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Supersonic propagation of lattice energy by phasons in fresnoite

Controlling the thermal energy of lattice vibrations separately from electrons is vital to many applications including electronic devices and thermoelectric energy conversion. To remove heat without shorting electrical connections, heat must be carried in the lattice of electrical insulators. Phonon...

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Autores principales: Manley, M. E., Stonaha, P. J., Abernathy, D. L., Chi, S., Sahul, R., Hermann, R. P., Budai, J. D.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5940883/
https://www.ncbi.nlm.nih.gov/pubmed/29739934
http://dx.doi.org/10.1038/s41467-018-04229-1
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author Manley, M. E.
Stonaha, P. J.
Abernathy, D. L.
Chi, S.
Sahul, R.
Hermann, R. P.
Budai, J. D.
author_facet Manley, M. E.
Stonaha, P. J.
Abernathy, D. L.
Chi, S.
Sahul, R.
Hermann, R. P.
Budai, J. D.
author_sort Manley, M. E.
collection PubMed
description Controlling the thermal energy of lattice vibrations separately from electrons is vital to many applications including electronic devices and thermoelectric energy conversion. To remove heat without shorting electrical connections, heat must be carried in the lattice of electrical insulators. Phonons are limited to the speed of sound, which, compared to the speed of electronic processes, puts a fundamental constraint on thermal management. Here we report a supersonic channel for the propagation of lattice energy in the technologically promising piezoelectric mineral fresnoite (Ba(2)TiSi(2)O(8)) using neutron scattering. Lattice energy propagates 2.8−4.3 times the speed of sound in the form of phasons, which are caused by an incommensurate modulation in the flexible framework structure of fresnoite. The phasons enhance the thermal conductivity by 20% at room temperature and carry lattice-energy signals at speeds beyond the limits of phonons.
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spelling pubmed-59408832018-05-10 Supersonic propagation of lattice energy by phasons in fresnoite Manley, M. E. Stonaha, P. J. Abernathy, D. L. Chi, S. Sahul, R. Hermann, R. P. Budai, J. D. Nat Commun Article Controlling the thermal energy of lattice vibrations separately from electrons is vital to many applications including electronic devices and thermoelectric energy conversion. To remove heat without shorting electrical connections, heat must be carried in the lattice of electrical insulators. Phonons are limited to the speed of sound, which, compared to the speed of electronic processes, puts a fundamental constraint on thermal management. Here we report a supersonic channel for the propagation of lattice energy in the technologically promising piezoelectric mineral fresnoite (Ba(2)TiSi(2)O(8)) using neutron scattering. Lattice energy propagates 2.8−4.3 times the speed of sound in the form of phasons, which are caused by an incommensurate modulation in the flexible framework structure of fresnoite. The phasons enhance the thermal conductivity by 20% at room temperature and carry lattice-energy signals at speeds beyond the limits of phonons. Nature Publishing Group UK 2018-05-08 /pmc/articles/PMC5940883/ /pubmed/29739934 http://dx.doi.org/10.1038/s41467-018-04229-1 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Manley, M. E.
Stonaha, P. J.
Abernathy, D. L.
Chi, S.
Sahul, R.
Hermann, R. P.
Budai, J. D.
Supersonic propagation of lattice energy by phasons in fresnoite
title Supersonic propagation of lattice energy by phasons in fresnoite
title_full Supersonic propagation of lattice energy by phasons in fresnoite
title_fullStr Supersonic propagation of lattice energy by phasons in fresnoite
title_full_unstemmed Supersonic propagation of lattice energy by phasons in fresnoite
title_short Supersonic propagation of lattice energy by phasons in fresnoite
title_sort supersonic propagation of lattice energy by phasons in fresnoite
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5940883/
https://www.ncbi.nlm.nih.gov/pubmed/29739934
http://dx.doi.org/10.1038/s41467-018-04229-1
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