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Excitonic Emission of Monolayer Semiconductors Near-Field Coupled to High-Q Microresonators
[Image: see text] We present quantum yield measurements of single layer WSe(2) (1L-WSe(2)) integrated with high-Q (Q > 10(6)) optical microdisk cavities, using an efficient (η > 90%) near-field coupling scheme based on a tapered optical fiber. Coupling of the excitonic emission is achieved by...
Autores principales: | , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2018
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5946169/ https://www.ncbi.nlm.nih.gov/pubmed/29624396 http://dx.doi.org/10.1021/acs.nanolett.8b00749 |
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author | Javerzac-Galy, Clément Kumar, Anshuman Schilling, Ryan D. Piro, Nicolas Khorasani, Sina Barbone, Matteo Goykhman, Ilya Khurgin, Jacob B. Ferrari, Andrea C. Kippenberg, Tobias J. |
author_facet | Javerzac-Galy, Clément Kumar, Anshuman Schilling, Ryan D. Piro, Nicolas Khorasani, Sina Barbone, Matteo Goykhman, Ilya Khurgin, Jacob B. Ferrari, Andrea C. Kippenberg, Tobias J. |
author_sort | Javerzac-Galy, Clément |
collection | PubMed |
description | [Image: see text] We present quantum yield measurements of single layer WSe(2) (1L-WSe(2)) integrated with high-Q (Q > 10(6)) optical microdisk cavities, using an efficient (η > 90%) near-field coupling scheme based on a tapered optical fiber. Coupling of the excitonic emission is achieved by placing 1L-WSe(2) in the evanescent cavity field. This preserves the microresonator high intrinsic quality factor (Q > 10(6)) below the bandgap of 1L-WSe(2). The cavity quantum yield is QY(c) ≈ 10(–3), consistent with operation in the broad emitter regime (i.e., the emission lifetime of 1L-WSe(2) is significantly shorter than the bare cavity decay time). This scheme can serve as a precise measurement tool for the excitonic emission of layered materials into cavity modes, for both in plane and out of plane excitation. |
format | Online Article Text |
id | pubmed-5946169 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2018 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-59461692018-05-13 Excitonic Emission of Monolayer Semiconductors Near-Field Coupled to High-Q Microresonators Javerzac-Galy, Clément Kumar, Anshuman Schilling, Ryan D. Piro, Nicolas Khorasani, Sina Barbone, Matteo Goykhman, Ilya Khurgin, Jacob B. Ferrari, Andrea C. Kippenberg, Tobias J. Nano Lett [Image: see text] We present quantum yield measurements of single layer WSe(2) (1L-WSe(2)) integrated with high-Q (Q > 10(6)) optical microdisk cavities, using an efficient (η > 90%) near-field coupling scheme based on a tapered optical fiber. Coupling of the excitonic emission is achieved by placing 1L-WSe(2) in the evanescent cavity field. This preserves the microresonator high intrinsic quality factor (Q > 10(6)) below the bandgap of 1L-WSe(2). The cavity quantum yield is QY(c) ≈ 10(–3), consistent with operation in the broad emitter regime (i.e., the emission lifetime of 1L-WSe(2) is significantly shorter than the bare cavity decay time). This scheme can serve as a precise measurement tool for the excitonic emission of layered materials into cavity modes, for both in plane and out of plane excitation. American Chemical Society 2018-04-06 2018-05-09 /pmc/articles/PMC5946169/ /pubmed/29624396 http://dx.doi.org/10.1021/acs.nanolett.8b00749 Text en Copyright © 2018 American Chemical Society This is an open access article published under a Creative Commons Attribution (CC-BY) License (http://pubs.acs.org/page/policy/authorchoice_ccby_termsofuse.html) , which permits unrestricted use, distribution and reproduction in any medium, provided the author and source are cited. |
spellingShingle | Javerzac-Galy, Clément Kumar, Anshuman Schilling, Ryan D. Piro, Nicolas Khorasani, Sina Barbone, Matteo Goykhman, Ilya Khurgin, Jacob B. Ferrari, Andrea C. Kippenberg, Tobias J. Excitonic Emission of Monolayer Semiconductors Near-Field Coupled to High-Q Microresonators |
title | Excitonic Emission
of Monolayer Semiconductors Near-Field
Coupled to High-Q Microresonators |
title_full | Excitonic Emission
of Monolayer Semiconductors Near-Field
Coupled to High-Q Microresonators |
title_fullStr | Excitonic Emission
of Monolayer Semiconductors Near-Field
Coupled to High-Q Microresonators |
title_full_unstemmed | Excitonic Emission
of Monolayer Semiconductors Near-Field
Coupled to High-Q Microresonators |
title_short | Excitonic Emission
of Monolayer Semiconductors Near-Field
Coupled to High-Q Microresonators |
title_sort | excitonic emission
of monolayer semiconductors near-field
coupled to high-q microresonators |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5946169/ https://www.ncbi.nlm.nih.gov/pubmed/29624396 http://dx.doi.org/10.1021/acs.nanolett.8b00749 |
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