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Optical near-field mapping of plasmonic nanostructures prepared by nanosphere lithography

We introduce a simple, fast, efficient and non-destructive method to study the optical near-field properties of plasmonic nanotriangles prepared by nanosphere lithography. Using a rectangular Fourier filter on the blurred signal together with filtering of the lower spatial frequencies to remove the...

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Autores principales: Kolhatkar, Gitanjali, Merlen, Alexandre, Zhang, Jiawei, Dab, Chahinez, Wallace, Gregory Q, Lagugné-Labarthet, François, Ruediger, Andreas
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Beilstein-Institut 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6009220/
https://www.ncbi.nlm.nih.gov/pubmed/29977686
http://dx.doi.org/10.3762/bjnano.9.144
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author Kolhatkar, Gitanjali
Merlen, Alexandre
Zhang, Jiawei
Dab, Chahinez
Wallace, Gregory Q
Lagugné-Labarthet, François
Ruediger, Andreas
author_facet Kolhatkar, Gitanjali
Merlen, Alexandre
Zhang, Jiawei
Dab, Chahinez
Wallace, Gregory Q
Lagugné-Labarthet, François
Ruediger, Andreas
author_sort Kolhatkar, Gitanjali
collection PubMed
description We introduce a simple, fast, efficient and non-destructive method to study the optical near-field properties of plasmonic nanotriangles prepared by nanosphere lithography. Using a rectangular Fourier filter on the blurred signal together with filtering of the lower spatial frequencies to remove the far-field contribution, the pure near-field contributions of the optical images were extracted. We performed measurements using two excitation wavelengths (532.1 nm and 632.8 nm) and two different polarizations. After the processing of the optical images, the distribution of hot spots can be correlated with the topography of the structures, as indicated by the presence of brighter spots at the apexes of the nanostructures. This technique is validated by comparison of the results to numerical simulations, where agreement is obtained, thereby confirming the near-field nature of the images. Our approach does not require any advanced equipment and we suggest that it could be applied to any type of sample, while keeping the measurement times reasonably short.
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spelling pubmed-60092202018-07-05 Optical near-field mapping of plasmonic nanostructures prepared by nanosphere lithography Kolhatkar, Gitanjali Merlen, Alexandre Zhang, Jiawei Dab, Chahinez Wallace, Gregory Q Lagugné-Labarthet, François Ruediger, Andreas Beilstein J Nanotechnol Full Research Paper We introduce a simple, fast, efficient and non-destructive method to study the optical near-field properties of plasmonic nanotriangles prepared by nanosphere lithography. Using a rectangular Fourier filter on the blurred signal together with filtering of the lower spatial frequencies to remove the far-field contribution, the pure near-field contributions of the optical images were extracted. We performed measurements using two excitation wavelengths (532.1 nm and 632.8 nm) and two different polarizations. After the processing of the optical images, the distribution of hot spots can be correlated with the topography of the structures, as indicated by the presence of brighter spots at the apexes of the nanostructures. This technique is validated by comparison of the results to numerical simulations, where agreement is obtained, thereby confirming the near-field nature of the images. Our approach does not require any advanced equipment and we suggest that it could be applied to any type of sample, while keeping the measurement times reasonably short. Beilstein-Institut 2018-05-23 /pmc/articles/PMC6009220/ /pubmed/29977686 http://dx.doi.org/10.3762/bjnano.9.144 Text en Copyright © 2018, Kolhatkar et al. https://creativecommons.org/licenses/by/4.0https://www.beilstein-journals.org/bjnano/termsThis is an Open Access article under the terms of the Creative Commons Attribution License (https://creativecommons.org/licenses/by/4.0), which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited. The license is subject to the Beilstein Journal of Nanotechnology terms and conditions: (https://www.beilstein-journals.org/bjnano/terms)
spellingShingle Full Research Paper
Kolhatkar, Gitanjali
Merlen, Alexandre
Zhang, Jiawei
Dab, Chahinez
Wallace, Gregory Q
Lagugné-Labarthet, François
Ruediger, Andreas
Optical near-field mapping of plasmonic nanostructures prepared by nanosphere lithography
title Optical near-field mapping of plasmonic nanostructures prepared by nanosphere lithography
title_full Optical near-field mapping of plasmonic nanostructures prepared by nanosphere lithography
title_fullStr Optical near-field mapping of plasmonic nanostructures prepared by nanosphere lithography
title_full_unstemmed Optical near-field mapping of plasmonic nanostructures prepared by nanosphere lithography
title_short Optical near-field mapping of plasmonic nanostructures prepared by nanosphere lithography
title_sort optical near-field mapping of plasmonic nanostructures prepared by nanosphere lithography
topic Full Research Paper
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6009220/
https://www.ncbi.nlm.nih.gov/pubmed/29977686
http://dx.doi.org/10.3762/bjnano.9.144
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