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Valley-selective directional emission from a transition-metal dichalcogenide monolayer mediated by a plasmonic nanoantenna

Background: Two-dimensional (2D) transition-metal dichalcogenides (TMDCs) with intrinsically crystal inversion-symmetry breaking have shown many advanced optical properties. In particular, the valley polarization in 2D TMDCs that can be addressed optically has inspired new physical phenomena and gre...

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Autores principales: Chen, Haitao, Liu, Mingkai, Xu, Lei, Neshev, Dragomir N
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Beilstein-Institut 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5852623/
https://www.ncbi.nlm.nih.gov/pubmed/29600139
http://dx.doi.org/10.3762/bjnano.9.71
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author Chen, Haitao
Liu, Mingkai
Xu, Lei
Neshev, Dragomir N
author_facet Chen, Haitao
Liu, Mingkai
Xu, Lei
Neshev, Dragomir N
author_sort Chen, Haitao
collection PubMed
description Background: Two-dimensional (2D) transition-metal dichalcogenides (TMDCs) with intrinsically crystal inversion-symmetry breaking have shown many advanced optical properties. In particular, the valley polarization in 2D TMDCs that can be addressed optically has inspired new physical phenomena and great potential applications in valleytronics. Results: Here, we propose a TMDC–nanoantenna system that could effectively enhance and direct emission from the two valleys in TMDCs into diametrically opposite directions. By mimicking the emission from each valley of the monolayer of WSe(2) as a chiral point-dipole emitter, we demonstrate numerically that the emission from different valleys is directed into opposite directions when coupling to a double-bar plasmonic nanoantenna. The directionality derives from the interference between the dipole and quadrupole modes excited in the two bars, respectively. Thus, we could tune the emission direction from the proposed TMDC–nanoantenna system by tuning the pumping without changing the antenna structure. Furthermore, we discuss the general principles and the opportunities to improve the average performance of the nanoantenna structure. Conclusion: The scheme we propose here can potentially serve as an important component for valley-based applications, such as non-volatile information storage and processing.
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spelling pubmed-58526232018-03-29 Valley-selective directional emission from a transition-metal dichalcogenide monolayer mediated by a plasmonic nanoantenna Chen, Haitao Liu, Mingkai Xu, Lei Neshev, Dragomir N Beilstein J Nanotechnol Full Research Paper Background: Two-dimensional (2D) transition-metal dichalcogenides (TMDCs) with intrinsically crystal inversion-symmetry breaking have shown many advanced optical properties. In particular, the valley polarization in 2D TMDCs that can be addressed optically has inspired new physical phenomena and great potential applications in valleytronics. Results: Here, we propose a TMDC–nanoantenna system that could effectively enhance and direct emission from the two valleys in TMDCs into diametrically opposite directions. By mimicking the emission from each valley of the monolayer of WSe(2) as a chiral point-dipole emitter, we demonstrate numerically that the emission from different valleys is directed into opposite directions when coupling to a double-bar plasmonic nanoantenna. The directionality derives from the interference between the dipole and quadrupole modes excited in the two bars, respectively. Thus, we could tune the emission direction from the proposed TMDC–nanoantenna system by tuning the pumping without changing the antenna structure. Furthermore, we discuss the general principles and the opportunities to improve the average performance of the nanoantenna structure. Conclusion: The scheme we propose here can potentially serve as an important component for valley-based applications, such as non-volatile information storage and processing. Beilstein-Institut 2018-03-02 /pmc/articles/PMC5852623/ /pubmed/29600139 http://dx.doi.org/10.3762/bjnano.9.71 Text en Copyright © 2018, Chen et al. https://creativecommons.org/licenses/by/4.0https://www.beilstein-journals.org/bjnano/termsThis is an Open Access article under the terms of the Creative Commons Attribution License (https://creativecommons.org/licenses/by/4.0), which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited. The license is subject to the Beilstein Journal of Nanotechnology terms and conditions: (https://www.beilstein-journals.org/bjnano/terms)
spellingShingle Full Research Paper
Chen, Haitao
Liu, Mingkai
Xu, Lei
Neshev, Dragomir N
Valley-selective directional emission from a transition-metal dichalcogenide monolayer mediated by a plasmonic nanoantenna
title Valley-selective directional emission from a transition-metal dichalcogenide monolayer mediated by a plasmonic nanoantenna
title_full Valley-selective directional emission from a transition-metal dichalcogenide monolayer mediated by a plasmonic nanoantenna
title_fullStr Valley-selective directional emission from a transition-metal dichalcogenide monolayer mediated by a plasmonic nanoantenna
title_full_unstemmed Valley-selective directional emission from a transition-metal dichalcogenide monolayer mediated by a plasmonic nanoantenna
title_short Valley-selective directional emission from a transition-metal dichalcogenide monolayer mediated by a plasmonic nanoantenna
title_sort valley-selective directional emission from a transition-metal dichalcogenide monolayer mediated by a plasmonic nanoantenna
topic Full Research Paper
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5852623/
https://www.ncbi.nlm.nih.gov/pubmed/29600139
http://dx.doi.org/10.3762/bjnano.9.71
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