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Effect of Time-Delayed Feedback on the Interaction of a Dimer System with its Environment

In this work, we report modeling of non-Markovian open quantum systems, consisting of an excitonic dimer that displays memory effect due to time delayed interaction with its environment. We, indeed investigate the effect of these time delays on quantum coherence and excitation dynamical behavior in...

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Detalles Bibliográficos
Autores principales: Farhat, M., Kais, S., Alharbi, F. H.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2017
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5684406/
https://www.ncbi.nlm.nih.gov/pubmed/29133789
http://dx.doi.org/10.1038/s41598-017-15185-z
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author Farhat, M.
Kais, S.
Alharbi, F. H.
author_facet Farhat, M.
Kais, S.
Alharbi, F. H.
author_sort Farhat, M.
collection PubMed
description In this work, we report modeling of non-Markovian open quantum systems, consisting of an excitonic dimer that displays memory effect due to time delayed interaction with its environment. We, indeed investigate the effect of these time delays on quantum coherence and excitation dynamical behavior in the time domain generally considered for photosynthetic experiments (few hundred femtoseconds). In particular, we show that the coherence is maintained for periods proportional to time delays. Additionally, if delay is taken into account, coupling to the environment can be tuned to lower values, unlike in previous studies. This kind of intriguing effect can, therefore, when generalized to complete systems, permit more control on the experimental parameters, which may lead to more accurate description of the photosynthetic energy transfer functioning and subsequent applications in artificial photovoltaic research.
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spelling pubmed-56844062017-11-29 Effect of Time-Delayed Feedback on the Interaction of a Dimer System with its Environment Farhat, M. Kais, S. Alharbi, F. H. Sci Rep Article In this work, we report modeling of non-Markovian open quantum systems, consisting of an excitonic dimer that displays memory effect due to time delayed interaction with its environment. We, indeed investigate the effect of these time delays on quantum coherence and excitation dynamical behavior in the time domain generally considered for photosynthetic experiments (few hundred femtoseconds). In particular, we show that the coherence is maintained for periods proportional to time delays. Additionally, if delay is taken into account, coupling to the environment can be tuned to lower values, unlike in previous studies. This kind of intriguing effect can, therefore, when generalized to complete systems, permit more control on the experimental parameters, which may lead to more accurate description of the photosynthetic energy transfer functioning and subsequent applications in artificial photovoltaic research. Nature Publishing Group UK 2017-11-13 /pmc/articles/PMC5684406/ /pubmed/29133789 http://dx.doi.org/10.1038/s41598-017-15185-z Text en © The Author(s) 2017 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Farhat, M.
Kais, S.
Alharbi, F. H.
Effect of Time-Delayed Feedback on the Interaction of a Dimer System with its Environment
title Effect of Time-Delayed Feedback on the Interaction of a Dimer System with its Environment
title_full Effect of Time-Delayed Feedback on the Interaction of a Dimer System with its Environment
title_fullStr Effect of Time-Delayed Feedback on the Interaction of a Dimer System with its Environment
title_full_unstemmed Effect of Time-Delayed Feedback on the Interaction of a Dimer System with its Environment
title_short Effect of Time-Delayed Feedback on the Interaction of a Dimer System with its Environment
title_sort effect of time-delayed feedback on the interaction of a dimer system with its environment
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5684406/
https://www.ncbi.nlm.nih.gov/pubmed/29133789
http://dx.doi.org/10.1038/s41598-017-15185-z
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