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Novel insights on new particle formation derived from a pan-european observing system

The formation of new atmospheric particles involves an initial step forming stable clusters less than a nanometre in size (<~1 nm), followed by growth into quasi-stable aerosol particles a few nanometres (~1–10 nm) and larger (>~10 nm). Although at times, the same species can be responsible fo...

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Autores principales: Dall’Osto, M., Beddows, D. C. S., Asmi, A., Poulain, L., Hao, L., Freney, E., Allan, J. D., Canagaratna, M., Crippa, M., Bianchi, F., de Leeuw, G., Eriksson, A., Swietlicki, E., Hansson, H. C., Henzing, J. S., Granier, C., Zemankova, K., Laj, P., Onasch, T., Prevot, A., Putaud, J. P., Sellegri, K., Vidal, M., Virtanen, A., Simo, R., Worsnop, D., O’Dowd, C., Kulmala, M., Harrison, Roy M.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5784154/
https://www.ncbi.nlm.nih.gov/pubmed/29367716
http://dx.doi.org/10.1038/s41598-017-17343-9
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author Dall’Osto, M.
Beddows, D. C. S.
Asmi, A.
Poulain, L.
Hao, L.
Freney, E.
Allan, J. D.
Canagaratna, M.
Crippa, M.
Bianchi, F.
de Leeuw, G.
Eriksson, A.
Swietlicki, E.
Hansson, H. C.
Henzing, J. S.
Granier, C.
Zemankova, K.
Laj, P.
Onasch, T.
Prevot, A.
Putaud, J. P.
Sellegri, K.
Vidal, M.
Virtanen, A.
Simo, R.
Worsnop, D.
O’Dowd, C.
Kulmala, M.
Harrison, Roy M.
author_facet Dall’Osto, M.
Beddows, D. C. S.
Asmi, A.
Poulain, L.
Hao, L.
Freney, E.
Allan, J. D.
Canagaratna, M.
Crippa, M.
Bianchi, F.
de Leeuw, G.
Eriksson, A.
Swietlicki, E.
Hansson, H. C.
Henzing, J. S.
Granier, C.
Zemankova, K.
Laj, P.
Onasch, T.
Prevot, A.
Putaud, J. P.
Sellegri, K.
Vidal, M.
Virtanen, A.
Simo, R.
Worsnop, D.
O’Dowd, C.
Kulmala, M.
Harrison, Roy M.
author_sort Dall’Osto, M.
collection PubMed
description The formation of new atmospheric particles involves an initial step forming stable clusters less than a nanometre in size (<~1 nm), followed by growth into quasi-stable aerosol particles a few nanometres (~1–10 nm) and larger (>~10 nm). Although at times, the same species can be responsible for both processes, it is thought that more generally each step comprises differing chemical contributors. Here, we present a novel analysis of measurements from a unique multi-station ground-based observing system which reveals new insights into continental-scale patterns associated with new particle formation. Statistical cluster analysis of this unique 2-year multi-station dataset comprising size distribution and chemical composition reveals that across Europe, there are different major seasonal trends depending on geographical location, concomitant with diversity in nucleating species while it seems that the growth phase is dominated by organic aerosol formation. The diversity and seasonality of these events requires an advanced observing system to elucidate the key processes and species driving particle formation, along with detecting continental scale changes in aerosol formation into the future.
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spelling pubmed-57841542018-02-07 Novel insights on new particle formation derived from a pan-european observing system Dall’Osto, M. Beddows, D. C. S. Asmi, A. Poulain, L. Hao, L. Freney, E. Allan, J. D. Canagaratna, M. Crippa, M. Bianchi, F. de Leeuw, G. Eriksson, A. Swietlicki, E. Hansson, H. C. Henzing, J. S. Granier, C. Zemankova, K. Laj, P. Onasch, T. Prevot, A. Putaud, J. P. Sellegri, K. Vidal, M. Virtanen, A. Simo, R. Worsnop, D. O’Dowd, C. Kulmala, M. Harrison, Roy M. Sci Rep Article The formation of new atmospheric particles involves an initial step forming stable clusters less than a nanometre in size (<~1 nm), followed by growth into quasi-stable aerosol particles a few nanometres (~1–10 nm) and larger (>~10 nm). Although at times, the same species can be responsible for both processes, it is thought that more generally each step comprises differing chemical contributors. Here, we present a novel analysis of measurements from a unique multi-station ground-based observing system which reveals new insights into continental-scale patterns associated with new particle formation. Statistical cluster analysis of this unique 2-year multi-station dataset comprising size distribution and chemical composition reveals that across Europe, there are different major seasonal trends depending on geographical location, concomitant with diversity in nucleating species while it seems that the growth phase is dominated by organic aerosol formation. The diversity and seasonality of these events requires an advanced observing system to elucidate the key processes and species driving particle formation, along with detecting continental scale changes in aerosol formation into the future. Nature Publishing Group UK 2018-01-24 /pmc/articles/PMC5784154/ /pubmed/29367716 http://dx.doi.org/10.1038/s41598-017-17343-9 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Dall’Osto, M.
Beddows, D. C. S.
Asmi, A.
Poulain, L.
Hao, L.
Freney, E.
Allan, J. D.
Canagaratna, M.
Crippa, M.
Bianchi, F.
de Leeuw, G.
Eriksson, A.
Swietlicki, E.
Hansson, H. C.
Henzing, J. S.
Granier, C.
Zemankova, K.
Laj, P.
Onasch, T.
Prevot, A.
Putaud, J. P.
Sellegri, K.
Vidal, M.
Virtanen, A.
Simo, R.
Worsnop, D.
O’Dowd, C.
Kulmala, M.
Harrison, Roy M.
Novel insights on new particle formation derived from a pan-european observing system
title Novel insights on new particle formation derived from a pan-european observing system
title_full Novel insights on new particle formation derived from a pan-european observing system
title_fullStr Novel insights on new particle formation derived from a pan-european observing system
title_full_unstemmed Novel insights on new particle formation derived from a pan-european observing system
title_short Novel insights on new particle formation derived from a pan-european observing system
title_sort novel insights on new particle formation derived from a pan-european observing system
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5784154/
https://www.ncbi.nlm.nih.gov/pubmed/29367716
http://dx.doi.org/10.1038/s41598-017-17343-9
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