tutuncuoglu, Gozde, Matteini, Federico, Martinez, Karen L., Fontcuberta i Morral, Anna, Alarcon-Llado, Esther
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2017
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5617333/
https://www.ncbi.nlm.nih.gov/pubmed/28966933
http://dx.doi.org/10.1021/acsphotonics.7b00434
_version_ 1783266966506569728
author Frederiksen, Rune
Tutuncuoglu, Gozde
Matteini, Federico
Martinez, Karen L.
Fontcuberta i Morral, Anna
Alarcon-Llado, Esther
author_facet Frederiksen, Rune
Tutuncuoglu, Gozde
Matteini, Federico
Martinez, Karen L.
Fontcuberta i Morral, Anna
Alarcon-Llado, Esther
author_sort Frederiksen, Rune
collection PubMed
description [Image: see text] Semiconductor nanowires are promising building blocks for next-generation photonics. Indirect proofs of large absorption cross sections have been reported in nanostructures with subwavelength diameters, an effect that is even more prominent in vertically standing nanowires. In this work we provide a three-dimensional map of the light around vertical GaAs nanowires standing on a substrate by using fluorescence confocal microscopy, where the strong long-range disruption of the light path along the nanowire is illustrated. We find that the actual long-distance perturbation is much larger in size than calculated extinction cross sections. While the size of the perturbation remains similar, the intensity of the interaction changes dramatically over the visible spectrum. Numerical simulations allow us to distinguish the effects of scattering and absorption in the nanowire leading to these phenomena. This work provides a visual understanding of light absorption in semiconductor nanowire structures, which is of high interest for solar energy conversion applications.
format Online
Article
Text
id pubmed-5617333
institution National Center for Biotechnology Information
language English
publishDate 2017
publisher American Chemical Society
record_format MEDLINE/PubMed
spelling pubmed-56173332017-09-28 Visual Understanding of Light Absorption and Waveguiding in Standing Nanowires with 3D Fluorescence Confocal Microscopy Frederiksen, Rune Tutuncuoglu, Gozde Matteini, Federico Martinez, Karen L. Fontcuberta i Morral, Anna Alarcon-Llado, Esther ACS Photonics [Image: see text] Semiconductor nanowires are promising building blocks for next-generation photonics. Indirect proofs of large absorption cross sections have been reported in nanostructures with subwavelength diameters, an effect that is even more prominent in vertically standing nanowires. In this work we provide a three-dimensional map of the light around vertical GaAs nanowires standing on a substrate by using fluorescence confocal microscopy, where the strong long-range disruption of the light path along the nanowire is illustrated. We find that the actual long-distance perturbation is much larger in size than calculated extinction cross sections. While the size of the perturbation remains similar, the intensity of the interaction changes dramatically over the visible spectrum. Numerical simulations allow us to distinguish the effects of scattering and absorption in the nanowire leading to these phenomena. This work provides a visual understanding of light absorption in semiconductor nanowire structures, which is of high interest for solar energy conversion applications. American Chemical Society 2017-08-21 2017-09-20 /pmc/articles/PMC5617333/ /pubmed/28966933 http://dx.doi.org/10.1021/acsphotonics.7b00434 Text en Copyright © 2017 American Chemical Society This is an open access article published under a Creative Commons Non-Commercial No Derivative Works (CC-BY-NC-ND) Attribution License (http://pubs.acs.org/page/policy/authorchoice_ccbyncnd_termsofuse.html) , which permits copying and redistribution of the article, and creation of adaptations, all for non-commercial purposes.
spellingShingle Frederiksen, Rune
Tutuncuoglu, Gozde
Matteini, Federico
Martinez, Karen L.
Fontcuberta i Morral, Anna
Alarcon-Llado, Esther
Visual Understanding of Light Absorption and Waveguiding in Standing Nanowires with 3D Fluorescence Confocal Microscopy
title Visual Understanding of Light Absorption and Waveguiding in Standing Nanowires with 3D Fluorescence Confocal Microscopy
title_full Visual Understanding of Light Absorption and Waveguiding in Standing Nanowires with 3D Fluorescence Confocal Microscopy
title_fullStr Visual Understanding of Light Absorption and Waveguiding in Standing Nanowires with 3D Fluorescence Confocal Microscopy
title_full_unstemmed Visual Understanding of Light Absorption and Waveguiding in Standing Nanowires with 3D Fluorescence Confocal Microscopy
title_short Visual Understanding of Light Absorption and Waveguiding in Standing Nanowires with 3D Fluorescence Confocal Microscopy
title_sort visual understanding of light absorption and waveguiding in standing nanowires with 3d fluorescence confocal microscopy
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5617333/
https://www.ncbi.nlm.nih.gov/pubmed/28966933
http://dx.doi.org/10.1021/acsphotonics.7b00434
work_keys_str_mv AT frederiksenrune visualunderstandingoflightabsorptionandwaveguidinginstandingnanowireswith3dfluorescenceconfocalmicroscopy
AT tutuncuoglugozde visualunderstandingoflightabsorptionandwaveguidinginstandingnanowireswith3dfluorescenceconfocalmicroscopy
AT matteinifederico visualunderstandingoflightabsorptionandwaveguidinginstandingnanowireswith3dfluorescenceconfocalmicroscopy
AT martinezkarenl visualunderstandingoflightabsorptionandwaveguidinginstandingnanowireswith3dfluorescenceconfocalmicroscopy
AT fontcubertaimorralanna visualunderstandingoflightabsorptionandwaveguidinginstandingnanowireswith3dfluorescenceconfocalmicroscopy
AT alarconlladoesther visualunderstandingoflightabsorptionandwaveguidinginstandingnanowireswith3dfluorescenceconfocalmicroscopy