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Excitonic Emission of Monolayer Semiconductors Near-Field Coupled to High-Q Microresonators

[Image: see text] We present quantum yield measurements of single layer WSe(2) (1L-WSe(2)) integrated with high-Q (Q > 10(6)) optical microdisk cavities, using an efficient (η > 90%) near-field coupling scheme based on a tapered optical fiber. Coupling of the excitonic emission is achieved by...

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Autores principales: Javerzac-Galy, Clément, Kumar, Anshuman, Schilling, Ryan D., Piro, Nicolas, Khorasani, Sina, Barbone, Matteo, Goykhman, Ilya, Khurgin, Jacob B., Ferrari, Andrea C., Kippenberg, Tobias J.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2018
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5946169/
https://www.ncbi.nlm.nih.gov/pubmed/29624396
http://dx.doi.org/10.1021/acs.nanolett.8b00749
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author Javerzac-Galy, Clément
Kumar, Anshuman
Schilling, Ryan D.
Piro, Nicolas
Khorasani, Sina
Barbone, Matteo
Goykhman, Ilya
Khurgin, Jacob B.
Ferrari, Andrea C.
Kippenberg, Tobias J.
author_facet Javerzac-Galy, Clément
Kumar, Anshuman
Schilling, Ryan D.
Piro, Nicolas
Khorasani, Sina
Barbone, Matteo
Goykhman, Ilya
Khurgin, Jacob B.
Ferrari, Andrea C.
Kippenberg, Tobias J.
author_sort Javerzac-Galy, Clément
collection PubMed
description [Image: see text] We present quantum yield measurements of single layer WSe(2) (1L-WSe(2)) integrated with high-Q (Q > 10(6)) optical microdisk cavities, using an efficient (η > 90%) near-field coupling scheme based on a tapered optical fiber. Coupling of the excitonic emission is achieved by placing 1L-WSe(2) in the evanescent cavity field. This preserves the microresonator high intrinsic quality factor (Q > 10(6)) below the bandgap of 1L-WSe(2). The cavity quantum yield is QY(c) ≈ 10(–3), consistent with operation in the broad emitter regime (i.e., the emission lifetime of 1L-WSe(2) is significantly shorter than the bare cavity decay time). This scheme can serve as a precise measurement tool for the excitonic emission of layered materials into cavity modes, for both in plane and out of plane excitation.
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spelling pubmed-59461692018-05-13 Excitonic Emission of Monolayer Semiconductors Near-Field Coupled to High-Q Microresonators Javerzac-Galy, Clément Kumar, Anshuman Schilling, Ryan D. Piro, Nicolas Khorasani, Sina Barbone, Matteo Goykhman, Ilya Khurgin, Jacob B. Ferrari, Andrea C. Kippenberg, Tobias J. Nano Lett [Image: see text] We present quantum yield measurements of single layer WSe(2) (1L-WSe(2)) integrated with high-Q (Q > 10(6)) optical microdisk cavities, using an efficient (η > 90%) near-field coupling scheme based on a tapered optical fiber. Coupling of the excitonic emission is achieved by placing 1L-WSe(2) in the evanescent cavity field. This preserves the microresonator high intrinsic quality factor (Q > 10(6)) below the bandgap of 1L-WSe(2). The cavity quantum yield is QY(c) ≈ 10(–3), consistent with operation in the broad emitter regime (i.e., the emission lifetime of 1L-WSe(2) is significantly shorter than the bare cavity decay time). This scheme can serve as a precise measurement tool for the excitonic emission of layered materials into cavity modes, for both in plane and out of plane excitation. American Chemical Society 2018-04-06 2018-05-09 /pmc/articles/PMC5946169/ /pubmed/29624396 http://dx.doi.org/10.1021/acs.nanolett.8b00749 Text en Copyright © 2018 American Chemical Society This is an open access article published under a Creative Commons Attribution (CC-BY) License (http://pubs.acs.org/page/policy/authorchoice_ccby_termsofuse.html) , which permits unrestricted use, distribution and reproduction in any medium, provided the author and source are cited.
spellingShingle Javerzac-Galy, Clément
Kumar, Anshuman
Schilling, Ryan D.
Piro, Nicolas
Khorasani, Sina
Barbone, Matteo
Goykhman, Ilya
Khurgin, Jacob B.
Ferrari, Andrea C.
Kippenberg, Tobias J.
Excitonic Emission of Monolayer Semiconductors Near-Field Coupled to High-Q Microresonators
title Excitonic Emission of Monolayer Semiconductors Near-Field Coupled to High-Q Microresonators
title_full Excitonic Emission of Monolayer Semiconductors Near-Field Coupled to High-Q Microresonators
title_fullStr Excitonic Emission of Monolayer Semiconductors Near-Field Coupled to High-Q Microresonators
title_full_unstemmed Excitonic Emission of Monolayer Semiconductors Near-Field Coupled to High-Q Microresonators
title_short Excitonic Emission of Monolayer Semiconductors Near-Field Coupled to High-Q Microresonators
title_sort excitonic emission of monolayer semiconductors near-field coupled to high-q microresonators
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5946169/
https://www.ncbi.nlm.nih.gov/pubmed/29624396
http://dx.doi.org/10.1021/acs.nanolett.8b00749
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