Photothermal Catalysis: Photothermal Catalyst Engineering: Hydrogenation of Gaseous CO(2) with High Activity and Tailored Selectivity (Adv. Sci. 10/2017)

The size dependence of the photothermal effect of palladium nanocrystals enables the selectivity of the solar powered heterogeneous catalytic hydrogenation of carbon dioxide to be finely tailored towards producing either carbon monoxide through the reverse water gas shift reaction, CO(2) + H(2) → CO...

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Autores principales: Jia, Jia, Wang, Hong, Lu, Zhuole, O'Brien, Paul G., Ghoussoub, Mireille, Duchesne, Paul, Zheng, Ziqi, Li, Peicheng, Qiao, Qiao, Wang, Lu, Gu, Alan, Jelle, Abdinoor A., Dong, Yuchan, Wang, Qiang, Ghuman, Kulbir Kaur, Wood, Thomas, Qian, Chenxi, Shao, Yue, Qiu, Chenyue, Ye, Miaomiao, Zhu, Yimei, Lu, Zheng‐Hong, Zhang, Peng, Helmy, Amr S., Singh, Chandra Veer, Kherani, Nazir P., Perovic, Doug D., Ozin, Geoffrey A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: John Wiley and Sons Inc. 2017
Materias:
Back Cover
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5644238/
http://dx.doi.org/10.1002/advs.201770052
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author Jia, Jia
Wang, Hong
Lu, Zhuole
O'Brien, Paul G.
Ghoussoub, Mireille
Duchesne, Paul
Zheng, Ziqi
Li, Peicheng
Qiao, Qiao
Wang, Lu
Gu, Alan
Jelle, Abdinoor A.
Dong, Yuchan
Wang, Qiang
Ghuman, Kulbir Kaur
Wood, Thomas
Qian, Chenxi
Shao, Yue
Qiu, Chenyue
Ye, Miaomiao
Zhu, Yimei
Lu, Zheng‐Hong
Zhang, Peng
Helmy, Amr S.
Singh, Chandra Veer
Kherani, Nazir P.
Perovic, Doug D.
Ozin, Geoffrey A.
author_facet Jia, Jia
Wang, Hong
Lu, Zhuole
O'Brien, Paul G.
Ghoussoub, Mireille
Duchesne, Paul
Zheng, Ziqi
Li, Peicheng
Qiao, Qiao
Wang, Lu
Gu, Alan
Jelle, Abdinoor A.
Dong, Yuchan
Wang, Qiang
Ghuman, Kulbir Kaur
Wood, Thomas
Qian, Chenxi
Shao, Yue
Qiu, Chenyue
Ye, Miaomiao
Zhu, Yimei
Lu, Zheng‐Hong
Zhang, Peng
Helmy, Amr S.
Singh, Chandra Veer
Kherani, Nazir P.
Perovic, Doug D.
Ozin, Geoffrey A.
author_sort Jia, Jia
collection PubMed
description The size dependence of the photothermal effect of palladium nanocrystals enables the selectivity of the solar powered heterogeneous catalytic hydrogenation of carbon dioxide to be finely tailored towards producing either carbon monoxide through the reverse water gas shift reaction, CO(2) + H(2) → CO + H(2)O, favored for small nanocrystals or to methane, via the Sabatier methanation reaction, CO(2) + 4H(2) → CH(4) + 2H(2)O, preferred for larger nanocrystals. This is described by Geoffrey A. Ozin and co‐workers in article number 1700252. [Image: see text]
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spelling pubmed-56442382017-10-19 Photothermal Catalysis: Photothermal Catalyst Engineering: Hydrogenation of Gaseous CO(2) with High Activity and Tailored Selectivity (Adv. Sci. 10/2017) Jia, Jia Wang, Hong Lu, Zhuole O'Brien, Paul G. Ghoussoub, Mireille Duchesne, Paul Zheng, Ziqi Li, Peicheng Qiao, Qiao Wang, Lu Gu, Alan Jelle, Abdinoor A. Dong, Yuchan Wang, Qiang Ghuman, Kulbir Kaur Wood, Thomas Qian, Chenxi Shao, Yue Qiu, Chenyue Ye, Miaomiao Zhu, Yimei Lu, Zheng‐Hong Zhang, Peng Helmy, Amr S. Singh, Chandra Veer Kherani, Nazir P. Perovic, Doug D. Ozin, Geoffrey A. Adv Sci (Weinh) Back Cover The size dependence of the photothermal effect of palladium nanocrystals enables the selectivity of the solar powered heterogeneous catalytic hydrogenation of carbon dioxide to be finely tailored towards producing either carbon monoxide through the reverse water gas shift reaction, CO(2) + H(2) → CO + H(2)O, favored for small nanocrystals or to methane, via the Sabatier methanation reaction, CO(2) + 4H(2) → CH(4) + 2H(2)O, preferred for larger nanocrystals. This is described by Geoffrey A. Ozin and co‐workers in article number 1700252. [Image: see text] John Wiley and Sons Inc. 2017-10-17 /pmc/articles/PMC5644238/ http://dx.doi.org/10.1002/advs.201770052 Text en © 2017 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim This is an open access article under the terms of the Creative Commons Attribution‐NonCommercial (http://creativecommons.org/licenses/by-nc/4.0/) License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited and is not used for commercial purposes.
spellingShingle Back Cover
Jia, Jia
Wang, Hong
Lu, Zhuole
O'Brien, Paul G.
Ghoussoub, Mireille
Duchesne, Paul
Zheng, Ziqi
Li, Peicheng
Qiao, Qiao
Wang, Lu
Gu, Alan
Jelle, Abdinoor A.
Dong, Yuchan
Wang, Qiang
Ghuman, Kulbir Kaur
Wood, Thomas
Qian, Chenxi
Shao, Yue
Qiu, Chenyue
Ye, Miaomiao
Zhu, Yimei
Lu, Zheng‐Hong
Zhang, Peng
Helmy, Amr S.
Singh, Chandra Veer
Kherani, Nazir P.
Perovic, Doug D.
Ozin, Geoffrey A.
Photothermal Catalysis: Photothermal Catalyst Engineering: Hydrogenation of Gaseous CO(2) with High Activity and Tailored Selectivity (Adv. Sci. 10/2017)
title Photothermal Catalysis: Photothermal Catalyst Engineering: Hydrogenation of Gaseous CO(2) with High Activity and Tailored Selectivity (Adv. Sci. 10/2017)
title_full Photothermal Catalysis: Photothermal Catalyst Engineering: Hydrogenation of Gaseous CO(2) with High Activity and Tailored Selectivity (Adv. Sci. 10/2017)
title_fullStr Photothermal Catalysis: Photothermal Catalyst Engineering: Hydrogenation of Gaseous CO(2) with High Activity and Tailored Selectivity (Adv. Sci. 10/2017)
title_full_unstemmed Photothermal Catalysis: Photothermal Catalyst Engineering: Hydrogenation of Gaseous CO(2) with High Activity and Tailored Selectivity (Adv. Sci. 10/2017)
title_short Photothermal Catalysis: Photothermal Catalyst Engineering: Hydrogenation of Gaseous CO(2) with High Activity and Tailored Selectivity (Adv. Sci. 10/2017)
title_sort photothermal catalysis: photothermal catalyst engineering: hydrogenation of gaseous co(2) with high activity and tailored selectivity (adv. sci. 10/2017)
topic Back Cover
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5644238/
http://dx.doi.org/10.1002/advs.201770052
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