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Large positive linear magnetoresistance in the two-dimensional t(2g) electron gas at the EuO/SrTiO(3) interface

The development of novel nano-oxide spintronic devices would benefit greatly from interfacing with emergent phenomena at oxide interfaces. In this paper, we integrate highly spin-split ferromagnetic semiconductor EuO onto perovskite SrTiO(3) (001). A careful deposition of Eu metal by molecular beam...

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Autores principales: Kormondy, Kristy J., Gao, Lingyuan, Li, Xiang, Lu, Sirong, Posadas, Agham B., Shen, Shida, Tsoi, Maxim, McCartney, Martha R., Smith, David J., Zhou, Jianshi, Lev, Leonid L., Husanu, Marius-Adrian, Strocov, Vladimir N., Demkov, Alexander A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5955958/
https://www.ncbi.nlm.nih.gov/pubmed/29769572
http://dx.doi.org/10.1038/s41598-018-26017-z
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author Kormondy, Kristy J.
Gao, Lingyuan
Li, Xiang
Lu, Sirong
Posadas, Agham B.
Shen, Shida
Tsoi, Maxim
McCartney, Martha R.
Smith, David J.
Zhou, Jianshi
Lev, Leonid L.
Husanu, Marius-Adrian
Strocov, Vladimir N.
Demkov, Alexander A.
author_facet Kormondy, Kristy J.
Gao, Lingyuan
Li, Xiang
Lu, Sirong
Posadas, Agham B.
Shen, Shida
Tsoi, Maxim
McCartney, Martha R.
Smith, David J.
Zhou, Jianshi
Lev, Leonid L.
Husanu, Marius-Adrian
Strocov, Vladimir N.
Demkov, Alexander A.
author_sort Kormondy, Kristy J.
collection PubMed
description The development of novel nano-oxide spintronic devices would benefit greatly from interfacing with emergent phenomena at oxide interfaces. In this paper, we integrate highly spin-split ferromagnetic semiconductor EuO onto perovskite SrTiO(3) (001). A careful deposition of Eu metal by molecular beam epitaxy results in EuO growth via oxygen out-diffusion from SrTiO(3). This in turn leaves behind a highly conductive interfacial layer through generation of oxygen vacancies. Below the Curie temperature of 70 K of EuO, this spin-polarized two-dimensional t(2g) electron gas at the EuO/SrTiO(3) interface displays very large positive linear magnetoresistance (MR). Soft x-ray angle-resolved photoemission spectroscopy (SX-ARPES) reveals the t(2g) nature of the carriers. First principles calculations strongly suggest that Zeeman splitting, caused by proximity magnetism and oxygen vacancies in SrTiO(3), is responsible for the MR. This system offers an as-yet-unexplored route to pursue proximity-induced effects in the oxide two-dimensional t(2g) electron gas.
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spelling pubmed-59559582018-05-21 Large positive linear magnetoresistance in the two-dimensional t(2g) electron gas at the EuO/SrTiO(3) interface Kormondy, Kristy J. Gao, Lingyuan Li, Xiang Lu, Sirong Posadas, Agham B. Shen, Shida Tsoi, Maxim McCartney, Martha R. Smith, David J. Zhou, Jianshi Lev, Leonid L. Husanu, Marius-Adrian Strocov, Vladimir N. Demkov, Alexander A. Sci Rep Article The development of novel nano-oxide spintronic devices would benefit greatly from interfacing with emergent phenomena at oxide interfaces. In this paper, we integrate highly spin-split ferromagnetic semiconductor EuO onto perovskite SrTiO(3) (001). A careful deposition of Eu metal by molecular beam epitaxy results in EuO growth via oxygen out-diffusion from SrTiO(3). This in turn leaves behind a highly conductive interfacial layer through generation of oxygen vacancies. Below the Curie temperature of 70 K of EuO, this spin-polarized two-dimensional t(2g) electron gas at the EuO/SrTiO(3) interface displays very large positive linear magnetoresistance (MR). Soft x-ray angle-resolved photoemission spectroscopy (SX-ARPES) reveals the t(2g) nature of the carriers. First principles calculations strongly suggest that Zeeman splitting, caused by proximity magnetism and oxygen vacancies in SrTiO(3), is responsible for the MR. This system offers an as-yet-unexplored route to pursue proximity-induced effects in the oxide two-dimensional t(2g) electron gas. Nature Publishing Group UK 2018-05-16 /pmc/articles/PMC5955958/ /pubmed/29769572 http://dx.doi.org/10.1038/s41598-018-26017-z Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Kormondy, Kristy J.
Gao, Lingyuan
Li, Xiang
Lu, Sirong
Posadas, Agham B.
Shen, Shida
Tsoi, Maxim
McCartney, Martha R.
Smith, David J.
Zhou, Jianshi
Lev, Leonid L.
Husanu, Marius-Adrian
Strocov, Vladimir N.
Demkov, Alexander A.
Large positive linear magnetoresistance in the two-dimensional t(2g) electron gas at the EuO/SrTiO(3) interface
title Large positive linear magnetoresistance in the two-dimensional t(2g) electron gas at the EuO/SrTiO(3) interface
title_full Large positive linear magnetoresistance in the two-dimensional t(2g) electron gas at the EuO/SrTiO(3) interface
title_fullStr Large positive linear magnetoresistance in the two-dimensional t(2g) electron gas at the EuO/SrTiO(3) interface
title_full_unstemmed Large positive linear magnetoresistance in the two-dimensional t(2g) electron gas at the EuO/SrTiO(3) interface
title_short Large positive linear magnetoresistance in the two-dimensional t(2g) electron gas at the EuO/SrTiO(3) interface
title_sort large positive linear magnetoresistance in the two-dimensional t(2g) electron gas at the euo/srtio(3) interface
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC5955958/
https://www.ncbi.nlm.nih.gov/pubmed/29769572
http://dx.doi.org/10.1038/s41598-018-26017-z
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