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Direct observation of impact propagation and absorption in dense colloidal monolayers

Dense colloidal suspensions can propagate and absorb large mechanical stresses, including impacts and shocks. The wave transport stems from the delicate interplay between the spatial arrangement of the structural units and solvent-mediated effects. For dynamic microscopic systems, elastic deformatio...

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Autores principales: Buttinoni, Ivo, Cha, Jinwoong, Lin, Wei-Hsun, Job, Stéphane, Daraio, Chiara, Isa, Lucio
Formato: Online Artículo Texto
Lenguaje:English
Publicado: National Academy of Sciences 2017
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5699069/
https://www.ncbi.nlm.nih.gov/pubmed/29087329
http://dx.doi.org/10.1073/pnas.1712266114
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author Buttinoni, Ivo
Cha, Jinwoong
Lin, Wei-Hsun
Job, Stéphane
Daraio, Chiara
Isa, Lucio
author_facet Buttinoni, Ivo
Cha, Jinwoong
Lin, Wei-Hsun
Job, Stéphane
Daraio, Chiara
Isa, Lucio
author_sort Buttinoni, Ivo
collection PubMed
description Dense colloidal suspensions can propagate and absorb large mechanical stresses, including impacts and shocks. The wave transport stems from the delicate interplay between the spatial arrangement of the structural units and solvent-mediated effects. For dynamic microscopic systems, elastic deformations of the colloids are usually disregarded due to the damping imposed by the surrounding fluid. Here, we study the propagation of localized mechanical pulses in aqueous monolayers of micron-sized particles of controlled microstructure. We generate extreme localized deformation rates by exciting a target particle via pulsed-laser ablation. In crystalline monolayers, stress propagation fronts take place, where fast-moving particles (V approximately a few meters per second) are aligned along the symmetry axes of the lattice. Conversely, more viscous solvents and disordered structures lead to faster and isotropic energy absorption. Our results demonstrate the accessibility of a regime where elastic collisions also become relevant for suspensions of microscopic particles, behaving as “billiard balls” in a liquid, in analogy with regular packings of macroscopic spheres. We furthermore quantify the scattering of an impact as a function of the local structural disorder.
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spelling pubmed-56990692017-11-27 Direct observation of impact propagation and absorption in dense colloidal monolayers Buttinoni, Ivo Cha, Jinwoong Lin, Wei-Hsun Job, Stéphane Daraio, Chiara Isa, Lucio Proc Natl Acad Sci U S A Physical Sciences Dense colloidal suspensions can propagate and absorb large mechanical stresses, including impacts and shocks. The wave transport stems from the delicate interplay between the spatial arrangement of the structural units and solvent-mediated effects. For dynamic microscopic systems, elastic deformations of the colloids are usually disregarded due to the damping imposed by the surrounding fluid. Here, we study the propagation of localized mechanical pulses in aqueous monolayers of micron-sized particles of controlled microstructure. We generate extreme localized deformation rates by exciting a target particle via pulsed-laser ablation. In crystalline monolayers, stress propagation fronts take place, where fast-moving particles (V approximately a few meters per second) are aligned along the symmetry axes of the lattice. Conversely, more viscous solvents and disordered structures lead to faster and isotropic energy absorption. Our results demonstrate the accessibility of a regime where elastic collisions also become relevant for suspensions of microscopic particles, behaving as “billiard balls” in a liquid, in analogy with regular packings of macroscopic spheres. We furthermore quantify the scattering of an impact as a function of the local structural disorder. National Academy of Sciences 2017-11-14 2017-10-30 /pmc/articles/PMC5699069/ /pubmed/29087329 http://dx.doi.org/10.1073/pnas.1712266114 Text en Copyright © 2017 the Author(s). Published by PNAS. https://creativecommons.org/licenses/by-nc-nd/4.0/ This open access article is distributed under Creative Commons Attribution-NonCommercial-NoDerivatives License 4.0 (CC BY-NC-ND) (https://creativecommons.org/licenses/by-nc-nd/4.0/) .
spellingShingle Physical Sciences
Buttinoni, Ivo
Cha, Jinwoong
Lin, Wei-Hsun
Job, Stéphane
Daraio, Chiara
Isa, Lucio
Direct observation of impact propagation and absorption in dense colloidal monolayers
title Direct observation of impact propagation and absorption in dense colloidal monolayers
title_full Direct observation of impact propagation and absorption in dense colloidal monolayers
title_fullStr Direct observation of impact propagation and absorption in dense colloidal monolayers
title_full_unstemmed Direct observation of impact propagation and absorption in dense colloidal monolayers
title_short Direct observation of impact propagation and absorption in dense colloidal monolayers
title_sort direct observation of impact propagation and absorption in dense colloidal monolayers
topic Physical Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5699069/
https://www.ncbi.nlm.nih.gov/pubmed/29087329
http://dx.doi.org/10.1073/pnas.1712266114
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