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Exciton–Exciton Annihilation Is Coherently Suppressed in H-Aggregates, but Not in J-Aggregates

[Image: see text] We theoretically demonstrate a strong dependence of the annihilation rate between (singlet) excitons on the sign of dipole–dipole couplings between molecules. For molecular H-aggregates, where this sign is positive, the phase relation of the delocalized two-exciton wave functions c...

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Detalles Bibliográficos
Autores principales: Tempelaar, Roel, Jansen, Thomas L. C., Knoester, Jasper
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2017
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5742477/
https://www.ncbi.nlm.nih.gov/pubmed/29190421
http://dx.doi.org/10.1021/acs.jpclett.7b02745