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O(2) evolution and recovery of the water-oxidizing enzyme
In photosystem II, light-induced water oxidation occurs at the Mn(4)CaO(5) cluster. Here we demonstrate proton releases, dioxygen formation, and substrate water incorporation in response to Mn(4)CaO(5) oxidation in the protein environment, using a quantum mechanical/molecular mechanical approach and...
Autores principales: | Kawashima, Keisuke, Takaoka, Tomohiro, Kimura, Hiroki, Saito, Keisuke, Ishikita, Hiroshi |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2018
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5871790/ https://www.ncbi.nlm.nih.gov/pubmed/29593210 http://dx.doi.org/10.1038/s41467-018-03545-w |
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