Cargando…
Novel insights on new particle formation derived from a pan-european observing system
The formation of new atmospheric particles involves an initial step forming stable clusters less than a nanometre in size (<~1 nm), followed by growth into quasi-stable aerosol particles a few nanometres (~1–10 nm) and larger (>~10 nm). Although at times, the same species can be responsible fo...
Autores principales: | , , , , , , , , , , , , , , , , , , , , , , , , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2018
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5784154/ https://www.ncbi.nlm.nih.gov/pubmed/29367716 http://dx.doi.org/10.1038/s41598-017-17343-9 |
_version_ | 1783295392202358784 |
---|---|
author | Dall’Osto, M. Beddows, D. C. S. Asmi, A. Poulain, L. Hao, L. Freney, E. Allan, J. D. Canagaratna, M. Crippa, M. Bianchi, F. de Leeuw, G. Eriksson, A. Swietlicki, E. Hansson, H. C. Henzing, J. S. Granier, C. Zemankova, K. Laj, P. Onasch, T. Prevot, A. Putaud, J. P. Sellegri, K. Vidal, M. Virtanen, A. Simo, R. Worsnop, D. O’Dowd, C. Kulmala, M. Harrison, Roy M. |
author_facet | Dall’Osto, M. Beddows, D. C. S. Asmi, A. Poulain, L. Hao, L. Freney, E. Allan, J. D. Canagaratna, M. Crippa, M. Bianchi, F. de Leeuw, G. Eriksson, A. Swietlicki, E. Hansson, H. C. Henzing, J. S. Granier, C. Zemankova, K. Laj, P. Onasch, T. Prevot, A. Putaud, J. P. Sellegri, K. Vidal, M. Virtanen, A. Simo, R. Worsnop, D. O’Dowd, C. Kulmala, M. Harrison, Roy M. |
author_sort | Dall’Osto, M. |
collection | PubMed |
description | The formation of new atmospheric particles involves an initial step forming stable clusters less than a nanometre in size (<~1 nm), followed by growth into quasi-stable aerosol particles a few nanometres (~1–10 nm) and larger (>~10 nm). Although at times, the same species can be responsible for both processes, it is thought that more generally each step comprises differing chemical contributors. Here, we present a novel analysis of measurements from a unique multi-station ground-based observing system which reveals new insights into continental-scale patterns associated with new particle formation. Statistical cluster analysis of this unique 2-year multi-station dataset comprising size distribution and chemical composition reveals that across Europe, there are different major seasonal trends depending on geographical location, concomitant with diversity in nucleating species while it seems that the growth phase is dominated by organic aerosol formation. The diversity and seasonality of these events requires an advanced observing system to elucidate the key processes and species driving particle formation, along with detecting continental scale changes in aerosol formation into the future. |
format | Online Article Text |
id | pubmed-5784154 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2018 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-57841542018-02-07 Novel insights on new particle formation derived from a pan-european observing system Dall’Osto, M. Beddows, D. C. S. Asmi, A. Poulain, L. Hao, L. Freney, E. Allan, J. D. Canagaratna, M. Crippa, M. Bianchi, F. de Leeuw, G. Eriksson, A. Swietlicki, E. Hansson, H. C. Henzing, J. S. Granier, C. Zemankova, K. Laj, P. Onasch, T. Prevot, A. Putaud, J. P. Sellegri, K. Vidal, M. Virtanen, A. Simo, R. Worsnop, D. O’Dowd, C. Kulmala, M. Harrison, Roy M. Sci Rep Article The formation of new atmospheric particles involves an initial step forming stable clusters less than a nanometre in size (<~1 nm), followed by growth into quasi-stable aerosol particles a few nanometres (~1–10 nm) and larger (>~10 nm). Although at times, the same species can be responsible for both processes, it is thought that more generally each step comprises differing chemical contributors. Here, we present a novel analysis of measurements from a unique multi-station ground-based observing system which reveals new insights into continental-scale patterns associated with new particle formation. Statistical cluster analysis of this unique 2-year multi-station dataset comprising size distribution and chemical composition reveals that across Europe, there are different major seasonal trends depending on geographical location, concomitant with diversity in nucleating species while it seems that the growth phase is dominated by organic aerosol formation. The diversity and seasonality of these events requires an advanced observing system to elucidate the key processes and species driving particle formation, along with detecting continental scale changes in aerosol formation into the future. Nature Publishing Group UK 2018-01-24 /pmc/articles/PMC5784154/ /pubmed/29367716 http://dx.doi.org/10.1038/s41598-017-17343-9 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Dall’Osto, M. Beddows, D. C. S. Asmi, A. Poulain, L. Hao, L. Freney, E. Allan, J. D. Canagaratna, M. Crippa, M. Bianchi, F. de Leeuw, G. Eriksson, A. Swietlicki, E. Hansson, H. C. Henzing, J. S. Granier, C. Zemankova, K. Laj, P. Onasch, T. Prevot, A. Putaud, J. P. Sellegri, K. Vidal, M. Virtanen, A. Simo, R. Worsnop, D. O’Dowd, C. Kulmala, M. Harrison, Roy M. Novel insights on new particle formation derived from a pan-european observing system |
title | Novel insights on new particle formation derived from a pan-european observing system |
title_full | Novel insights on new particle formation derived from a pan-european observing system |
title_fullStr | Novel insights on new particle formation derived from a pan-european observing system |
title_full_unstemmed | Novel insights on new particle formation derived from a pan-european observing system |
title_short | Novel insights on new particle formation derived from a pan-european observing system |
title_sort | novel insights on new particle formation derived from a pan-european observing system |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5784154/ https://www.ncbi.nlm.nih.gov/pubmed/29367716 http://dx.doi.org/10.1038/s41598-017-17343-9 |
work_keys_str_mv | AT dallostom novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT beddowsdcs novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT asmia novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT poulainl novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT haol novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT freneye novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT allanjd novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT canagaratnam novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT crippam novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT bianchif novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT deleeuwg novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT erikssona novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT swietlickie novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT hanssonhc novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT henzingjs novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT granierc novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT zemankovak novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT lajp novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT onascht novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT prevota novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT putaudjp novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT sellegrik novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT vidalm novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT virtanena novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT simor novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT worsnopd novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT odowdc novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT kulmalam novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem AT harrisonroym novelinsightsonnewparticleformationderivedfromapaneuropeanobservingsystem |