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Configurable topological textures in strain graded ferroelectric nanoplates

Topological defects in matter behave collectively to form highly non-trivial structures called topological textures that are characterised by conserved quantities such as the winding number. Here we show that an epitaxial ferroelectric square nanoplate of bismuth ferrite subjected to a large strain...

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Autores principales: Kim, Kwang-Eun, Jeong, Seuri, Chu, Kanghyun, Lee, Jin Hong, Kim, Gi-Yeop, Xue, Fei, Koo, Tae Yeong, Chen, Long-Qing, Choi, Si-Young, Ramesh, Ramamoorthy, Yang, Chan-Ho
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5785989/
https://www.ncbi.nlm.nih.gov/pubmed/29374260
http://dx.doi.org/10.1038/s41467-017-02813-5
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author Kim, Kwang-Eun
Jeong, Seuri
Chu, Kanghyun
Lee, Jin Hong
Kim, Gi-Yeop
Xue, Fei
Koo, Tae Yeong
Chen, Long-Qing
Choi, Si-Young
Ramesh, Ramamoorthy
Yang, Chan-Ho
author_facet Kim, Kwang-Eun
Jeong, Seuri
Chu, Kanghyun
Lee, Jin Hong
Kim, Gi-Yeop
Xue, Fei
Koo, Tae Yeong
Chen, Long-Qing
Choi, Si-Young
Ramesh, Ramamoorthy
Yang, Chan-Ho
author_sort Kim, Kwang-Eun
collection PubMed
description Topological defects in matter behave collectively to form highly non-trivial structures called topological textures that are characterised by conserved quantities such as the winding number. Here we show that an epitaxial ferroelectric square nanoplate of bismuth ferrite subjected to a large strain gradient (as much as 10(5) m(−1)) associated with misfit strain relaxation enables five discrete levels for the ferroelectric topological invariant of the entire system because of its peculiar radial quadrant domain texture and its inherent domain wall chirality. The total winding number of the topological texture can be configured from − 1 to 3 by selective non-local electric switching of the quadrant domains. By using angle-resolved piezoresponse force microscopy in conjunction with local winding number analysis, we directly identify the existence of vortices and anti-vortices, observe pair creation and annihilation and manipulate the net number of vortices. Our findings offer a useful concept for multi-level topological defect memory.
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spelling pubmed-57859892018-01-29 Configurable topological textures in strain graded ferroelectric nanoplates Kim, Kwang-Eun Jeong, Seuri Chu, Kanghyun Lee, Jin Hong Kim, Gi-Yeop Xue, Fei Koo, Tae Yeong Chen, Long-Qing Choi, Si-Young Ramesh, Ramamoorthy Yang, Chan-Ho Nat Commun Article Topological defects in matter behave collectively to form highly non-trivial structures called topological textures that are characterised by conserved quantities such as the winding number. Here we show that an epitaxial ferroelectric square nanoplate of bismuth ferrite subjected to a large strain gradient (as much as 10(5) m(−1)) associated with misfit strain relaxation enables five discrete levels for the ferroelectric topological invariant of the entire system because of its peculiar radial quadrant domain texture and its inherent domain wall chirality. The total winding number of the topological texture can be configured from − 1 to 3 by selective non-local electric switching of the quadrant domains. By using angle-resolved piezoresponse force microscopy in conjunction with local winding number analysis, we directly identify the existence of vortices and anti-vortices, observe pair creation and annihilation and manipulate the net number of vortices. Our findings offer a useful concept for multi-level topological defect memory. Nature Publishing Group UK 2018-01-26 /pmc/articles/PMC5785989/ /pubmed/29374260 http://dx.doi.org/10.1038/s41467-017-02813-5 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Kim, Kwang-Eun
Jeong, Seuri
Chu, Kanghyun
Lee, Jin Hong
Kim, Gi-Yeop
Xue, Fei
Koo, Tae Yeong
Chen, Long-Qing
Choi, Si-Young
Ramesh, Ramamoorthy
Yang, Chan-Ho
Configurable topological textures in strain graded ferroelectric nanoplates
title Configurable topological textures in strain graded ferroelectric nanoplates
title_full Configurable topological textures in strain graded ferroelectric nanoplates
title_fullStr Configurable topological textures in strain graded ferroelectric nanoplates
title_full_unstemmed Configurable topological textures in strain graded ferroelectric nanoplates
title_short Configurable topological textures in strain graded ferroelectric nanoplates
title_sort configurable topological textures in strain graded ferroelectric nanoplates
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5785989/
https://www.ncbi.nlm.nih.gov/pubmed/29374260
http://dx.doi.org/10.1038/s41467-017-02813-5
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