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Fractal analysis of collision cascades in pulsed-ion-beam-irradiated solids

The buildup of radiation damage in ion-irradiated crystals often depends on the spatial distribution of atomic displacements within collision cascades. Although collision cascades have previously been described as fractals, the correlation of their fractal parameters with experimental observations o...

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Autores principales: Wallace, J. B., Aji, L. B. Bayu, Shao, L., Kucheyev, S. O.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2017
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5730615/
https://www.ncbi.nlm.nih.gov/pubmed/29242621
http://dx.doi.org/10.1038/s41598-017-17781-5
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author Wallace, J. B.
Aji, L. B. Bayu
Shao, L.
Kucheyev, S. O.
author_facet Wallace, J. B.
Aji, L. B. Bayu
Shao, L.
Kucheyev, S. O.
author_sort Wallace, J. B.
collection PubMed
description The buildup of radiation damage in ion-irradiated crystals often depends on the spatial distribution of atomic displacements within collision cascades. Although collision cascades have previously been described as fractals, the correlation of their fractal parameters with experimental observations of radiation damage buildup remains elusive. Here, we use a pulsed-ion-beam method to study defect interaction dynamics in 3C-SiC irradiated at 100 °C with ions of different masses. These data, together with results of previous studies of SiC and Si, are analyzed with a model of radiation damage formation which accounts for the fractal nature of collision cascades. Our emphasis is on the extraction of the effective defect diffusion length from pulsed beam measurements. Results show that, for both Si and SiC, collision cascades are mass fractals with fractal dimensions in the range of ~1–2, depending on ion mass, energy, and the depth from the sample surface. Within our fractal model, the effective defect diffusion length is ~10 nm for SiC and ~20 nm for Si, and it decreases with increasing cascade density. These results demonstrate a general method by which the fractal nature of collision cascades can be used to explain experimental observations and predict material’s response to radiation.
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spelling pubmed-57306152017-12-18 Fractal analysis of collision cascades in pulsed-ion-beam-irradiated solids Wallace, J. B. Aji, L. B. Bayu Shao, L. Kucheyev, S. O. Sci Rep Article The buildup of radiation damage in ion-irradiated crystals often depends on the spatial distribution of atomic displacements within collision cascades. Although collision cascades have previously been described as fractals, the correlation of their fractal parameters with experimental observations of radiation damage buildup remains elusive. Here, we use a pulsed-ion-beam method to study defect interaction dynamics in 3C-SiC irradiated at 100 °C with ions of different masses. These data, together with results of previous studies of SiC and Si, are analyzed with a model of radiation damage formation which accounts for the fractal nature of collision cascades. Our emphasis is on the extraction of the effective defect diffusion length from pulsed beam measurements. Results show that, for both Si and SiC, collision cascades are mass fractals with fractal dimensions in the range of ~1–2, depending on ion mass, energy, and the depth from the sample surface. Within our fractal model, the effective defect diffusion length is ~10 nm for SiC and ~20 nm for Si, and it decreases with increasing cascade density. These results demonstrate a general method by which the fractal nature of collision cascades can be used to explain experimental observations and predict material’s response to radiation. Nature Publishing Group UK 2017-12-14 /pmc/articles/PMC5730615/ /pubmed/29242621 http://dx.doi.org/10.1038/s41598-017-17781-5 Text en © The Author(s) 2017 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Wallace, J. B.
Aji, L. B. Bayu
Shao, L.
Kucheyev, S. O.
Fractal analysis of collision cascades in pulsed-ion-beam-irradiated solids
title Fractal analysis of collision cascades in pulsed-ion-beam-irradiated solids
title_full Fractal analysis of collision cascades in pulsed-ion-beam-irradiated solids
title_fullStr Fractal analysis of collision cascades in pulsed-ion-beam-irradiated solids
title_full_unstemmed Fractal analysis of collision cascades in pulsed-ion-beam-irradiated solids
title_short Fractal analysis of collision cascades in pulsed-ion-beam-irradiated solids
title_sort fractal analysis of collision cascades in pulsed-ion-beam-irradiated solids
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5730615/
https://www.ncbi.nlm.nih.gov/pubmed/29242621
http://dx.doi.org/10.1038/s41598-017-17781-5
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