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Facile synthesis of TiO(2)/ZrO(2) nanofibers/nitrogen co-doped activated carbon to enhance the desalination and bacterial inactivation via capacitive deionization

Capacitive deionization, as a second generation electrosorption technique to obtain water, is one of the most promising water desalination technologies. Yet; in order to achieve high CDI performance, a well-designed structure of the electrode materials is needed, and is in high demand. Here, a novel...

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Autores principales: Yasin, Ahmed S., Mohamed, Ibrahim M. A., Mousa, Hamouda M., Park, Chan Hee, Kim, Cheol Sang
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5765043/
https://www.ncbi.nlm.nih.gov/pubmed/29323229
http://dx.doi.org/10.1038/s41598-017-19027-w
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author Yasin, Ahmed S.
Mohamed, Ibrahim M. A.
Mousa, Hamouda M.
Park, Chan Hee
Kim, Cheol Sang
author_facet Yasin, Ahmed S.
Mohamed, Ibrahim M. A.
Mousa, Hamouda M.
Park, Chan Hee
Kim, Cheol Sang
author_sort Yasin, Ahmed S.
collection PubMed
description Capacitive deionization, as a second generation electrosorption technique to obtain water, is one of the most promising water desalination technologies. Yet; in order to achieve high CDI performance, a well-designed structure of the electrode materials is needed, and is in high demand. Here, a novel composite nitrogen-TiO(2)/ZrO(2) nanofibers incorporated activated carbon (NACTZ) is synthesized for the first time with enhanced desalination efficiency as well as disinfection performance towards brackish water. Nitrogen and TiO(2)/ZrO(2) nanofibers are used as the support of activated carbon to improve its low capacitance and hydrophobicity, which had dramatically limited its adequacy during the CDI process. Importantly, the as-fabricated NACTZ nanocomposite demonstrates enhanced electrochemical performance with significant specific capacitance of 691.78 F g(−1), low internal resistance and good cycling stability. In addition, it offers a high capacitive deionization performance of NACTZ yield with electrosorptive capacity of 3.98 mg g(−1), and, good antibacterial effects as well. This work will provide an effective solution for developing highly performance and low-cost design for CDI electrode materials.
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spelling pubmed-57650432018-01-17 Facile synthesis of TiO(2)/ZrO(2) nanofibers/nitrogen co-doped activated carbon to enhance the desalination and bacterial inactivation via capacitive deionization Yasin, Ahmed S. Mohamed, Ibrahim M. A. Mousa, Hamouda M. Park, Chan Hee Kim, Cheol Sang Sci Rep Article Capacitive deionization, as a second generation electrosorption technique to obtain water, is one of the most promising water desalination technologies. Yet; in order to achieve high CDI performance, a well-designed structure of the electrode materials is needed, and is in high demand. Here, a novel composite nitrogen-TiO(2)/ZrO(2) nanofibers incorporated activated carbon (NACTZ) is synthesized for the first time with enhanced desalination efficiency as well as disinfection performance towards brackish water. Nitrogen and TiO(2)/ZrO(2) nanofibers are used as the support of activated carbon to improve its low capacitance and hydrophobicity, which had dramatically limited its adequacy during the CDI process. Importantly, the as-fabricated NACTZ nanocomposite demonstrates enhanced electrochemical performance with significant specific capacitance of 691.78 F g(−1), low internal resistance and good cycling stability. In addition, it offers a high capacitive deionization performance of NACTZ yield with electrosorptive capacity of 3.98 mg g(−1), and, good antibacterial effects as well. This work will provide an effective solution for developing highly performance and low-cost design for CDI electrode materials. Nature Publishing Group UK 2018-01-11 /pmc/articles/PMC5765043/ /pubmed/29323229 http://dx.doi.org/10.1038/s41598-017-19027-w Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Yasin, Ahmed S.
Mohamed, Ibrahim M. A.
Mousa, Hamouda M.
Park, Chan Hee
Kim, Cheol Sang
Facile synthesis of TiO(2)/ZrO(2) nanofibers/nitrogen co-doped activated carbon to enhance the desalination and bacterial inactivation via capacitive deionization
title Facile synthesis of TiO(2)/ZrO(2) nanofibers/nitrogen co-doped activated carbon to enhance the desalination and bacterial inactivation via capacitive deionization
title_full Facile synthesis of TiO(2)/ZrO(2) nanofibers/nitrogen co-doped activated carbon to enhance the desalination and bacterial inactivation via capacitive deionization
title_fullStr Facile synthesis of TiO(2)/ZrO(2) nanofibers/nitrogen co-doped activated carbon to enhance the desalination and bacterial inactivation via capacitive deionization
title_full_unstemmed Facile synthesis of TiO(2)/ZrO(2) nanofibers/nitrogen co-doped activated carbon to enhance the desalination and bacterial inactivation via capacitive deionization
title_short Facile synthesis of TiO(2)/ZrO(2) nanofibers/nitrogen co-doped activated carbon to enhance the desalination and bacterial inactivation via capacitive deionization
title_sort facile synthesis of tio(2)/zro(2) nanofibers/nitrogen co-doped activated carbon to enhance the desalination and bacterial inactivation via capacitive deionization
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5765043/
https://www.ncbi.nlm.nih.gov/pubmed/29323229
http://dx.doi.org/10.1038/s41598-017-19027-w
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