Cargando…
Attosecond recorder of the polarization state of light
High harmonic generation in multi-color laser fields opens the opportunity of generating isolated attosecond pulses with high ellipticity. Such pulses hold the potential for time-resolving chiral electronic, magnetization, and spin dynamics at their natural timescale. However, this potential cannot...
Autores principales: | , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2018
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5829146/ https://www.ncbi.nlm.nih.gov/pubmed/29487288 http://dx.doi.org/10.1038/s41467-018-03167-2 |
_version_ | 1783302746828439552 |
---|---|
author | Jiménez-Galán, Álvaro Dixit, Gopal Patchkovskii, Serguei Smirnova, Olga Morales, Felipe Ivanov, Misha |
author_facet | Jiménez-Galán, Álvaro Dixit, Gopal Patchkovskii, Serguei Smirnova, Olga Morales, Felipe Ivanov, Misha |
author_sort | Jiménez-Galán, Álvaro |
collection | PubMed |
description | High harmonic generation in multi-color laser fields opens the opportunity of generating isolated attosecond pulses with high ellipticity. Such pulses hold the potential for time-resolving chiral electronic, magnetization, and spin dynamics at their natural timescale. However, this potential cannot be realized without characterizing the exact polarization state of light on the attosecond timescale. Here we propose and numerically demonstrate a complete solution of this problem. Our solution exploits the extrinsic two-dimensional chirality induced in an atom interacting with the chiral attosecond pulse and a linearly polarized infrared probe. The resulting asymmetry in the photoelectron spectra allows to reconstruct the complete polarization state of the attosecond pulse, including its possible time dependence. The challenging problem of distinguishing circularly polarized, partially polarized, or unpolarized pulses in the extreme ultraviolet range is also resolved. We expect this approach to become the core ingredient for attosecond measurements of chiral-sensitive processes in gas and condensed phase. |
format | Online Article Text |
id | pubmed-5829146 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2018 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-58291462018-03-02 Attosecond recorder of the polarization state of light Jiménez-Galán, Álvaro Dixit, Gopal Patchkovskii, Serguei Smirnova, Olga Morales, Felipe Ivanov, Misha Nat Commun Article High harmonic generation in multi-color laser fields opens the opportunity of generating isolated attosecond pulses with high ellipticity. Such pulses hold the potential for time-resolving chiral electronic, magnetization, and spin dynamics at their natural timescale. However, this potential cannot be realized without characterizing the exact polarization state of light on the attosecond timescale. Here we propose and numerically demonstrate a complete solution of this problem. Our solution exploits the extrinsic two-dimensional chirality induced in an atom interacting with the chiral attosecond pulse and a linearly polarized infrared probe. The resulting asymmetry in the photoelectron spectra allows to reconstruct the complete polarization state of the attosecond pulse, including its possible time dependence. The challenging problem of distinguishing circularly polarized, partially polarized, or unpolarized pulses in the extreme ultraviolet range is also resolved. We expect this approach to become the core ingredient for attosecond measurements of chiral-sensitive processes in gas and condensed phase. Nature Publishing Group UK 2018-02-27 /pmc/articles/PMC5829146/ /pubmed/29487288 http://dx.doi.org/10.1038/s41467-018-03167-2 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Jiménez-Galán, Álvaro Dixit, Gopal Patchkovskii, Serguei Smirnova, Olga Morales, Felipe Ivanov, Misha Attosecond recorder of the polarization state of light |
title | Attosecond recorder of the polarization state of light |
title_full | Attosecond recorder of the polarization state of light |
title_fullStr | Attosecond recorder of the polarization state of light |
title_full_unstemmed | Attosecond recorder of the polarization state of light |
title_short | Attosecond recorder of the polarization state of light |
title_sort | attosecond recorder of the polarization state of light |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5829146/ https://www.ncbi.nlm.nih.gov/pubmed/29487288 http://dx.doi.org/10.1038/s41467-018-03167-2 |
work_keys_str_mv | AT jimenezgalanalvaro attosecondrecorderofthepolarizationstateoflight AT dixitgopal attosecondrecorderofthepolarizationstateoflight AT patchkovskiiserguei attosecondrecorderofthepolarizationstateoflight AT smirnovaolga attosecondrecorderofthepolarizationstateoflight AT moralesfelipe attosecondrecorderofthepolarizationstateoflight AT ivanovmisha attosecondrecorderofthepolarizationstateoflight |