Cargando…

Ergodicity breaking transition in a glassy soft sphere system at small but non-zero temperatures

While the glass transition at non-zero temperature seems to be hard to access for experimental, theoretical, or simulation studies, jamming at zero temperature has been studied in great detail. Motivated by the exploration of the energy landscape that has been successfully used to investigate atherm...

Descripción completa

Detalles Bibliográficos
Autores principales: Maiti, Moumita, Schmiedeberg, Michael
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5789873/
https://www.ncbi.nlm.nih.gov/pubmed/29382860
http://dx.doi.org/10.1038/s41598-018-20152-3
_version_ 1783296367635988480
author Maiti, Moumita
Schmiedeberg, Michael
author_facet Maiti, Moumita
Schmiedeberg, Michael
author_sort Maiti, Moumita
collection PubMed
description While the glass transition at non-zero temperature seems to be hard to access for experimental, theoretical, or simulation studies, jamming at zero temperature has been studied in great detail. Motivated by the exploration of the energy landscape that has been successfully used to investigate athermal jamming, we introduce a new method that includes the possibility of the thermally excited crossing of energy barriers. We then determine whether the ground state configurations of a soft sphere system are accessible or not and as a consequence whether the system is ergodic or effectively non-ergodic. Interestingly, we find an transition where the system becomes effectively non-ergodic if the density is increased. The transition density in the limit of small but non-zero temperatures is independent of temperature and below the transition density of athermal jamming. This confirms recent computer simulation studies where athermal jamming occurs deep inside the glass phase. In addition, we show that the ergodicity breaking transition is in the universality class of directed percolation. Therefore, our approach not only makes the transition from an ergodic to an effectively non-ergodic systems easily accessible and helps to reveal its universality class but also shows that it is fundamentally different from athermal jamming.
format Online
Article
Text
id pubmed-5789873
institution National Center for Biotechnology Information
language English
publishDate 2018
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-57898732018-02-15 Ergodicity breaking transition in a glassy soft sphere system at small but non-zero temperatures Maiti, Moumita Schmiedeberg, Michael Sci Rep Article While the glass transition at non-zero temperature seems to be hard to access for experimental, theoretical, or simulation studies, jamming at zero temperature has been studied in great detail. Motivated by the exploration of the energy landscape that has been successfully used to investigate athermal jamming, we introduce a new method that includes the possibility of the thermally excited crossing of energy barriers. We then determine whether the ground state configurations of a soft sphere system are accessible or not and as a consequence whether the system is ergodic or effectively non-ergodic. Interestingly, we find an transition where the system becomes effectively non-ergodic if the density is increased. The transition density in the limit of small but non-zero temperatures is independent of temperature and below the transition density of athermal jamming. This confirms recent computer simulation studies where athermal jamming occurs deep inside the glass phase. In addition, we show that the ergodicity breaking transition is in the universality class of directed percolation. Therefore, our approach not only makes the transition from an ergodic to an effectively non-ergodic systems easily accessible and helps to reveal its universality class but also shows that it is fundamentally different from athermal jamming. Nature Publishing Group UK 2018-01-30 /pmc/articles/PMC5789873/ /pubmed/29382860 http://dx.doi.org/10.1038/s41598-018-20152-3 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Maiti, Moumita
Schmiedeberg, Michael
Ergodicity breaking transition in a glassy soft sphere system at small but non-zero temperatures
title Ergodicity breaking transition in a glassy soft sphere system at small but non-zero temperatures
title_full Ergodicity breaking transition in a glassy soft sphere system at small but non-zero temperatures
title_fullStr Ergodicity breaking transition in a glassy soft sphere system at small but non-zero temperatures
title_full_unstemmed Ergodicity breaking transition in a glassy soft sphere system at small but non-zero temperatures
title_short Ergodicity breaking transition in a glassy soft sphere system at small but non-zero temperatures
title_sort ergodicity breaking transition in a glassy soft sphere system at small but non-zero temperatures
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5789873/
https://www.ncbi.nlm.nih.gov/pubmed/29382860
http://dx.doi.org/10.1038/s41598-018-20152-3
work_keys_str_mv AT maitimoumita ergodicitybreakingtransitioninaglassysoftspheresystematsmallbutnonzerotemperatures
AT schmiedebergmichael ergodicitybreakingtransitioninaglassysoftspheresystematsmallbutnonzerotemperatures