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Attosecond recorder of the polarization state of light

High harmonic generation in multi-color laser fields opens the opportunity of generating isolated attosecond pulses with high ellipticity. Such pulses hold the potential for time-resolving chiral electronic, magnetization, and spin dynamics at their natural timescale. However, this potential cannot...

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Autores principales: Jiménez-Galán, Álvaro, Dixit, Gopal, Patchkovskii, Serguei, Smirnova, Olga, Morales, Felipe, Ivanov, Misha
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5829146/
https://www.ncbi.nlm.nih.gov/pubmed/29487288
http://dx.doi.org/10.1038/s41467-018-03167-2
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author Jiménez-Galán, Álvaro
Dixit, Gopal
Patchkovskii, Serguei
Smirnova, Olga
Morales, Felipe
Ivanov, Misha
author_facet Jiménez-Galán, Álvaro
Dixit, Gopal
Patchkovskii, Serguei
Smirnova, Olga
Morales, Felipe
Ivanov, Misha
author_sort Jiménez-Galán, Álvaro
collection PubMed
description High harmonic generation in multi-color laser fields opens the opportunity of generating isolated attosecond pulses with high ellipticity. Such pulses hold the potential for time-resolving chiral electronic, magnetization, and spin dynamics at their natural timescale. However, this potential cannot be realized without characterizing the exact polarization state of light on the attosecond timescale. Here we propose and numerically demonstrate a complete solution of this problem. Our solution exploits the extrinsic two-dimensional chirality induced in an atom interacting with the chiral attosecond pulse and a linearly polarized infrared probe. The resulting asymmetry in the photoelectron spectra allows to reconstruct the complete polarization state of the attosecond pulse, including its possible time dependence. The challenging problem of distinguishing circularly polarized, partially polarized, or unpolarized pulses in the extreme ultraviolet range is also resolved. We expect this approach to become the core ingredient for attosecond measurements of chiral-sensitive processes in gas and condensed phase.
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spelling pubmed-58291462018-03-02 Attosecond recorder of the polarization state of light Jiménez-Galán, Álvaro Dixit, Gopal Patchkovskii, Serguei Smirnova, Olga Morales, Felipe Ivanov, Misha Nat Commun Article High harmonic generation in multi-color laser fields opens the opportunity of generating isolated attosecond pulses with high ellipticity. Such pulses hold the potential for time-resolving chiral electronic, magnetization, and spin dynamics at their natural timescale. However, this potential cannot be realized without characterizing the exact polarization state of light on the attosecond timescale. Here we propose and numerically demonstrate a complete solution of this problem. Our solution exploits the extrinsic two-dimensional chirality induced in an atom interacting with the chiral attosecond pulse and a linearly polarized infrared probe. The resulting asymmetry in the photoelectron spectra allows to reconstruct the complete polarization state of the attosecond pulse, including its possible time dependence. The challenging problem of distinguishing circularly polarized, partially polarized, or unpolarized pulses in the extreme ultraviolet range is also resolved. We expect this approach to become the core ingredient for attosecond measurements of chiral-sensitive processes in gas and condensed phase. Nature Publishing Group UK 2018-02-27 /pmc/articles/PMC5829146/ /pubmed/29487288 http://dx.doi.org/10.1038/s41467-018-03167-2 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Jiménez-Galán, Álvaro
Dixit, Gopal
Patchkovskii, Serguei
Smirnova, Olga
Morales, Felipe
Ivanov, Misha
Attosecond recorder of the polarization state of light
title Attosecond recorder of the polarization state of light
title_full Attosecond recorder of the polarization state of light
title_fullStr Attosecond recorder of the polarization state of light
title_full_unstemmed Attosecond recorder of the polarization state of light
title_short Attosecond recorder of the polarization state of light
title_sort attosecond recorder of the polarization state of light
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5829146/
https://www.ncbi.nlm.nih.gov/pubmed/29487288
http://dx.doi.org/10.1038/s41467-018-03167-2
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