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Study on Scattering and Absorption Properties of Quantum-Dot-Converted Elements for Light-Emitting Diodes Using Finite-Difference Time-Domain Method

CdSe/ZnS quantum-dot-converted elements (QDCEs) are good candidates for substituting rare-earth phosphor-converted elements (PCEs) in white light-emitting diodes (LEDs); however, studies on their scattering and absorption properties are scarce, suppressing further increment in the optical and therma...

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Autores principales: Li, Jiasheng, Tang, Yong, Li, Zongtao, Ding, Xinrui, Yuan, Dong, Yu, Binhai
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2017
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5706211/
https://www.ncbi.nlm.nih.gov/pubmed/29099759
http://dx.doi.org/10.3390/ma10111264
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author Li, Jiasheng
Tang, Yong
Li, Zongtao
Ding, Xinrui
Yuan, Dong
Yu, Binhai
author_facet Li, Jiasheng
Tang, Yong
Li, Zongtao
Ding, Xinrui
Yuan, Dong
Yu, Binhai
author_sort Li, Jiasheng
collection PubMed
description CdSe/ZnS quantum-dot-converted elements (QDCEs) are good candidates for substituting rare-earth phosphor-converted elements (PCEs) in white light-emitting diodes (LEDs); however, studies on their scattering and absorption properties are scarce, suppressing further increment in the optical and thermal performance of quantum-dot-converted LEDs. Therefore, we introduce the finite-difference time-domain (FDTD) method to achieve the critical optical parameters of QDCEs when used in white LEDs; their scattering cross-section (coefficient), absorption cross-section (coefficient), and scattering phase distributions are presented and compared with those of traditional YAG phosphor-converted elements (PCEs) at varying particle size and concentration. At a commonly used concentration ([Formula: see text]), QDCEs exhibit stronger absorption (tens of millimeters, even for green-to-red-wavelength light) and weaker scattering ([Formula: see text]) compared to PCEs; the reabsorption, total internal reflection, angular uniformity, and thermal quenching would be more significant concerns for QDCEs. Therefore, the unique scattering and absorption properties of QDCEs should be considered when used in white LEDs. Furthermore, knowledge of these important optical parameters is helpful for beginning a theoretical study on quantum-dot-converted LEDs according to the ray tracing method.
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spelling pubmed-57062112017-12-04 Study on Scattering and Absorption Properties of Quantum-Dot-Converted Elements for Light-Emitting Diodes Using Finite-Difference Time-Domain Method Li, Jiasheng Tang, Yong Li, Zongtao Ding, Xinrui Yuan, Dong Yu, Binhai Materials (Basel) Article CdSe/ZnS quantum-dot-converted elements (QDCEs) are good candidates for substituting rare-earth phosphor-converted elements (PCEs) in white light-emitting diodes (LEDs); however, studies on their scattering and absorption properties are scarce, suppressing further increment in the optical and thermal performance of quantum-dot-converted LEDs. Therefore, we introduce the finite-difference time-domain (FDTD) method to achieve the critical optical parameters of QDCEs when used in white LEDs; their scattering cross-section (coefficient), absorption cross-section (coefficient), and scattering phase distributions are presented and compared with those of traditional YAG phosphor-converted elements (PCEs) at varying particle size and concentration. At a commonly used concentration ([Formula: see text]), QDCEs exhibit stronger absorption (tens of millimeters, even for green-to-red-wavelength light) and weaker scattering ([Formula: see text]) compared to PCEs; the reabsorption, total internal reflection, angular uniformity, and thermal quenching would be more significant concerns for QDCEs. Therefore, the unique scattering and absorption properties of QDCEs should be considered when used in white LEDs. Furthermore, knowledge of these important optical parameters is helpful for beginning a theoretical study on quantum-dot-converted LEDs according to the ray tracing method. MDPI 2017-11-03 /pmc/articles/PMC5706211/ /pubmed/29099759 http://dx.doi.org/10.3390/ma10111264 Text en © 2017 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Li, Jiasheng
Tang, Yong
Li, Zongtao
Ding, Xinrui
Yuan, Dong
Yu, Binhai
Study on Scattering and Absorption Properties of Quantum-Dot-Converted Elements for Light-Emitting Diodes Using Finite-Difference Time-Domain Method
title Study on Scattering and Absorption Properties of Quantum-Dot-Converted Elements for Light-Emitting Diodes Using Finite-Difference Time-Domain Method
title_full Study on Scattering and Absorption Properties of Quantum-Dot-Converted Elements for Light-Emitting Diodes Using Finite-Difference Time-Domain Method
title_fullStr Study on Scattering and Absorption Properties of Quantum-Dot-Converted Elements for Light-Emitting Diodes Using Finite-Difference Time-Domain Method
title_full_unstemmed Study on Scattering and Absorption Properties of Quantum-Dot-Converted Elements for Light-Emitting Diodes Using Finite-Difference Time-Domain Method
title_short Study on Scattering and Absorption Properties of Quantum-Dot-Converted Elements for Light-Emitting Diodes Using Finite-Difference Time-Domain Method
title_sort study on scattering and absorption properties of quantum-dot-converted elements for light-emitting diodes using finite-difference time-domain method
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5706211/
https://www.ncbi.nlm.nih.gov/pubmed/29099759
http://dx.doi.org/10.3390/ma10111264
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