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Fine platinum nanoparticles supported on a porous ceramic membrane as efficient catalysts for the removal of benzene

It would be desirable to remove volatile organic compounds (VOCs) while we eliminate the dusts using silicon carbide (SiC)-based porous ceramics from the hot gases. Aiming at functionalizing SiC-based porous ceramics with catalytic capability, we herein report a facile strategy to integrate high eff...

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Autores principales: Liu, Hui, Li, Chengyin, Ren, Xiaoyong, Liu, Kaiqi, Yang, Jun
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2017
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5707434/
https://www.ncbi.nlm.nih.gov/pubmed/29185476
http://dx.doi.org/10.1038/s41598-017-16833-0
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author Liu, Hui
Li, Chengyin
Ren, Xiaoyong
Liu, Kaiqi
Yang, Jun
author_facet Liu, Hui
Li, Chengyin
Ren, Xiaoyong
Liu, Kaiqi
Yang, Jun
author_sort Liu, Hui
collection PubMed
description It would be desirable to remove volatile organic compounds (VOCs) while we eliminate the dusts using silicon carbide (SiC)-based porous ceramics from the hot gases. Aiming at functionalizing SiC-based porous ceramics with catalytic capability, we herein report a facile strategy to integrate high efficient catalysts into the porous SiC substrates for the VOC removal. We demonstrate an aqueous salt method for uniformly distributing fine platinum (Pt) particles on the alumina (Al(2)O(3)) layers, which are pre-coated on the SiC substrates as supports for VOC catalysts. We confirm that at a Pt mass loading as low as 0.176% and a weight hourly space velocity of 6000 mL g(−1) h(−1), the as-prepared Pt/SiC@Al(2)O(3) catalysts can convert 90% benzene at a temperature of ca. 215 °C. The results suggest a promising way to design ceramics-based bi-functional materials for simultaneously eliminating dusts and harmful VOCs from various hot gases.
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spelling pubmed-57074342017-12-06 Fine platinum nanoparticles supported on a porous ceramic membrane as efficient catalysts for the removal of benzene Liu, Hui Li, Chengyin Ren, Xiaoyong Liu, Kaiqi Yang, Jun Sci Rep Article It would be desirable to remove volatile organic compounds (VOCs) while we eliminate the dusts using silicon carbide (SiC)-based porous ceramics from the hot gases. Aiming at functionalizing SiC-based porous ceramics with catalytic capability, we herein report a facile strategy to integrate high efficient catalysts into the porous SiC substrates for the VOC removal. We demonstrate an aqueous salt method for uniformly distributing fine platinum (Pt) particles on the alumina (Al(2)O(3)) layers, which are pre-coated on the SiC substrates as supports for VOC catalysts. We confirm that at a Pt mass loading as low as 0.176% and a weight hourly space velocity of 6000 mL g(−1) h(−1), the as-prepared Pt/SiC@Al(2)O(3) catalysts can convert 90% benzene at a temperature of ca. 215 °C. The results suggest a promising way to design ceramics-based bi-functional materials for simultaneously eliminating dusts and harmful VOCs from various hot gases. Nature Publishing Group UK 2017-11-29 /pmc/articles/PMC5707434/ /pubmed/29185476 http://dx.doi.org/10.1038/s41598-017-16833-0 Text en © The Author(s) 2017 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Liu, Hui
Li, Chengyin
Ren, Xiaoyong
Liu, Kaiqi
Yang, Jun
Fine platinum nanoparticles supported on a porous ceramic membrane as efficient catalysts for the removal of benzene
title Fine platinum nanoparticles supported on a porous ceramic membrane as efficient catalysts for the removal of benzene
title_full Fine platinum nanoparticles supported on a porous ceramic membrane as efficient catalysts for the removal of benzene
title_fullStr Fine platinum nanoparticles supported on a porous ceramic membrane as efficient catalysts for the removal of benzene
title_full_unstemmed Fine platinum nanoparticles supported on a porous ceramic membrane as efficient catalysts for the removal of benzene
title_short Fine platinum nanoparticles supported on a porous ceramic membrane as efficient catalysts for the removal of benzene
title_sort fine platinum nanoparticles supported on a porous ceramic membrane as efficient catalysts for the removal of benzene
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5707434/
https://www.ncbi.nlm.nih.gov/pubmed/29185476
http://dx.doi.org/10.1038/s41598-017-16833-0
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